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arXiv:cond-mat/0306603 · Physical Review Letters

Measuring Luttinger Liquid Correlations from Charge Fluctuations in a Nanoscale Structure

Paata Kakashvili, Henrik Johannesson

Published Oct 28, 2003• 11 citations
arXivHTMLPDF

Abstract

We suggest an experiment to study Luttinger liquid behavior in a one-dimensional nanostructure, avoiding the usual complications associated with transport measurements. The proposed setup consists of a quantum box, biased by a gate voltage, and side coupled to a quantum wire by a point contact. Close to the degeneracy points of the Coulomb blockaded box, and in the presence of a magnetic field sufficiently strong to spin polarize the electrons, the setup can be described as a Luttinger liquid interacting with an effective Kondo impurity. Using exact nonperturbative techniques, we predict that the differential capacitance of the box will exhibit distinctive Luttinger liquid scaling with temperature and gate voltage.

DOI
10.1103/physrevlett.91.186403

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Correlation effects in nanostructures

Paata Kakashvili

In this Ph.D. thesis I present the background and providefurther details to the work presented in the appended papers. The background consists of brief overviews of Kondo physics, Luttinger liquid theory, and conformal field theory. My own research is divided into three parts: the first deals with the interplay between Luttinger and Kondo physics (described in Papers I and II), the secondaddresses scanning tunneling microscopy (STM) response of a Luttinger liquid with an edge or an impurity (described in Paper III), and the third explores the boundary Green's function of 1D electrons in the spin-incoherent regime (described in Paper IV). In Papers I and II a setup is proposed which allows for acontrolled study of Kondo and Luttinger liquid physics. Itconsists of a quantum box, biased by a gate voltage, and side-coupled to a quantum wire by a point contact. Close to the degeneracy points of the Coulomb blockaded box the setup can be described as a Luttinger liquid interacting with an effective Kondo impurity. Using boundary conformal field theory techniques we predict that for the case of spin-polarized electrons the differential capacitance of the box will exhibit distinctive Luttinger liquid scaling with temperature and gate voltage. In the limit of zero magnetic field the Luttinger liquid behavior gets masked by two-channel Kondo screening, leading to a logarithmic scaling of the differential capacitance with temperatureand gate voltage. These effects should be possible to studyexperimentally, using the recently developed single-electrontransistor (SET) electrometer technique.In Paper III the finite-temperature local spectral weight (LSW) of a Luttinger liquid with a hard wall boundary is calculated. Close to the boundary the LSW exhibits characteristic oscillations indicative of spin-charge separation. The line shape of the LSW is also found to have a Fano-like asymmetry, a feature originating from the combined effect of electron-electron interaction and scattering off the boundary. Our results can be used to predict how edges and impurities influencethe STM response of one-dimensional electron systemsat low temperatures and voltage bias. Applications to STM onsingle-walled carbon nanotubes are also discussed.Paper IV, finally, presents a study of the spin-incoherent regime of 1D strongly interacting electrons. For sufficiently low densities the potential energy dominates the kinetic energy, and one can easily reach thespin-incoherent regime where the spin exchange energy is much less than the temperature. We have generalized the description of the spin-incoherent regime to account for the presence of a boundary. By calculating the exact Green's function we find that the charge sector critical exponent is highly sensitive to the boundary, strongly modifying the tunneling of electrons close to it. Our approach also allows for a detailed description of the crossover between boundary and bulk regimes.

