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arXiv:cond-mat/0404116 · Physical Review Letters

Spectroscopy of Superfluid Pairing in Atomic Fermi Gases

Hans Peter Büchler, P. Zoller, W. Zwerger

Published Aug 16, 2004• 50 citations
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Abstract

We study the dynamic structure factor for density and spin within the crossover from BCS superfluidity of atomic fermions to the Bose-Einstein condensation of molecules. Both structure factors are experimentally accessible via Bragg spectroscopy and allow for the identification of the pairing mechanism: the spin structure factor allows for the determination of the two particle gap, while the collective sound mode in the density structure reveals the superfluid state.

DOI
10.1103/physrevlett.93.080401

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We study the dynamic structure factor for density and spin within the crossover from BCS superfluidity of atomic fermions to the Bose-Einstein condensation of molecules. Both structure factors are experimentally accessible via Bragg spectroscopy and allow for the identification of the pairing mechanism: the spin structure factor allows for the determination of the two particle gap, while the collective sound mode in the density structure reveals the superfluid state.
We theoretically investigate the dynamic structure factor of a strongly interacting Fermi gas at the crossover from Bardeen–Cooper–Schrieffer superfluids to Bose–Einstein condensates, by developing an improved random phase approximation within the framework of a density functional theory (DFT)—the so-called superfluid local density approximation. Compared with the previous random-phase-approximation studies based on the standard Bogoliubov–de Gennes equations, the use of the DFT greatly improves the accuracy of the equation of state at the crossover, and leads to a better description of both collective Bogoliubov-Anderson-Goldstone phonon mode and single-particle fermionic excitations at small transferred momentum. Near unitarity, where the s -wave scattering length diverges, we show that the single-particle excitations start to significantly contribute to the spectrum of dynamic structure factor once the frequency is above a threshold of the energy gap at . The sharp rise in the spectrum at this threshold can be utilized to measure the pairing gap Δ. Together with the sound velocity determined from the phonon branch, the dynamic structure factor provides us some key information of the crossover Fermi superfluid. Our predictions could be examined in experiments with 6 Li or 40 K atoms using Bragg spectroscopy.
We present a comprehensive study of the Bose-Einstein condensate to Bardeen-Cooper-Schrieffer (BEC-BCS) crossover in fermionic 6Li using Bragg spectroscopy. A smooth transition from molecular to atomic spectra is observed with a clear signature of pairing at and above unitarity. These spectra probe the dynamic and static structure factors of the gas and provide a direct link to two-body correlations. We have characterized these correlations and measured their density dependence across the broad Feshbach resonance at 834 G.
Ultracold atomic gases are a powerful tool to experimentally study strongly correlated quantum many-body systems. In particular, ultracold Fermi gases with tunable interactions have allowed to realize the famous BEC-BCS crossover from a Bose-Einstein condensate (BEC) of molecules to a Bardeen-Cooper-Schrieffer (BCS) superfluid of weakly bound Cooper pairs. However, large parts of the excitation spectrum of fermionic superfluids in the BEC-BCS crossover are still unexplored. In this work, we use Bragg spectroscopy to measure the full momentum-resolved low-energy excitation spectrum of strongly interacting ultracold Fermi gases. This enables us to directly observe the smooth transformation from a bosonic to a fermionic superfluid that takes place in the BEC-BCS crossover. We also use our spectra to determine the evolution of the superfluid gap and find excellent agreement with previous experiments and self-consistent T-matrix calculations both in the BEC and crossover regime. However, toward the BCS regime a calculation that includes the effects of particle-hole correlations shows better agreement with our data.
Bragg spectroscopy shows the evolution of gapless Goldstone modes and single-particle-like excitations in an atomic Fermi superfluid as it crosses from a Bardeen–Cooper–Schrieffer superfluid to the Bose–Einstein condensate regime. Spontaneous symmetry breaking is a central paradigm of elementary particle physics1, magnetism2, superfluidity3 and superconductivity4. According to Goldstone’s theorem, phase transitions that break continuous symmetries lead to the existence of gapless excitations in the long-wavelength limit5. These Goldstone modes can become the dominant low-energy excitation, showing that symmetry breaking has a profound impact on the physical properties of matter. Here, we present a comprehensive study of the elementary excitations in a homogeneous strongly interacting Fermi gas through the crossover from a Bardeen–Cooper–Schrieffer (BCS) superfluid to a Bose–Einstein condensate (BEC) of molecules using two-photon Bragg spectroscopy. The spectra exhibit a discrete Goldstone mode, associated with the broken-symmetry superfluid phase, as well as pair-breaking single-particle excitations. Our techniques yield a direct determination of the superfluid pairing gap and speed of sound in close agreement with strong-coupling theories.
We propose a Bragg spectroscopy experiment to measure the onset of superfluid pairing in ultracold trapped Fermi gases. In particular, we study two-component Fermi gases in the weak coupling BCS and Bose Einstein condensation limits as well as in the strong coupling unitarity limit. The low-temperature Bragg spectrum exhibits a gap directly related to the pair-breaking energy. Furthermore, the Bragg spectrum has a large maximum just below the critical temperature when the gas is superfluid in the BCS limit. In the unitarity regime, we show how the pseudogap in the normal phase leads to a significant suppression of the low-frequency Bragg spectrum.
The superfluid, pair condensed spin-1/2 Fermi gases are supposed to exhibit at nonzero wave vector a still unobserved collective excitation mode in their pair-breaking continuum. Using BCS theory at zero temperature and in the long wavelength limit, we predict that this mode is quantitatively observable (in frequency, width and spectral weight) in the response of a cold atom gas to a laser Bragg excitation, if one measures the perturbation induced on the order parameter modulus rather than on the density.