This thesis reports on the experimental investigation of controlled spin dependent interactions in a sample of ultracold Rubidium atoms trapped in a periodic optical potential. In such a situation, the most basic interaction between only two atoms at one common potential well, forming a micro laboratory for this atom pair, can be investigated. Spin dependent interactions between the atoms can lead to an intriguing time evolution of the system. In this work, we present two examples of such spin interaction induced dynamics. First, we have been able to observe and control a coherent spin changing interaction. Second, we have \nachieved to examine and manipulate an interaction\ninduced time evolution of the relative phase of a spin 1/2-system, both in the case of particle pairs and in the more general case of N interacting particles. The first part of this thesis elucidates the spin-changing interaction mechanism underlying many fascinating effects resulting from interacting spins at ultracold temperatures. This process changes the spin states of two colliding particles, while preserving total magnetization. If initial and final states have almost equal energy, this process is resonant and leads to large amplitude\noscillations between different spin states. The measured coupling parameters of such a process allow to precisely infer atomic scattering length differences, that e.g. determine the nature of the magnetic ground state of the hyperfine states in Rubidium.\nMoreover, a method to tune the spin oscillations at will based on the AC-Zeeman effect has been implemented. This allowed us to use resonant spin changing \ncollisions as a quantitative and non-destructive particle pair probe in the optical lattice. This led to a series of experiments shedding light on the Bosonic superfluid to Mott insulator transition.\nIn a second series of experiments we have been able to coherently manipulate the interaction induced time evolution of the relative phase in an ensemble of spin 1/2-systems. For two particles, interactions can lead to an entanglement oscillation of the particle pair. For the general case of N interacting particles, the ideal time evolution leads to the creation of spin squeezed states and even Schrödinger cat states. In the experiment we have been able to control the underlying\ninteractions by a Feshbach resonance. For particle pairs we could directly observe the entanglement oscillations. For the many particle case we have been able to observe and reverse the interaction induced dispersion of the relative phase.\nThe presented results demonstrate how correlated spin states can be engineered through \ncontrol of atomic interactions. Moreover, the results point towards the possibility to simulate quantum\nmagnetism phenomena with ultracold atoms in optical traps, and to realize and analyze many novel quantum spin states which have not been experimentally realized so far.
This thesis reports on the experimental investigation of controlled spin dependent interactions in a sample of ultracold Rubidium atoms trapped in a periodic optical potential. In such a situation, the most basic interaction between only two atoms at one common potential well, forming a micro laboratory for this atom pair, can be investigated. Spin dependent interactions between the atoms can lead to an intriguing time evolution of the system. In this work, we present two examples of such spin interaction induced dynamics. First, we have been able to observe and control a coherent spin changing interaction. Second, we have \nachieved to examine and manipulate an interaction\ninduced time evolution of the relative phase of a spin 1/2-system, both in the case of particle pairs and in the more general case of N interacting particles. The first part of this thesis elucidates the spin-changing interaction mechanism underlying many fascinating effects resulting from interacting spins at ultracold temperatures. This process changes the spin states of two colliding particles, while preserving total magnetization. If initial and final states have almost equal energy, this process is resonant and leads to large amplitude\noscillations between different spin states. The measured coupling parameters of such a process allow to precisely infer atomic scattering length differences, that e.g. determine the nature of the magnetic ground state of the hyperfine states in Rubidium.\nMoreover, a method to tune the spin oscillations at will based on the AC-Zeeman effect has been implemented. This allowed us to use resonant spin changing \ncollisions as a quantitative and non-destructive particle pair probe in the optical lattice. This led to a series of experiments shedding light on the Bosonic superfluid to Mott insulator transition.\nIn a second series of experiments we have been able to coherently manipulate the interaction induced time evolution of the relative phase in an ensemble of spin 1/2-systems. For two particles, interactions can lead to an entanglement oscillation of the particle pair. For the general case of N interacting particles, the ideal time evolution leads to the creation of spin squeezed states and even Schrödinger cat states. In the experiment we have been able to control the underlying\ninteractions by a Feshbach resonance. For particle pairs we could directly observe the entanglement oscillations. For the many particle case we have been able to observe and reverse the interaction induced dispersion of the relative phase.\nThe presented results demonstrate how correlated spin states can be engineered through \ncontrol of atomic interactions. Moreover, the results point towards the possibility to simulate quantum\nmagnetism phenomena with ultracold atoms in optical traps, and to realize and analyze many novel quantum spin states which have not been experimentally realized so far.