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Theoretical studies suggest that an interacting one-dimensional electron system does not behave as a Fermi liquid. Instead, it is predicted to form a Luttinger liquid characterized e.g. by the absence of fermionic quasiparticles and interaction-dependent power-laws for transport quantities. So far, however, only a limited number of experiments have provided evidence for Luttinger liquid behavior. In this thesis we consider alternative methods to detect electronic correlations in one-dimensional electron systems based on our calculations of persistent currents and quantization of charge in ballistic single channel rings. The persistent current in an isolated impurity-free Luttinger liquid ring is found to be the same as for a system of non-interacting electrons. In contrast, a Luttinger liquid behavior is revealed if the ring is weakly connected to an electron reservoir and capacitively coupled to a gate electrode. The persistent current and the average charge in the ring are shown to change in a stepwise manner with the gate voltage at low temperatures. Both the step positions and the crossover temperatures are determined by the Luttinger liquid correlation parameter .alpha.(.alpha.c) which therefore can be measured. When a potential barrier is incorporated into the ring, the presence of strong interactions between electrons leads to a suppression of the persistent current and a change in its temperature dependence. A sharp maximum of the current is predicted to occur as a function of temperature. When two barriers are introduced into the ring, the possibility of resonant tunneling for the persistent current opens up. Two kinds of resonant behavior are discovered in the closed geometry: a current independent of the barrier transparency and a current analogous to the one with a single potential barrier. The persistent current in a ring containing a gas of fractionally charged excitations obeying fractional exclusion statistics is also studied. At finite temperatures, anomalous oscillations of the current are predicted as a manifestation of the statistics of the quasiparticles.

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Ilya V. Krive, P. Sandström, Robert I Shekhter +1 more

We propose a method to detect a Luttinger liquid (LL)-like behavior of a quasione-dimensional ring of electrons that does not depend on a transport measurement.Rather, a Coulomb blockade-induced quantization of the persistent current and excess charge in a ring of interacting electrons are shown to depend on the interaction strength.Both the average ring charge and the persistent current are step-like functions of an applied gate voltage at low temperatures.The step positions are determined by the LL parameter α, which therefore can be directly measured.

