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arXiv:0809.2145 · Physical Review Letters

Bragg Spectroscopy of a Strongly Interacting Fermi Gas

G. Veeravalli, E. D. Kuhnle, Paul Dyke, Chris J. Vale

Published Dec 19, 2008• 181 citations
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Abstract

We present a comprehensive study of the Bose-Einstein condensate to Bardeen-Cooper-Schrieffer (BEC-BCS) crossover in fermionic 6Li using Bragg spectroscopy. A smooth transition from molecular to atomic spectra is observed with a clear signature of pairing at and above unitarity. These spectra probe the dynamic and static structure factors of the gas and provide a direct link to two-body correlations. We have characterized these correlations and measured their density dependence across the broad Feshbach resonance at 834 G.

DOI
10.1103/physrevlett.101.250403

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We present a comprehensive study of the Bose-Einstein condensate to Bardeen-Cooper-Schrieffer (BEC-BCS) crossover in fermionic 6Li using Bragg spectroscopy. A smooth transition from molecular to atomic spectra is observed with a clear signature of pairing at and above unitarity. These spectra probe the dynamic and static structure factors of the gas and provide a direct link to two-body correlations. We have characterized these correlations and measured their density dependence across the broad Feshbach resonance at 834 G.
The pairing of fermionic particles is an essential ingredient of superconductivity and of the superfluidity of 3He. While such phenomena are accurately described by BCS theory in the limit of weak pairing strength, a complete understanding remains elusive when pairing strength is increased, such as in high temperature superconductors. We create ultracold gases of trapped fermionic 6Li atoms, through which we directly observe fermionic pairing. In our system, there are no impurities whatsoever, and parameters such as the number and temperature of the trapped atoms are precisely and independently controlled. In addition, a Feshbach resonance enables the continuous tuning of interaction strength and sign between the paired atoms. This control allows us to observe the smooth crossover of a molecular Bose Einstein condensate (MBEC) to a superfluid of weakly interacting Cooper pairs. With these tools, we have performed several fundamental measurements of pairing in fermionic systems.\nWe use optical molecular spectroscopy to precisely measure the closed-channel contribution to the many body state of paired 6Li atoms within a broad Feshbach resonance. The magnitude of this contribution is small, and supports the concept of universality for the description of broad Feshbach resonances. Moreover, the dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover, and for the first time, into the weakly interacting BCS regime.\nWe also prepare a polarized Fermi gas with unequal numbers of two spin states of 6Li atoms. The real-space densities of the polarized, strongly-interacting, two-component Fermi gas reveal two low temperature regimes. At the lowest temperatures, the gas separates into a phase with a uniformly paired superfluid core surrounded by a shell of normal, unpaired atoms. This phase separation is accompanied by a spatial deformation of the core. At higher temperatures, the uniformly paired core persists, though it does not deform. This temperature dependence is consistent with a tri-critical point in the phase diagram. These measurements of pairing in a polarized Fermi gas are relevant to predictions of exotic phases of quark matter and magnetized superconductors.
Ultracold atomic gases are a powerful tool to experimentally study strongly correlated quantum many-body systems. In particular, ultracold Fermi gases with tunable interactions have allowed to realize the famous BEC-BCS crossover from a Bose-Einstein condensate (BEC) of molecules to a Bardeen-Cooper-Schrieffer (BCS) superfluid of weakly bound Cooper pairs. However, large parts of the excitation spectrum of fermionic superfluids in the BEC-BCS crossover are still unexplored. In this work, we use Bragg spectroscopy to measure the full momentum-resolved low-energy excitation spectrum of strongly interacting ultracold Fermi gases. This enables us to directly observe the smooth transformation from a bosonic to a fermionic superfluid that takes place in the BEC-BCS crossover. We also use our spectra to determine the evolution of the superfluid gap and find excellent agreement with previous experiments and self-consistent T-matrix calculations both in the BEC and crossover regime. However, toward the BCS regime a calculation that includes the effects of particle-hole correlations shows better agreement with our data.
We report measurements showing the universal behaviour of the static structure factor and both the temperature and interaction dependence of pair correlations in a strongly interacting Fermi gas. We utilize Bragg spectroscopy to obtain the static structure factor by recording excitation spectra of trapped clouds of ultracold 6Li atoms. Our results show clear evidence of strong short-range pair correlations above the critical temperature for superfluidity through the BEC-BCS crossover and agree well with theoretical calculations.
We present an overview of our recent measurements on the crossover from a Bose‐Einstein condensate of molecules to a Bardeen‐Cooper‐Schrieffer superfluid. The experiments are performed on a two‐component spin‐mixture of 6Li atoms, where a Feshbach resonance serves as the experimental key to tune the s‐wave scattering length and thus to explore the various interaction regimes. In the BEC‐BCS crossover, we have characterized the interaction energy by measuring the size of the trapped gas, we have studied collective excitation modes, and we have observed the pairing gap. Our observations provide strong evidence for superfluidity in the strongly interacting Fermi gas.
Theoretical predictions for the dynamic structure factor of a harmonically trapped Fermi superfluid near the Bose-Einstein condensate--Bardeen-Cooper-Schrieffer (BEC-BCS) crossover are compared with recent Bragg spectroscopy measurements at large transferred momenta. The calculations are based on a random-phase (or time-dependent Hartree-Fock-Gorkov) approximation generalized to the strongly interacting regime. Excellent agreement with experimental spectra at low temperatures is obtained, with no free parameters. Theoretical predictions for zero-temperature static structure factor are also found to agree well with the experimental results and independent theoretical calculations based on the exact Tan relations. The temperature dependence of the structure factors at unitarity is predicted.
Bragg spectroscopy shows the evolution of gapless Goldstone modes and single-particle-like excitations in an atomic Fermi superfluid as it crosses from a Bardeen–Cooper–Schrieffer superfluid to the Bose–Einstein condensate regime. Spontaneous symmetry breaking is a central paradigm of elementary particle physics1, magnetism2, superfluidity3 and superconductivity4. According to Goldstone’s theorem, phase transitions that break continuous symmetries lead to the existence of gapless excitations in the long-wavelength limit5. These Goldstone modes can become the dominant low-energy excitation, showing that symmetry breaking has a profound impact on the physical properties of matter. Here, we present a comprehensive study of the elementary excitations in a homogeneous strongly interacting Fermi gas through the crossover from a Bardeen–Cooper–Schrieffer (BCS) superfluid to a Bose–Einstein condensate (BEC) of molecules using two-photon Bragg spectroscopy. The spectra exhibit a discrete Goldstone mode, associated with the broken-symmetry superfluid phase, as well as pair-breaking single-particle excitations. Our techniques yield a direct determination of the superfluid pairing gap and speed of sound in close agreement with strong-coupling theories.