The aim of this communication is to present in a concentrated form the main ideas of a method, developed by the author, for treating strongly nonequilibrium collective phenomena typical of the interaction of radiation with matter, as well as to give a survey of several applications of the method. The latter is called the Scale Separation Approach since its basic techniques rely on the possibility of separating different space-time scales in nonequilibrium statistical systems. This approach is rather general and can be applied to diverse physical problems, several of which are discussed here. These problems are: Superradiance of nuclear spins, filamentation in resonant media, semiconfinement of neutral atoms, negative electric current, and collective liberation of light.
The aim of this communication is to present in a concentrated form the main ideas of a method, developed by the author, for treating strongly nonequilibrium collective phenomena typical of the interaction of radiation with matter, as well as to give a survey of several applications of the method. The latter is called the Scale Separation Approach since its basic techniques rely on the possibility of separating different space-time scales in nonequilibrium statistical systems. This approach is rather general and can be applied to diverse physical problems, several of which are discussed here. These problems are: Superradiance of nuclear spins, filamentation in resonant media, semiconfinement of neutral atoms, negative electric current, and collective liberation of light.
The aim of this review is twofold. Firstly, a general approach is presented which can provide a unified description of the dynamics of radiating systems of different natures. Both atomic systems and spin assemblies can be treated within the same mathematical method, which is based on a pseudospin (or spin) representation of the evolution equations. The approach is applicable to all stages of radiation dynamics, including the most difficult initial quantum stage, where coherence is not yet developed. This makes it possible to study the process of coherent self-organization from the chaotic quantum stage. Secondly, the approach is illustrated by applying it to the description of several coherent phenomena. Different types of superradiance are characterized: pure superradiance, triggered superradiance, pulsing and punctuated superradiance. The theory of such interesting effects as triggering dipolar waves, turbulent photon filamentation, collective liberation of light, pseudospin atomic squeezing, and operator entanglement production is presented.
In this paper we attempt to unify the theoretical treatment of a variety of cooperative interaction phenomena occurring in resonantly interacting radiation-matter systems. The system consists of a multimode optical field interacting with N resonant atoms in a region of large spatial extent. The field and atoms may or may not be coupled to reservoirs. We derive a set of coupled master equations for the reduced matter and radiation density operators of the composite system in the first Born approximation, using a method due to Bogoliubov. These equations describe within a single framework phenomena involving superradiant emission and coherent propagation. In the first place, our theory generalizes existing formulations of the superradiance problem by treating the radiation field as part of the dynamical system rather than as a reservoir. Hence, our equations describe stimulated interaction effects, which are entirely absent in the usual superradiance master equations. Moreover, our equations contain terms describing the self-consistent interaction of an average field with a set of polarizable atoms, as in the coupled Bloch and Maxwell equations of the theory of coherent pulse propagation, and enable us to describe fluctuations, arising from incoherent emission, about the average behavior described by the Bloch-Maxwell theory. We solve formally the dynamical equation for the radiation density operator and obtain a displaced multivariate Gaussian distribution centered on the solution of the Maxwell wave equation, which has as parameters the first and second moments of the matter density operator. Then we derive and discuss the field and atomic-moment equations, both in the wave-number and position representations. The moment equations enable us to show the relationship between descriptions of superradiant damping based on the Bloch equations and those based on the existence of correlated atomic states, including both as special cases. We introduce reduced matter moments, which allow us to separate incoherent- and coherent-emission effects and enable us to discuss the question of the closure of the moment equations. Then we consider cases where the behavior of the atomic system is dominated by a strong coherent pump wave or where the atoms are in a symmetric correlated state and show how the slowly-varying-envelope approximation simplifies the radiation-moment equations in these two cases. In the former case, we obtain an approximate theory which consists, in lowest order, of the Bloch-Maxwell equations with radiative-damping terms, plus an equation describing the time development of the correlation function for field fluctuations. Returning to our general formalism, we relate the usual parameters of the theory of radiative decay and of resonant interactions to the more general quantities appearing in our spatial analysis. Finally, we discuss the importance of the stimulated-emission terms appearing in our theory and describe several extensions, including the introduction of inhomogeneous broadening.