Europhysics Letters (EPL)•Apr 20, 1997•9 citations
We suggest an experiment to study Luttinger liquid behavior in a one-dimensional nanostructure, avoiding the usual complications associated with transport measurements. The proposed setup consists of a quantum box, biased by a gate voltage, and side coupled to a quantum wire by a point contact. Close to the degeneracy points of the Coulomb blockaded box, and in the presence of a magnetic field sufficiently strong to spin polarize the electrons, the setup can be described as a Luttinger liquid interacting with an effective Kondo impurity. Using exact nonperturbative techniques, we predict that the differential capacitance of the box will exhibit distinctive Luttinger liquid scaling with temperature and gate voltage.
In this Ph.D. thesis I present the background and providefurther details to the work presented in the appended papers. The background consists of brief overviews of Kondo physics, Luttinger liquid theory, and conformal field theory. My own research is divided into three parts: the first deals with the interplay between Luttinger and Kondo physics (described in Papers I and II), the secondaddresses scanning tunneling microscopy (STM) response of a Luttinger liquid with an edge or an impurity (described in Paper III), and the third explores the boundary Green's function of 1D electrons in the spin-incoherent regime (described in Paper IV). In Papers I and II a setup is proposed which allows for acontrolled study of Kondo and Luttinger liquid physics. Itconsists of a quantum box, biased by a gate voltage, and side-coupled to a quantum wire by a point contact. Close to the degeneracy points of the Coulomb blockaded box the setup can be described as a Luttinger liquid interacting with an effective Kondo impurity. Using boundary conformal field theory techniques we predict that for the case of spin-polarized electrons the differential capacitance of the box will exhibit distinctive Luttinger liquid scaling with temperature and gate voltage. In the limit of zero magnetic field the Luttinger liquid behavior gets masked by two-channel Kondo screening, leading to a logarithmic scaling of the differential capacitance with temperatureand gate voltage. These effects should be possible to studyexperimentally, using the recently developed single-electrontransistor (SET) electrometer technique.In Paper III the finite-temperature local spectral weight (LSW) of a Luttinger liquid with a hard wall boundary is calculated. Close to the boundary the LSW exhibits characteristic oscillations indicative of spin-charge separation. The line shape of the LSW is also found to have a Fano-like asymmetry, a feature originating from the combined effect of electron-electron interaction and scattering off the boundary. Our results can be used to predict how edges and impurities influencethe STM response of one-dimensional electron systemsat low temperatures and voltage bias. Applications to STM onsingle-walled carbon nanotubes are also discussed.Paper IV, finally, presents a study of the spin-incoherent regime of 1D strongly interacting electrons. For sufficiently low densities the potential energy dominates the kinetic energy, and one can easily reach thespin-incoherent regime where the spin exchange energy is much less than the temperature. We have generalized the description of the spin-incoherent regime to account for the presence of a boundary. By calculating the exact Green's function we find that the charge sector critical exponent is highly sensitive to the boundary, strongly modifying the tunneling of electrons close to it. Our approach also allows for a detailed description of the crossover between boundary and bulk regimes.
We propose a design for a one-dimensional quantum box device where the charge fluctuations are described by an anisotropic two-channel Kondo model. The device consists of a quantum box in the Coulomb blockade regime, weakly coupled to a quantum wire by a single-mode point contact. The electron correlations in the wire produce strong backscattering at the contact, significantly increasing the Kondo temperature as compared to the case of non-interacting electrons. By employing boundary conformal field theory techniques we show that the differential capacitance of the box exhibits manifest two-channel Kondo scaling with temperature and gate voltage, uncontaminated by the one-dimensional electron correlations. We discuss the prospect to experimentally access the Kondo regime with this type of device.
We investigate the effects of the electron-electron interactions on the quantum transport through a charge Kondo circuit. The setup consists of a quantum dot sandwiched between two leads by two nearly transparent single mode quantum point contacts. The size of the interacting area LLL in the Luttinger liquid formed in the vicinities of the narrow constrictions is assumed to be much smaller compared to the size of the quantum dot aaa. We predict that the interplay between the electron-electron interactions in the Luttinger liquid and the fingerprints of the non-Fermi liquid behavior in the vicinity of the two channel Kondo intermediate coupling fixed point allows one to determine the interaction strength through the power-law temperature scaling of the electric conductance.
Theoretical studies suggest that an interacting one-dimensional electron system does not behave as a Fermi liquid. Instead, it is predicted to form a Luttinger liquid characterized e.g. by the absence of fermionic quasiparticles and interaction-dependent power-laws for transport quantities. So far, however, only a limited number of experiments have provided evidence for Luttinger liquid behavior. In this thesis we consider alternative methods to detect electronic correlations in one-dimensional electron systems based on our calculations of persistent currents and quantization of charge in ballistic single channel rings. The persistent current in an isolated impurity-free Luttinger liquid ring is found to be the same as for a system of non-interacting electrons. In contrast, a Luttinger liquid behavior is revealed if the ring is weakly connected to an electron reservoir and capacitively coupled to a gate electrode. The persistent current and the average charge in the ring are shown to change in a stepwise manner with the gate voltage at low temperatures. Both the step positions and the crossover temperatures are determined by the Luttinger liquid correlation parameter .alpha.(.alpha.c) which therefore can be measured. When a potential barrier is incorporated into the ring, the presence of strong interactions between electrons leads to a suppression of the persistent current and a change in its temperature dependence. A sharp maximum of the current is predicted to occur as a function of temperature. When two barriers are introduced into the ring, the possibility of resonant tunneling for the persistent current opens up. Two kinds of resonant behavior are discovered in the closed geometry: a current independent of the barrier transparency and a current analogous to the one with a single potential barrier. The persistent current in a ring containing a gas of fractionally charged excitations obeying fractional exclusion statistics is also studied. At finite temperatures, anomalous oscillations of the current are predicted as a manifestation of the statistics of the quasiparticles.
Luttinger-liquid behavior of one-dimensional correlated electron systems is characterized by power-law scaling of a variety of physical observables with exponents determined by a single interaction dependent parameter KKK. We suggest a setup to study Luttinger-liquid behavior in quantum wires which allows us to determine KKK from two independent measurements: transport through a quantum dot embedded in the wire and the charge on the dot. Consistency of the two KKK's for a single probe would provide strong experimental evidence for the Luttinger-liquid paradigm.
We propose a method to detect a Luttinger liquid (LL)-like behavior of a quasione-dimensional ring of electrons that does not depend on a transport measurement.Rather, a Coulomb blockade-induced quantization of the persistent current and excess charge in a ring of interacting electrons are shown to depend on the interaction strength.Both the average ring charge and the persistent current are step-like functions of an applied gate voltage at low temperatures.The step positions are determined by the LL parameter α, which therefore can be directly measured.