Advances in experiments on dilute ultracold atomic gases have given us access to highly tunable quantum systems. In particular, there have been substantial improvements in achieving different kinds of interaction between atoms. As a result, utracold atomic gases oer an ideal platform to simulate many-body phenomena in condensed matter physics, and engineer other novel phenomena that are a result of the exotic interactions produced between atoms. In this dissertation, I present a series of studies that explore the physics of dilute ultracold atomic gases in different settings. In each setting, I explore a different form of the inter-particle interaction. Motivated by experiments which induce artificial spin-orbit coupling for cold fermions, I explore this system in my first project. In this project, I propose a method to perform universal quantum computation using the excitations of interacting spin-orbit coupled fermions, in which effective p-wave interactions lead to the formation of a topological superfluid. Motivated by experiments which explore the physics of exotic interactions between atoms trapped inside optical cavities, I explore this system in a second project. I calculate the phase diagram of lattice bosons trapped in an optical cavity, where the cavity modes mediates effective global range checkerboard interactions between the atoms. I compare this phase diagram with one that was recently measured experimentally. In two other projects, I explore quantum simulation of condensed matter phenomena due to spin-dependent interactions between particles. I propose a method to produce tunable spin-dependent interactions between atoms, using an optical Feshbach resonance. In one project, I use these spin-dependent interactions in an ultracold Bose-Fermi system, and propose a method to produce the Kondo model. I propose an experiment to directly observe the Kondo effect in this system. In another project, I propose using lattice bosons with a large hyperfine spin, which have Feshbach-induced spin-dependent interactions, to produce a quantum dimer model. I propose an experiment to detect the ground state in this system. In a final project, I develop tools to simulate the dynamics of fermionic superfluids in which fermions interact via a short-range interaction.
We report on the observation of coherent, purely collisionally driven spin dynamics of neutral atoms in an optical lattice. For high lattice depths, atom pairs confined to the same lattice site show weakly damped Rabi-type oscillations between two-particle Zeeman states of equal magnetization, induced by spin-changing collisions. Moreover, measurement of the oscillation frequency allows for precise determination of the spin-changing collisional coupling strengths, which are directly related to fundamental scattering lengths describing interatomic collisions at ultracold temperatures.
Ultracold atoms in optical lattices provide a highly controllable environment for the clean experimental realization of various model Hamiltonians from condensed matter and statistical physics. For example, the two-component Bose-Hubbard model, which reduces to an anisotropic spin-1/2 Heisenberg model in a certain limit and thus allows for the study of quantum magnetism, can be implemented by using bosons with two different internal states that couple differently to an optical lattice potential. In this thesis, I present our first experiments with two-component hyperfine-state mixtures of ultracold 87Rb atoms in a state-dependent optical lattice, both in the strongly correlated regime and in the context of nonlinear atom optics. For the production of 87Rb Bose-Einstein condensates we have developed a moving-coil transporter apparatus featuring a magnetic TOP trap which serves as a 'phase-space funnel' to load a crossed optical dipole trap. The apparatus further incorporates a three-dimensional optical lattice setup with simultaneously usable hyperfine state-dependent and state-independent lattice beams of different spacing along the vertical axis. Internal state control is performed via rf and microwave Rabi pulses and Landau-Zener sweeps. As a first step towards studying strongly correlated two-component mixtures, we have realized a state-selective superfluid-to-Mott insulator transition, where one component enters the Mott insulator regime, while the other one stays superfluid. Using the state-dependent lattice we can tune the second component's properties from highly superfluid to strongly localized. At both extremes we find a reduction of the coherence of the primary component, i.e. a shift of the Mott transition to smaller values of the ratio U/t of interaction to tunneling. We ascribe this to a polaron-like dressing on the one hand, and a 'quantum emulsion' causing a disordered atomic background potential on the other hand. Further, we have observed and studied four-wave mixing of two-component matter waves. Using state-selective Kapitza-Dirac diffraction of a two-component BEC, we prepare seed and pump modes differing both in momentum and internal state. A novel collinear four-wave mixing process then populates the initially empty output modes. While