Based on the separability with respect to position variables of the susceptibility for a finite system, we have developed a formulation which solves Schri:idinger and Maxwell equations selfconsistently. The case of linear response is' described in detail. As a manifes tation of the selfconsistency between the two equations, the appearance of radiative damping rate with correct magnitude has been demonstrated for a two-level atom in vacuum. The interaction of electromagnetic (EM) radiation with matter has been studied in various aspects for quite a long time. The relevant phenomena range, in the scale of wavelength, from rf wave (NMR, for example) to gamma ray (Mossbauer effect): They are related with the absorption, reflection, transmission, propagation, refrac tion, scattering, diffraction, emission, etc. of EM wave in linear and nonlinear manner. For the theoretical treatment of these phenomena, we need Schrodinger equation for the description of matter and Maxwell equations in classical or quantized form for radiation field. When the Maxwell equations are treated in classical form, this is called semiclassical treatment of radiation-matter interaction. Though it has a certain limitation, the semiclassical treatment can be appliedto most of the phenom ena mentioned above. For the treatment of the interaction of EM radiation with solids, it is usual to employ a susceptibility function to describe the solid, and solve the Maxwell equa tions containing that susceptibility as an integral kernel. In doing so, we must consider the boundary conditions (BC) arising from the shape of the sample in question. However, we do not consider BC's in treating microscopic systems such as an atom or small molecule. This would mean that the use of BC(s is in general not compulsory, although we are so much accustomed to it. In this respect, there has been a long debated problem of additional boundary condition (ABC) in relation with exciton polaritons in semiconductors or insulators, where the nonlocal nature of the medium allows the existence of two or more eigenmodes of the coupled exciton-EM radiation. After the long history of the ABC problem,r>- 4 > we now have a recipe to derive the appropriate form(s) of ABC(s) from a microscopic model of the medium including the details of the surface. 5 >-s> Another form of the microscopic solution of the ABC problem has been given as an ABC-free formulation, 9 >-n> where one needs
The interaction between matter and radiation has fascinated physicists for a long time. On the material side, the most detailed investigations of these processes concentrate on atoms, the basic constituents of matter. The radiation that is involved in these processes is primarily light, i.e., radiation whose wavelength is in the range of a few tenths of a micron to a few microns. Under today's laboratory conditions, this radiation is generally produced by a laser. This introduction outlines our picture of these constituents and presents some of the concepts and models that we will use throughout this book. Atoms Historical Early models: atoms as building blocks The term “atom” was coined by the Greek philosopher Democritus of Abdera (460–370 B.C.), who tried to reconcile change with eternal existence. His solution to this dilemma was that matter was not indefinitely divisible, but consisted of structureless building blocks that he called atoms. According to Democritus and other proponents of this idea, the diverse aspects of matter, as we know it, are a result of different arrangements of the same building blocks in empty space (Melsen 1957; Simonyi 1990). The most important opponent of this theory was Aristotle (384–322 B.C.), and his great influence is probably the main reason that the atomic hypothesis was not widely accepted, but lay dormant for two thousand years. It reappeared only in the eighteenth century, when the emerging experimental science found convincing evidence that matter does indeed consist of elementary building blocks.
In this work we shall study the interaction of matter and light. In so doing we shall rely heavily on the description of such processes provided by quantum mechanics. This appears on a number of levels: firstly, a quantum description of matter is indispensable if one wants to understand on the microscopic scale the different kinds of interaction processes that can occur. Secondly, a quantum description of light often turns out to be useful, sometimes necessary, to better understand these processes. We shall study phenomena such as spontaneous emission, which can only be properly treated by a theory taking into account the quantum nature of both light and matter. In the following chapters we shall address, amongst others, the following question: ‘given an atom prepared at a given time in a particular state and subjected from this time onwards to electromagnetic radiation, what is the state of the atom and radiation at any later moment in time?’ In order to be able to answer this question it will be necessary for us to know how to calculate the evolution of a quantum system in a small number of typical situations. These methods we shall demonstrate in the first chapter. The evolution of the coupled atom–light system depends on the temporal dependence of the applied light field, which could, for example, be applied from a given moment and thereafter remain unchanged in intensity, or, perhaps, be appreciable only for a finite period of time (pulsed excitation).
The present state of theoretical and experimental research on collective spontaneous emission (superradiance) in a system of radiators (atoms, molecules, or nuclei) is reviewed. The distinction between superradiance and the amplification of spontaneous emission is discussed. There is also a discussion of conditions under which the effect can be observed and of various theoretical methods for describing superradiance: the quantum single-mode and multimode models and the semiclassical approach. Theoretical papers on superradiance in systems with dimensions smaller than the wavelength of the radiation and also in extended systems are reviewed. It is shown that superradiance may occur in weakly amplifying media. A situation in which the superradiance is oscillatory is described. The possible use of superradiance to generate coherent emission in the x-ray and ? ranges is discussed. The superradiance accompanying Raman scattering of light in atomic and molecular media is studied. The theoretical results are compared with experimental observations of superradiance in the optical range. In an appendix, the nature of the phase transition in a system of radiators interacting through an electromagnetic field is discussed.