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arXiv:cond-mat/0403049 · Physical Review Letters

Condensation of Pairs of Fermionic Atoms near a Feshbach Resonance

Martin W. Zwierlein, Claudiu A. Stan, Christian H. Schunck, S. M. F. Raupach, Andrew J. Kerman, Wolfgang Ketterle

Published Mar 25, 2004• 1,228 citations
arXivHTMLPDF

Abstract

We have observed Bose-Einstein condensation of pairs of fermionic atoms in an ultracold 6Li gas at magnetic fields above a Feshbach resonance, where no stable 6Li2 molecules would exist in vacuum. We accurately determined the position of the resonance to be 822+/-3 G. Molecular Bose-Einstein condensates were detected after a fast magnetic field ramp, which transferred pairs of atoms at close distances into bound molecules. Condensate fractions as high as 80% were obtained. The large condensate fractions are interpreted in terms of preexisting molecules which are quasistable even above the two-body Feshbach resonance due to the presence of the degenerate Fermi gas.

DOI
10.1103/physrevlett.92.120403

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We have observed Bose-Einstein condensation of pairs of fermionic atoms in an ultracold 6Li gas at magnetic fields above a Feshbach resonance, where no stable 6Li2 molecules would exist in vacuum. We accurately determined the position of the resonance to be 822+/-3 G. Molecular Bose-Einstein condensates were detected after a fast magnetic field ramp, which transferred pairs of atoms at close distances into bound molecules. Condensate fractions as high as 80% were obtained. The large condensate fractions are interpreted in terms of preexisting molecules which are quasistable even above the two-body Feshbach resonance due to the presence of the degenerate Fermi gas.
We have observed Bose-Einstein condensation of molecules. When a spin mixture of fermionic 6Li atoms was evaporatively cooled in an optical dipole trap near a Feshbach resonance, the atomic gas was converted into 6Li2 molecules. Below 600 nK, a Bose-Einstein condensate of up to 900 000 molecules was identified by the sudden onset of a bimodal density distribution. This condensate realizes the limit of tightly bound fermion pairs in the crossover between BCS superfluidity and Bose-Einstein condensation.
Fast-sweep projection onto Feshbach molecules has been widely used as a probe of fermionic condensates. By determining the exact dynamics of a pair of atoms in time-varying magnetic fields, we calculate the number of condensed and noncondensed molecules created after fast magnetic field sweeps from the BCS to the Bose-Einstein condensate side of the resonances in 40K and 6Li, for different sweep rates and a range of initial and final fields. We discuss the relation between the initial fermionic condensate fraction and the molecular condensate fraction measured after the sweep.
We theoretically examine a system of Fermi degenerate atoms coupled to bosonic molecules by a Feshbach resonance, focusing on the superfluid transition to a molecular Bose-Einstein condensate dressed by Cooper pairs of atoms. This problem raises interest because it is unclear at present whether bimodal density distributions observed recently in 40K and 6Li are due to a condensate of bosonic molecules or fermionic atom pairs. As opposed to 40K, we find that any measurable fraction of above-threshold bosonic molecules is necessarily absent for the 6Li system in question, which strongly implicates Cooper pairs as the culprit behind its bimodal distributions.
The dynamics of pair condensate formation in a strongly interacting Fermi gas close to a Feshbach resonance was studied. We employed a phase-shift method in which the delayed response of the many-body system to a modulation of the interaction strength was recorded. The observable was the fraction of condensed molecules in the cloud after a rapid magnetic field ramp across the Feshbach resonance. The measured response time was slow compared to the rapid ramp, which provides final proof that the molecular condensates reflect the presence of fermion pair condensates before the ramp.
The use of Feshbach resonances in the field of ultracold gases has received a lot of attention recently. In first instance it was realized that these resonances can be used to alter the interaction strength in an atomic gas, by means of tuning an external magnetic field. Furthermore, by sweeping the magnetic field from one side of the resonance to the other, a degenerate gas of bosonic molecules can be created, a significant accomplishment. By making the interactions between fermionic atoms strongly attractive, a fermionic superfluid was recently made, a feat that has drawn a lot of attention in the physics community and from the media. We present work that describes these many-particle systems near a Feshbach resonance in a comprehensive way by using the concept of dressed molecules. These dressed molecules are essentially two-particle states that are a superposition of a tightly bound bare molecule, and two unbound bare atoms. This description reduces to the correct paired wave-function in the two-body limit. Moreover it gives a physically correct description of all the phenomena mentioned above: the Bose-condensation of a gas near a Feshbach resonance, that contains molecules, is more correctly interpreted as a Bose-condensation of dressed molecules. The fermionic superfluid contains a condensate of bosonic pairs, normally called Cooper pairs, that can be understood as the dressed molecules. For the latter case, the dressed-molecule picture also gives an elegant characterization of the crossover between a Bose condensate of pure molecules on one side of the resonance, to a fermionic Bardeen-Cooper-Schrieffer superfluid on the other side. Then, the dressed molecules change continuously from being mostly a bare molecule, to being mostly a loose pair of two atoms. It is clear that the nature of the dressed molecules is much determined by the probability for it to be in the bare-molecular state. This probability we denote with a single parameter Z. We present various ways of calculating it, and study how it affects the macroscopic physics.