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arXiv:1707.00406 · Nature Physics

Goldstone mode and pair-breaking excitations in atomic Fermi superfluids

Sascha Hoinka, Paul Dyke, Marcus Lingham, J. J. Kinnunen, Georg M. Bruun, Chris J. Vale

Published Jun 26, 2017• 106 citations
arXivHTMLPDF

Abstract

Bragg spectroscopy shows the evolution of gapless Goldstone modes and single-particle-like excitations in an atomic Fermi superfluid as it crosses from a Bardeen–Cooper–Schrieffer superfluid to the Bose–Einstein condensate regime. Spontaneous symmetry breaking is a central paradigm of elementary particle physics1, magnetism2, superfluidity3 and superconductivity4. According to Goldstone’s theorem, phase transitions that break continuous symmetries lead to the existence of gapless excitations in the long-wavelength limit5. These Goldstone modes can become the dominant low-energy excitation, showing that symmetry breaking has a profound impact on the physical properties of matter. Here, we present a comprehensive study of the elementary excitations in a homogeneous strongly interacting Fermi gas through the crossover from a Bardeen–Cooper–Schrieffer (BCS) superfluid to a Bose–Einstein condensate (BEC) of molecules using two-photon Bragg spectroscopy. The spectra exhibit a discrete Goldstone mode, associated with the broken-symmetry superfluid phase, as well as pair-breaking single-particle excitations. Our techniques yield a direct determination of the superfluid pairing gap and speed of sound in close agreement with strong-coupling theories.

