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arXiv:cond-mat/0110335 · Physical review. B, Condensed matter

Noncrossing approximation for the anisotropic Kondo model: Charge fluctuations in a quantum box

Eran Lebanon, Avraham Schiller, Vilen Zevin

Published Dec 10, 2001• 13 citations
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Abstract

The noncrossing approximation (NCA) is generalized to the multichannel Kondo-spin Hamiltonian with arbitrary anisotropic exchange couplings and an external magnetic field, and applied---in the framework of Matveev's mapping---to the charge fluctuations in a single-electron box at the Coulomb blockade. The temperature dependences of the charge step and the capacitance are calculated for a narrow point contact. At low temperatures and close to the degeneracy point, the capacitance line shape exhibits an approximate scaling with $U/\sqrt{T},$ where U is the deviation in gate voltage from the degeneracy point. This scaling relation is proposed as a sharp experimental diagnostic for the non-Fermi-liquid physics of the system at low temperatures. Both the reliability and shortcomings of the Kondo NCA are discussed in detail. Through comparison with poor-man's scaling, we are able to pinpoint the omission of particle-particle processes as the origin of the NCA flaws. An extended diagrammatic scheme is devised to amend the NCA flaws.

DOI
10.1103/physrevb.64.245338

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The noncrossing approximation (NCA) is generalized to the multichannel Kondo-spin Hamiltonian with arbitrary anisotropic exchange couplings and an external magnetic field, and applied---in the framework of Matveev's mapping---to the charge fluctuations in a single-electron box at the Coulomb blockade. The temperature dependences of the charge step and the capacitance are calculated for a narrow point contact. At low temperatures and close to the degeneracy point, the capacitance line shape exhibits an approximate scaling with U/T,U/\sqrt{T},U/T​, where U is the deviation in gate voltage from the degeneracy point. This scaling relation is proposed as a sharp experimental diagnostic for the non-Fermi-liquid physics of the system at low temperatures. Both the reliability and shortcomings of the Kondo NCA are discussed in detail. Through comparison with poor-man's scaling, we are able to pinpoint the omission of particle-particle processes as the origin of the NCA flaws. An extended diagrammatic scheme is devised to amend the NCA flaws.
We propose a design for a one-dimensional quantum box device where the charge fluctuations are described by an anisotropic two-channel Kondo model. The device consists of a quantum box in the Coulomb blockade regime, weakly coupled to a quantum wire by a single-mode point contact. The electron correlations in the wire produce strong backscattering at the contact, significantly increasing the Kondo temperature as compared to the case of non-interacting electrons. By employing boundary conformal field theory techniques we show that the differential capacitance of the box exhibits manifest two-channel Kondo scaling with temperature and gate voltage, uncontaminated by the one-dimensional electron correlations. We discuss the prospect to experimentally access the Kondo regime with this type of device.
The Anderson impurity model is studied by means of the self-consistent hybridization expansions in its noncrossing (NCA) and one-crossing (OCA) approximations. We have found that for the one-channel spin-1/21/21/2 particle-hole symmetric Anderson model, the NCA results are qualitatively wrong for any temperature, even when the approximation gives the exact threshold exponents of the ionic states. Actually, the NCA solution describes an overscreened Kondo effect, because it is the same as for the two-channel infinite-UUU single-level Anderson model. We explicitly show that the NCA is unable to distinguish between these two very different physical systems, independently of temperature. Using the impurity entropy as an example, we show that the low-temperature values of the NCA entropy for the symmetric case yield the limit ${S}_{\mathrm{imp}}(T=0)\ensuremath{\rightarrow}ln\sqrt{2},$ which corresponds to the zero temperature entropy of the overscreened Kondo model. Similar pathologies are predicted for any other thermodynamic property. On the other hand, we have found that the OCA approach lifts the artificial mapping between the models and restores correct properties of the ground state, for instance, a vanishing entropy at low enough temperatures ${S}_{\mathrm{imp}}(T=0)\ensuremath{\rightarrow}0$. Our results indicate that the very well known NCA should be used with caution close to the symmetric point of the Anderson model.
In the present work, we calculate the conductance through a single quantum dot weakly coupled to metallic contacts. We use the spin-1/2 Anderson model to describe the quantum dot, while considering a finite Coulomb repulsion. We solve the interacting system using the noncrossing approximation (NCA) and the one-crossing approximation (OCA). We obtain the linear response conductance as a function of temperature and energy position of the localized level. From the comparison of both approximations we extract the role of the vertex corrections, which are introduced in the OCA calculations and neglected in the NCA scheme. As a function of the energy position, we observe that the diagrams omitted within the NCA are really important for appropriately describing transport phenomena in Kondo systems as well as in the mixed valence regime. On the other hand, as a function of temperature, the corrections introduced by the OCA partly recover the universal scaling properties known from numerical approaches such as the numerical renormalization group.
We suggest an experiment to study Luttinger liquid behavior in a one-dimensional nanostructure, avoiding the usual complications associated with transport measurements. The proposed setup consists of a quantum box, biased by a gate voltage, and side coupled to a quantum wire by a point contact. Close to the degeneracy points of the Coulomb blockaded box, and in the presence of a magnetic field sufficiently strong to spin polarize the electrons, the setup can be described as a Luttinger liquid interacting with an effective Kondo impurity. Using exact nonperturbative techniques, we predict that the differential capacitance of the box will exhibit distinctive Luttinger liquid scaling with temperature and gate voltage.
We investigate the low-temperature dynamics of single electron boxes and transistors close to their degeneracy point using renormalization group methods. We show that intermode scattering is a relevant perturbation and always drives the system to the two-channel Kondo fixed point, where the two channels correspond to the real spins of the conduction electrons. However, the crossover temperature T^*, below which Matveev's two-channel Kondo scenario [K.A. Matveev, Phys. Rev. B 51, 1743 (1995)] develops decreases exponentially with the number of conduction modes in the tunneling junctions and is extremely small in most cases. Above T^* the 'infinite channel model' of Ref.{onlinecite{Schoen}} turns out to be a rather good approximation. We discuss the experimental limitations and suggest a new experimental setup to observe the multichannel Kondo behavior.
We reinvestigate the large degeneracy solution of the multichannel Kondo problem, and show how in the universal regime the complicated integral equations simplifying the problem can be mapped onto a first-order differential equation. This leads to an explicit expression for the full zero-temperature scaling functions at---and away from---the intermediate non-Fermi-liquid fixed point, providing complete analytic information on the universal low---and intermediate---energy properties of the model. These results also apply to the widely used noncrossing approximation of the Anderson model, taken in the Kondo regime. An extension of this formalism for studying finite-temperature effects is also proposed and offers a simple approach to solve models of strongly correlated electrons with relevance to the physics of heavy fermion compounds.