this process can complicate studies of bosonic mixtures loaded into state-dependent optical lattices, it might prove useful for possible applications in quantum atom optics. | Ultracold atoms in optical lattices provide a highly controllable environment for the clean experimental realization of various model Hamiltonians from condensed matter and statistical physics. For example, the two-component Bose-Hubbard model, which reduces to an anisotropic spin-1/2 Heisenberg model in a certain limit and thus allows for the study of quantum magnetism, can be implemented by using bosons with two different internal states that couple differently to an optical lattice potential. In this thesis, I present our first experiments with two-component hyperfine-state mixtures of ultracold 87Rb atoms in a state-dependent optical lattice, both in the strongly correlated regime and in the context of nonlinear atom optics. For the production of 87Rb Bose-Einstein condensates we have developed a moving-coil transporter apparatus featuring a magnetic TOP trap which serves as a 'phase-space funnel' to load a crossed optical dipole trap. The apparatus further incorporates a three-dimensional optical lattice setup with simultaneously usable hyperfine state-dependent and state-independent lattice beams of different spacing along the vertical axis. Internal state control is performed via rf and microwave Rabi pulses and Landau-Zener sweeps. As a first step towards studying strongly correlated two-component mixtures, we have realized a state-selective superfluid-to-Mott insulator transition, where one component enters the Mott insulator regime, while the other one stays superfluid. Using the state-dependent lattice we can tune the second component's properties from highly superfluid to strongly localized. At both extremes we find a reduction of the coherence of the primary component, i.e. a shift of the Mott transition to smaller values of the ratio U/t of interaction to tunneling. We ascribe this to a polaron-like dressing on the one hand, and a 'quantum emulsion' causing a disordered atomic background potential on the other hand. Further, we have observed and studied four-wave mixing of two-component matter waves. Using state-selective Kapitza-Dirac diffraction of a two-component BEC, we prepare seed and pump modes differing both in momentum and internal state. A novel collinear four-wave mixing process then populates the initially empty output modes. While this process can complicate studies of bosonic mixtures loaded into state-dependent optical lattices, it might prove useful for possible applications in quantum atom optics. | 110 pages
Optical lattices make it possible to trap and coherently control large ensembles of ultracold atoms. They provide the possibility to create lattice potentials that mimic the structure of solid-state systems, and to control these potentials dynamically. In this thesis, we study how dynamical manipulations of the lattice geometry can be used to perform different tasks, ranging from quantum information processing to the creation of diatomic molecules. We first examine the dynamical properties of ultracold atoms trapped in a lattice whose periodicity is dynamically doubled. We derive a model describing the dynamics of the atoms during this process, and compute the different interaction parameters of this model. We investigate different ways of using this lattice manipulation to optimise the initialisation time of a Mott-insulating state with one atom per site, and provide a scaling law related to the interaction parameters of the system. We go on to show that entangling operations between the spin of adjacent atoms are realisable with optical lattices forming arrays of double-well potentials. We study the creation of a lattice containing a spin-encoded Bell-pair in each double-well, and show that resilient, highly-entangled many-body states are realisable using lattice manipulations. We show that the creation of cluster-like states encoded on Bell-pairs can be achieved using these systems, and we provide measurement networks that allow the execution of quantum algorithms while maintaining intact the resilience of the system. Finally, we investigate the possibility to create a diatomic molecular state and simulate Fermi systems via the excitation to Rydberg levels of ground-state atoms trapped in optical lattices. We develop a method based on symbolical manipulations to compute the interaction parameters between highly-excited electrons, and evaluate them for different electronic configurations. We use these parameters to investigate the existence of diatomic molecular states with equilibrium distances comparable to typical lattice spacings. Considering the possibility to excite atoms trapped in an optical lattice to Rydberg levels such that the electronic cloud of neighbouring atoms overlap, we propose a model describing their interactions and compute its parameters. If such systems were realised, they would allow the simulation of Fermi systems at a temperature much below the Fermi temperature, thus enabling the observation of quantum phenomena hitherto inaccessible with current technology.