DOI
10.1038/nphys4187

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Bragg spectroscopy shows the evolution of gapless Goldstone modes and single-particle-like excitations in an atomic Fermi superfluid as it crosses from a Bardeen–Cooper–Schrieffer superfluid to the Bose–Einstein condensate regime. Spontaneous symmetry breaking is a central paradigm of elementary particle physics1, magnetism2, superfluidity3 and superconductivity4. According to Goldstone’s theorem, phase transitions that break continuous symmetries lead to the existence of gapless excitations in the long-wavelength limit5. These Goldstone modes can become the dominant low-energy excitation, showing that symmetry breaking has a profound impact on the physical properties of matter. Here, we present a comprehensive study of the elementary excitations in a homogeneous strongly interacting Fermi gas through the crossover from a Bardeen–Cooper–Schrieffer (BCS) superfluid to a Bose–Einstein condensate (BEC) of molecules using two-photon Bragg spectroscopy. The spectra exhibit a discrete Goldstone mode, associated with the broken-symmetry superfluid phase, as well as pair-breaking single-particle excitations. Our techniques yield a direct determination of the superfluid pairing gap and speed of sound in close agreement with strong-coupling theories.
In phase transitions, spontaneous symmetry breaking results in a nonzero order parameter and two collective excitations: the Goldstone and the amplitude mode. These modes, which define key properties of superconductors and fermionic superfluids, are well understood in homogeneous systems. However, their behavior under strong confinement remains largely unexplored, particularly when their excitation energy becomes comparable to the imposed discrete level spacing. In this scenario, hybridization between different collective modes is expected to take place. Here, we show how the amplitude mode hybridizes with a spatial mode in a confined fermionic superfluid. Using lattice modulation spectroscopy, we observe the evolution of the mode throughout the entire crossover from the Bardeen-Cooper-Schrieffer (BCS) state to Bose-Einstein condensation (BEC) of molecules. In the BCS regime, the excitation energy is located at twice the pairing gap, then gradually becomes an in-gap excitation in the strongly correlated regime. Further to the BEC limit, the excitation energy approaches twice the level spacing. The spectral weight of this mode vanishes when approaching the superfluid critical temperature. Our experimental results are in excellent agreement with an effective field theory, providing strong evidence that amplitude oscillations hybridize with and eventually transform into breathing oscillations of the order parameter. The strong modification of the excitation spectrum reveals how confinement and finite-size effects impact fundamental modes of symmetry-broken states.
Ultracold atomic gases are a powerful tool to experimentally study strongly correlated quantum many-body systems. In particular, ultracold Fermi gases with tunable interactions have allowed to realize the famous BEC-BCS crossover from a Bose-Einstein condensate (BEC) of molecules to a Bardeen-Cooper-Schrieffer (BCS) superfluid of weakly bound Cooper pairs. However, large parts of the excitation spectrum of fermionic superfluids in the BEC-BCS crossover are still unexplored. In this work, we use Bragg spectroscopy to measure the full momentum-resolved low-energy excitation spectrum of strongly interacting ultracold Fermi gases. This enables us to directly observe the smooth transformation from a bosonic to a fermionic superfluid that takes place in the BEC-BCS crossover. We also use our spectra to determine the evolution of the superfluid gap and find excellent agreement with previous experiments and self-consistent T-matrix calculations both in the BEC and crossover regime. However, toward the BCS regime a calculation that includes the effects of particle-hole correlations shows better agreement with our data.
The continuous crossover between a Bardeen-Cooper-Schrieffer (BCS)-type superfluid of fermion pairs and a Bose-Einstein condensate (BEC) of tightly bound bosonic molecules can be attributed to the spontaneous breaking of global U(1)U(1)U(1) gauge symmetry which underlies both quantum condensation phenomena. Recently much attention has been paid to this problem, since Feshbach resonances allow for an experimental implementation of crossover physics in cold fermion gases. The strong interactions close to resonance call for an analysis beyond Mean Field Theory. We develop a systematic functional integral approach for the description of this phenomenon. Starting from a Yukawa-type atom-molecule model, a symmetry analysis allows to both construct the equation of state and to classify the thermodynamic phases in a unified way. The onset of superfluidity is signalled by the emergence of a massless Goldstone mode associated with the broken continuous U(1) symmetry. Beyond Mean Field, we include fluctuations of the molecule field self-consistently via the solution of suitable Schwinger-Dyson equations. The phase diagram is computed, and a variety of universal features are established. A new form of crossover from an exactly solvable narrow resonance limit to broad resonances or pointlike interactions is found. At low temperature our results agree well with quantum Monte Carlo simulations and recent experiments. Our approach is further developed in the frame of functional renormalization group equations. While the effective bosonic theory in the BEC regime shows the characteristics of a Bogoliubov theory for small temperatures, the phase transition is of second order.
We present a comprehensive study of the Bose-Einstein condensate to Bardeen-Cooper-Schrieffer (BEC-BCS) crossover in fermionic 6Li using Bragg spectroscopy. A smooth transition from molecular to atomic spectra is observed with a clear signature of pairing at and above unitarity. These spectra probe the dynamic and static structure factors of the gas and provide a direct link to two-body correlations. We have characterized these correlations and measured their density dependence across the broad Feshbach resonance at 834 G.
We discuss the derivation of a low-energy effective field theory of phase (Goldstone) and amplitude (Higgs) modes of the pairing field from a microscopic theory of attractive fermions. The coupled equations for Goldstone and Higgs fields are critically analyzed in the Bardeen–Cooper–Schrieffer (BCS)-to-Bose–Einstein condensate (BEC) crossover—both in three spatial dimensions and in two spatial dimensions. The crucial role of pair fluctuations is investigated, and the beyond-mean-field Gaussian theory of the BCS–BEC crossover is compared with available experimental data of the two-dimensional ultracold Fermi superfluid.
We theoretically investigate the dynamic structure factor of a strongly interacting Fermi gas at the crossover from Bardeen–Cooper–Schrieffer superfluids to Bose–Einstein condensates, by developing an improved random phase approximation within the framework of a density functional theory (DFT)—the so-called superfluid local density approximation. Compared with the previous random-phase-approximation studies based on the standard Bogoliubov–de Gennes equations, the use of the DFT greatly improves the accuracy of the equation of state at the crossover, and leads to a better description of both collective Bogoliubov-Anderson-Goldstone phonon mode and single-particle fermionic excitations at small transferred momentum. Near unitarity, where the s -wave scattering length diverges, we show that the single-particle excitations start to significantly contribute to the spectrum of dynamic structure factor once the frequency is above a threshold of the energy gap at . The sharp rise in the spectrum at this threshold can be utilized to measure the pairing gap Δ. Together with the sound velocity determined from the phonon branch, the dynamic structure factor provides us some key information of the crossover Fermi superfluid. Our predictions could be examined in experiments with 6 Li or 40 K atoms using Bragg spectroscopy.