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arXiv:cond-mat/0402663 · Physical Review B

The Luther-Emery liquid: Spin gap and anomalous flux period

Alexander Seidel, D. H. Lee

Published Jan 14, 2005• 27 citations
arXivHTMLPDF

Abstract

We study the dependence of the ground state energy on an applied Aharonov-Bohm flux $\ensuremath{\Phi}$ for the Luttinger model with large momentum scattering. Employing the method of finite size bosonization, we show that for systems with a spin gap but with gapless charge degrees of freedom, the ground state energy has an exact period of $hc∕2e$, i.e., half a flux quantum, in the limit of large system size $L$. Finite size corrections are found to vanish exponentially in $L$. This behavior is contrasted to that of the spin gapless case, for both even and odd particle number. Generalizations to finite temperature are also discussed.

DOI
10.1103/physrevb.71.045113

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We study the dependence of the ground state energy on an applied Aharonov-Bohm flux \ensuremathΦ\ensuremath{\Phi}\ensuremathΦ for the Luttinger model with large momentum scattering. Employing the method of finite size bosonization, we show that for systems with a spin gap but with gapless charge degrees of freedom, the ground state energy has an exact period of hc∕2ehc∕2ehc∕2e, i.e., half a flux quantum, in the limit of large system size LLL. Finite size corrections are found to vanish exponentially in LLL. This behavior is contrasted to that of the spin gapless case, for both even and odd particle number. Generalizations to finite temperature are also discussed.
The one-dimensional Holstein model and its generalizations have been studied extensively to understand the effects of electron-phonon interaction. The half-filled case is of particular interest, as it describes a transition from a metallic phase with a spin gap due to attractive backscattering to a Peierls insulator with charge-density-wave order. Our quantum Monte Carlo results support the existence of a metallic phase with dominant power-law charge correlations, as described by the Luther-Emery fixed point. We demonstrate that for Holstein and also for purely fermionic models the spin gap significantly complicates finite-size numerical studies, and explains inconsistent previous results for Luttinger parameters and phase boundaries. On the other hand, no such complications arise in spinless models. The correct low-energy theory of the spinful Holstein model is argued to be that of singlet bipolarons with a repulsive, mutual interaction. This picture naturally explains the existence of a metallic phase, but also implies that gapless Luttinger liquid theory is not applicable.
In systems with the spin-charge separation, the period of the Aharonov-Bohm (AB) oscillation becomes half of the flux quantum. This effect is at least related to the fact that for the creation of the holons (spinons) are needed two electrons. The effect is illustrated on the example of the Hubbard Hamiltonian with the aid of the bosonization including topological numbers and exists also in the Luttinger liquid on two chains. The relation to a fractional 1/N- AB effect, which can be associated with a modified Luttinger liquid, is discussed.
Single- and two-particle excitation spectra of the one-dimensional, half-filled Holstein-Hubbard model are calculated using the continuous-time quantum Monte Carlo method. In the metallic phase, the results are consistent with a Luther-Emery liquid that has gapped spin and single-particle excitations but a gapless charge mode. However, given the initially exponential dependence of the spin gap on the backscattering matrix element, the numerical excitation spectra appear gapless in the weak-coupling regime, and therefore resemble those of a Luttinger liquid. The Mott phase has the expected charge gap and gapless spin excitations. The Peierls state shows a charge, spin, and single-particle gap, a soft phonon mode, backfolded shadow bands, and soliton excitations. Arguments and numerical evidence for the existence of a nonzero spin gap throughout the metallic phase are provided in terms of equal-time spin and charge correlation functions.
One-dimensional (1D) interacting Fermi gases underpin a rich variety of quantum liquids, ranging from the Tomonaga-Luttinger liquid and the Fulde-Ferrell-Larkin-Ovchinnikov paired state to the Luther-Emery liquid (LEL). Notably, the LEL-characterized by gapless excitations in charge or spin degree of freedom and gapped excitations in the other-has long been theoretically predicted but has eluded definitive experimental observation to date. By exactly solving the attractive Yang-Gaudin model via the Bethe ansatz, we fully determine the low-energy excitation spectra for both spin and charge channels. For fully paired fermions, the spectrum features gapped spin excitation coexisting with gapless charge excitation. We further employ bosonization to derive analytical expressions for the dynamical structure factor (DSF) of the gapped spin excitation, which is a long-standing challenge in this study. In the trapped gas, we find that the spin Bragg spectroscopy peak occurs at a much higher frequency than the charge-mode peak, where the splitting frequency between these two peaks scales approximately linearly with the interaction strength. Crucially, the spin gap manifests as a sharp threshold in the spin DSF, below which spectral weight is completely absent, proving a direct and unambiguous spectroscopic fingerprint of the LEL. Our work establishes quasi-1D trapped attractive Fermi gases as a pristine experimental platform for the long-sought direct observation of the LEL.
We show that one-dimensional quantum systems with gapless degrees of freedom and open boundary conditions form a universality class of quantum critical behavior, which we propose to call ``bounded Luttinger liquids.'' They share the following properties with ordinary (periodic) Luttinger liquids: the absence of fermionic quasiparticle excitations, charge-spin separation, and anomalous power-law correlations with exponents whose scaling relations are parametrized by a single coupling constant per degree of freedom, ${K}_{\ensuremath{\nu}}.$ The values of ${K}_{\ensuremath{\nu}}$ are independent of boundary conditions, but the representation of the critical exponents in terms of these ${K}_{\ensuremath{\nu}}'\mathrm{s}$ depends on boundary conditions. We illustrate these scaling relations by exploring general rules for boundary critical exponents derived earlier using the Bethe ansatz solution of the one-dimensional Hubbard model together with boundary conformal field theory, and the theory of Luttinger liquids in finite-size systems. We apply this theory to the photoemission properties of the organic conductors (TMTSF)2X,(\mathrm{TMTSF}{)}_{2}X,(TMTSF)2​X, where TMTSF is tetramethyltetraselenafulvalene, and X=ClO9,X={\mathrm{ClO}}_{9},X=ClO9​, PF6,{\mathrm{PF}}_{6},PF6​, ReO4,\mathrm{Re}{\mathrm{O}}_{4},ReO4​, and discuss to what extent the assumption of finite strands with open boundaries at the sample surface can reconcile the experimental results with independent information on the Luttinger-liquid state in these materials.
We use a recently developed extension of the weak-coupling diagrammatic determinantal quantum Monte Carlo method to investigate the spin, charge, and single-particle spectral functions of the one-dimensional quarter filled Holstein model with phonon frequency ${\ensuremath{\omega}}_{0}=0.1t$. As a function of the dimensionless electron-phonon coupling we observe a transition from a Luttinger to a Luther-Emery liquid with dominant 2kf2{k}_{f}2kf​ charge fluctuations. Emphasis is placed on the temperature dependence of the single-particle spectral function. At high temperatures and in both phases it is well accounted for within a self-consistent Born approximation. In the low-temperature Luttinger liquid phase we observe features that compare favorably with a bosonization approach retaining only forward scattering. In the Luther-Emery phase, the spectral function at low temperatures shows a quasiparticle gap that matches half the spin gap, whereas at temperatures above which this quasiparticle gap closes characteristic features of the Luttinger liquid model are apparent. Our results are based on lattice simulations on chains up to L=20L=20L=20 for two-particle properties and on cluster dynamical mean-field theory calculations with clusters up to 12 sites for the single-particle spectral function.