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arXiv:cond-mat/9805323

Inter-Condensate Tunneling in Bose-Einstein Condensates with Feshbach Resonances

Eddy Timmermans, Paolo Tommasini, Robin Côté, Mahir Saleh Hussein, Arthur K. Kerman

Published May 25, 1998• 0 citations
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Abstract

Recently, effects of Feshbach resonances in atom-atom interactions were observed by varying the external magnetic field of an atomic Bose-Einstein condensate (BEC). We point out that the quasi-bound molecules created in the intermediate state of the resonance can form a second, molecular condensate. The many-body state of the system is then a hybrid atomic/molecular condensate with inter-condensate tunneling of atom pairs. A sudden variation of the magnetic field results in oscillations of the number of atoms and molecules in their respective condensates, providing a signature of this novel type of quantum tunneling.

DOI
10.48550/arxiv.cond-mat/9805323

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Recently, effects of Feshbach resonances in atom-atom interactions were observed by varying the external magnetic field of an atomic Bose-Einstein condensate (BEC). We point out that the quasi-bound molecules created in the intermediate state of the resonance can form a second, molecular condensate. The many-body state of the system is then a hybrid atomic/molecular condensate with inter-condensate tunneling of atom pairs. A sudden variation of the magnetic field results in oscillations of the number of atoms and molecules in their respective condensates, providing a signature of this novel type of quantum tunneling.
Atom–molecule coherence in a Bose-Einstein condensate (BEC) has been demonstrated. Sudden changes were made to the magnetic field near a Feshbach resonance such that oscillations between atomic and molecular states were excited. The frequency of these oscillations was measured over a large range of magnetic fields and was found to be in excellent quantitative agreement with the predicted energy difference between two colliding atoms and the bound molecular state. This agreement indicates that we have created a quantum superposition of atoms and diatomic molecules, which are chemically different species. 1
In the atomic Bose-Einstein condensate, the interactions that bring a binary atom system to an intermediate state molecule in the Feshbach resonance create a second condensate component of molecules. The atomic and molecular condensates coherently exchange pairs of atoms. We discuss a signature of the coherent intercondensate exchange: Josephson-like oscillations of the atomic and molecular populations in response to a sudden change of the energy detuning. The dependence of the many-body ground state energy on volume suggests that the on-resonant ground state is a dilute condensate with the liquidlike property of a self-determined density.
Tunneling dynamics of multi-atomic molecules between any two multi-atomic molecular Bose–Einstein condensates with Feshbach resonance is investigated. It is indicated that the tunneling in the two Bose–Einstein condensates depends not only on the inter-molecular nonlinear interactions and the initial number of molecule in these condensates, but also on the tunneling coupling between them. It is discovered that besides oscillating tunneling current between the multi-atomic molecular condensates, the nonlinear multi-atomic molecular tunneling dynamics sustains a self-locked population imbalance: a macroscopic quantum self-trapping effect. The influence of de-coherence caused by non-condensate molecule on the tunneling dynamics is studied. It is shown that de-coherence suppresses the multi-atomic molecular tunneling.
Abstract Recent advances in the precise control of ultracold atomic systems have led to the realisation of Bose–Einstein condensates (BECs) and degenerate Fermi gases. An important challenge is to extend this level of control to more complicated molecular systems. One route for producing ultracold molecules is to form them from the atoms in a BEC. For example, a two-photon stimulated Raman transition in a 87Rb BEC has been used to produce 87Rb2 molecules in a single rotational-vibrational state1, and ultracold molecules have also been formed2 through photoassociation of a sodium BEC. Although the coherence properties of such systems have not hitherto been probed, the prospect of creating a superposition of atomic and molecular condensates has initiated much theoretical work3, 4, 5, 6, 7. Here we make use of a time-varying magnetic field near a Feshbach resonance8, 9, 10, 11, 12 to produce coherent coupling between atoms and molecules in a 85Rb BEC. A mixture of atomic and molecular states is created and probed by sudden changes in the magnetic field, which lead to oscillations in the number of atoms that remain in the condensate. The oscillation frequency, measured over a large range of magnetic fields, is in excellent agreement with the theoretical molecular binding energy, indicating that we have created a quantum superposition of atoms and diatomic molecules—two chemically different species.
As it was proposed and recently verified experimentally, the mechanism of Feshbach resonance in a condensate can create a second condensate component of molecules that coexists with the atomic condensate. In this work we investigate signatures of the presence of the molecular condensate through the equilibrium properties and collective excitations of the hybrid system of atoms and molecules, subjected to a trap, employing a time-dependent variational ansatz. We show that the shape of the condensate changes significantly by the presence of the molecules and that modes unique to this hybrid system appear at observable frequencies.
Tunneling dynamics of multi-atomic molecules between atomic and multi-atomic molecular Bose–Einstein condensates with Feshbach resonance is investigated. It is indicated that the tunneling in the two Bose–Einstein condensates depends on not only the inter-atomic-molecular nonlinear interactions and the initial number of atoms in these condensates, but also the tunneling coupling between the atomic condensate and the multi-atomic molecular condensate. It is discovered that besides oscillating tunneling current between the atomic condensate and the multi-atomic molecular condensate, the nonlinear multi-atomic molecular tunneling dynamics sustains a self-locked population imbalance: a macroscopic quantum self-trapping effect. The influence of de-coherence caused by non-condensate atoms on the tunneling dynamics is studied. It is shown that de-coherence suppresses the multi-atomic molecular tunneling. Moreover, the conception of the molecular Bose–Einstein condensate, which is different from the conventional single-atomic Bose–Einstein condensate, is specially emphasized in this paper.