In this thesis we investigate strongly-correlated states of ultracold bosonic atoms in rotating ring lattices and arrays of double-well potentials. In the first part of the thesis, we study the tunneling dynamics of ultracold bosons in double-well potentials. In the non-interacting limit single-particle transitions dominate, while in the interaction-dominated regime correlated tunneling of all particles prevails. At intermediate times of the many-particle flopping process correlated states occur, but the timescales of these processes increase dramatically with the number of particles. Using an array of double-well potentials, a large number of such few-particle superposition states can be produced in parallel. In the second part of the thesis, we study the effects of rotation on ultracold bosons confined to one-dimensional ring lattices. We find that at commensurate filling there exists a critical rotation frequency, at which the ground state of the weakly-interacting gas is fragmented into a macroscopic superposition of different quasi-momentum states. We demonstrate that the generation of such superposition states using slightly non-uniform ring lattices has several practical advantages. Moreover, we show that different quasi-momentum states can be distinguished in time-of-flight absorption imaging and propose to probe correlations via the many-body oscillations induced by a sudden change in the rotation frequency. Finally, we compare these macroscopic superposition states to those occurring in superconducting quantum interference devices. In the third part of the thesis, we demonstrate the creation of entangled states with ultracold bosonic atoms by dynamical manipulation of the shape of the lattice potential. To this end, we consider an optical superlattice that allows both the splitting of each site into a double-well potential and the variation of the height of the potential barrier between the sites. We show how to use this array of double-well potentials to perform entangling operations between neighboring qubits encoded on the Zeeman levels of the atoms. As one possible application, we present a method of realizing a resource state for measurement-based quantum computation via Bell-pair measurements. In the final part of the thesis, we study ultracold bosons on a two-dimensional square lattice in the presence of an effective magnetic field and point out a couple of features this system has in common with ultracold bosons in one-dimensional rotating ring lattices.
In this habilitation-thesis a collection of 14 experiments is presented. In these experiments we have developed and used novel techniques to control ultracold gases on the quantum level. In brief, Bose-Einstein condensates (BEC) and degenerate Fermi gases of laser-cooled alkali atoms are subjected to specially designed optical and magnetic fields. The fields influence in a coherent way the behavior, properties and dynamics of the gases. On this basis we developed tools to prepare, coherently manipulate, and analyze pre-defined quantum states. With this high level of control, it was possible to investigate interesting physics phenomena, and we were able to achieve several breakthroughs in the field of ultracold atoms. Highlights of our experimental results include the demonstration of phase engineering of a BEC wavefunction where we created solitons in a BEC and studied their propagation. In another experiment we constructed a spatially resolved matter wave interferometer with which we mapped out the phase distribution on a condensate. Illuminating the BEC with a periodic pattern, i.e. an optical lattice, allowed us to study solid states physics phenomena. In a second set of experiments we demonstrated optically tuning of the interaction between atoms with optical Feshbach resonances. Employing either magnetically tunable Feshbach resonances or laser radiation, we were able to produce ground state molecules in well defined quantum states. This led to the production of the first molecular BEC. By tuning the coupling of atom pairs in a Fermi gas of atoms, we could for the first time investigate the so-called BEC-BCS crossover which describes the continuous change from a BEC superfluid to a Bardeen-Cooper Schrieffer (BCS) superfluid. Due to the excellent control on the quantum level, the developed cold atom techniques open up intriguing prospects for future applications and experiments. They represent a general tool box to investigate fundamental physical phenomena in a pure and undisturbed environment. In the future, cold atoms might serve as a testing ground for fundamental theories or as quantum simulators for complex systems.