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arXiv:cond-mat/0304341 · New Journal of Physics

A two-atom picture of coherent atom–molecule quantum beats

Bogdan Borca, D. Blume, Chris H. Greene

Published Sep 2, 2003• 45 citations
arXivHTMLPDF

Abstract

A simple two-atom model is shown to describe a Bose–Einstein condensate of alkali atoms subjected to external magnetic field ramps near a Feshbach resonance. The implications uncovered for two atoms in a trap can be applied at least approximately to a many-atom condensate. A connection to observations is accomplished by scaling the trap frequency to achieve a density comparable to that of the experiments, which yields the fraction of atom pairs in the gas that become molecules. A sudden approximation is used to model the external magnetic field ramps in the vicinity of a two-body Feshbach resonance. The results of this model are compared with recent experimental observations of Donley et al (2002 Nature 417 529).

DOI
10.1088/1367-2630/5/1/111

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A simple two-atom model is shown to describe a Bose–Einstein condensate of alkali atoms subjected to external magnetic field ramps near a Feshbach resonance. The implications uncovered for two atoms in a trap can be applied at least approximately to a many-atom condensate. A connection to observations is accomplished by scaling the trap frequency to achieve a density comparable to that of the experiments, which yields the fraction of atom pairs in the gas that become molecules. A sudden approximation is used to model the external magnetic field ramps in the vicinity of a two-body Feshbach resonance. The results of this model are compared with recent experimental observations of Donley et al (2002 Nature 417 529).
Abstract. A simple two-atom model is shown to describe a Bose-Einstein condensate of alkali atoms subjected to external magnetic field ramps near a Feshbach resonance. The implications uncovered for two atoms in a trap can be applied at least approximately to a many-atom condensate. A connection to observations is accomplished by scaling the trap frequency to achieve a density comparable to that of the experiments, which yields the fraction of atom pairs in the gas that become molecules. A sudden approximation is used to model the external magnetic field ramps in the vicinity of a two-body Feshbach resonance. The results of this model are compared with recent experimental observations of Donley et al. [1]. PACS numbers: 03.75.Mn Submitted to: New J. Phys. A Two-Atom Picture of Coherent Atom-Molecule Quantum Beats 2 1.
We consider in detail the situation of applying a time-dependent external magnetic field to a 87 Rb atomic Bose–Einstein condensate held in a harmonic trap, in order to adiabatically sweep the interatomic interactions across a Feshbach resonance to produce diatomic molecules. To this end, we introduce a minimal two-body Hamiltonian depending on just five measurable parameters of a Feshbach resonance, which accurately determines all low-energy binary scattering observables, in particular, the molecular conversion efficiency of just two atoms. Based on this description of the microscopic collision phenomena, we use the many-body theory of Köhler and Burnett (2002 Phys. Rev. A 65 033601) to study the efficiency of the association of molecules in a 87 Rb Bose–Einstein condensate during a linear passage of the magnetic-field strength across the 100 mT Feshbach resonance. We explore different, experimentally accessible, parameter regimes, and compare the predictions of Landau–Zener, configuration interaction, and two-level mean-field calculations with those of the microscopic many-body approach. Our comparative studies reveal a remarkable insensitivity of the molecular conversion efficiency with respect to both the details of the microscopic binary collision physics and the coherent nature of the Bose–Einstein condensed gas, provided that the magnetic-field strength is varied linearly. We provide the reasons for this universality of the molecular production achieved by linear ramps of the magnetic-field strength, and identify the Landau–Zener coefficient determined by Mies et al (2000 Phys. Rev. A 61 022721) as the main parameter that controls the efficiency.
Recent experiments with Feshbach-resonant cesium Bose-Einstein condensates have led to unexplained molecule formation: a sudden switch of the magnetic field to its resonance value, followed by a finite hold time and another sudden switch to magnetic field values below threshold, converts about a third of the initial condensate atoms into molecules. Based on a model of coherent conversion between an atomic condensate, a molecular condensate, and magnetodissociated noncondensate atom pairs of equal and opposite momentum, we find that population trapping is strongly implicated as the physical mechanism responsible for molecule formation in switch experiments.
We have observed Bose-Einstein condensation of pairs of fermionic atoms in an ultracold 6Li gas at magnetic fields above a Feshbach resonance, where no stable 6Li2 molecules would exist in vacuum. We accurately determined the position of the resonance to be 822+/-3 G. Molecular Bose-Einstein condensates were detected after a fast magnetic field ramp, which transferred pairs of atoms at close distances into bound molecules. Condensate fractions as high as 80% were obtained. The large condensate fractions are interpreted in terms of preexisting molecules which are quasistable even above the two-body Feshbach resonance due to the presence of the degenerate Fermi gas.
Recently, effects of Feshbach resonances in atom-atom interactions were observed by varying the external magnetic field of an atomic Bose-Einstein condensate (BEC). We point out that the quasi-bound molecules created in the intermediate state of the resonance can form a second, molecular condensate. The many-body state of the system is then a hybrid atomic/molecular condensate with inter-condensate tunneling of atom pairs. A sudden variation of the magnetic field results in oscillations of the number of atoms and molecules in their respective condensates, providing a signature of this novel type of quantum tunneling.
Atom–molecule coherence in a Bose-Einstein condensate (BEC) has been demonstrated. Sudden changes were made to the magnetic field near a Feshbach resonance such that oscillations between atomic and molecular states were excited. The frequency of these oscillations was measured over a large range of magnetic fields and was found to be in excellent quantitative agreement with the predicted energy difference between two colliding atoms and the bound molecular state. This agreement indicates that we have created a quantum superposition of atoms and diatomic molecules, which are chemically different species. 1