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Soviet Physics Uspekhi

Collective spontaneous emission (Dicke superradiance)

Anatolii V Andreev, Vladimir I Emel'yanov, Yu A Il'inskiĭ

Published Aug 31, 1980• 143 citations
Publisher

Abstract

The present state of theoretical and experimental research on collective spontaneous emission (superradiance) in a system of radiators (atoms, molecules, or nuclei) is reviewed. The distinction between superradiance and the amplification of spontaneous emission is discussed. There is also a discussion of conditions under which the effect can be observed and of various theoretical methods for describing superradiance: the quantum single-mode and multimode models and the semiclassical approach. Theoretical papers on superradiance in systems with dimensions smaller than the wavelength of the radiation and also in extended systems are reviewed. It is shown that superradiance may occur in weakly amplifying media. A situation in which the superradiance is oscillatory is described. The possible use of superradiance to generate coherent emission in the x-ray and ? ranges is discussed. The superradiance accompanying Raman scattering of light in atomic and molecular media is studied. The theoretical results are compared with experimental observations of superradiance in the optical range. In an appendix, the nature of the phase transition in a system of radiators interacting through an electromagnetic field is discussed.

DOI
10.1070/pu1980v023n08abeh005024

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The present state of theoretical and experimental research on collective spontaneous emission (superradiance) in a system of radiators (atoms, molecules, or nuclei) is reviewed. The distinction between superradiance and the amplification of spontaneous emission is discussed. There is also a discussion of conditions under which the effect can be observed and of various theoretical methods for describing superradiance: the quantum single-mode and multimode models and the semiclassical approach. Theoretical papers on superradiance in systems with dimensions smaller than the wavelength of the radiation and also in extended systems are reviewed. It is shown that superradiance may occur in weakly amplifying media. A situation in which the superradiance is oscillatory is described. The possible use of superradiance to generate coherent emission in the x-ray and ? ranges is discussed. The superradiance accompanying Raman scattering of light in atomic and molecular media is studied. The theoretical results are compared with experimental observations of superradiance in the optical range. In an appendix, the nature of the phase transition in a system of radiators interacting through an electromagnetic field is discussed.
This chapter considers super-radiance on an elementary level in the sense that the main notions and concepts of the phenomenon will be treated as they evolved in the course of the early studies starting with the classical works by R. H. Dicke. It considers super-radiance from a system with dimensions small compared with the wavelength of the emission that is the Dicke model. The chapter discusses the results to be obtained are also applicable to the single-mode super-radiance of an extended system. It then considers mainly the cooperative spontaneous emission of a collection of N identical atoms confined within a small volume. If the audience wish to investigate the super-radiance of an extended system, the dimensions of which exceed the emission wavelength, the semiclassical method is more convenient. In essence, the semiclassical approach discussed in the chapter combines the quantum mechanical treatment of the atomic system that uses the density matrix formalism with the classical treatment of the radiation field.
A comparative analysis is given of spin superradiance and atomic superradiance. Their similarities and distinctions are emphasized. It is shown that, despite a close analogy, these phenomena are fundamentally different. In atomic systems, superradiance is a self-organized process, in which both the initial cause, being spontaneous emission, as well as the collectivizing mechanism of their interactions through the common radiation field, are of the same physical nature. Contrary to this, in actual spin systems with dipole interactions, the latter are the major reason for spin motion. Electromagnetic spin interactions through radiation are negligible and can never produce collective effects. The possibility of realizing superradiance in molecular magnets by coupling them to a resonant circuit is discussed.
Fully-excited two-level atoms separated by less than the transition wavelength cooperatively emit light in a short burst, a phenomenon called superradiance by R. Dicke in 1954. The burst is characterized by a maximum intensity scaling with the square of the number of atoms NNN and a temporal width reduced by NNN compared to the single atom spontaneous decay time. Both effects are usually attributed to a synchronization of the electric dipole moments of the atoms occurring during the process of light emission. Contrary to this explanation, it was recently shown by use of a quantum path description that the peak intensity results from the quantum correlations among the atoms when occupying symmetric Dicke states. Here we investigate from this perspective the temporal evolution of the ensemble, starting in the small sample limit, i.e., when the atoms have mutual separations much smaller than the transition wavelength λλλ and pass down the ladder of symmetric Dicke states. In addition, we explore the temporal evolution for the case of non-interacting atoms with mutual separations much larger than λλλ. We show that in this case a similar superradiant burst of the emitted radiation is observed if the quantum correlations of the atoms are generated by conditional photon measurements retaining the atomic ensemble within or close to the symmetric subspace.
For pt.II see ibid., vol.19, p.2109 (1986). This paper is the third in a theoretical study of subradiance, i.e. the cooperative inhibition of spontaneous emission by a destructive interatomic interference, a phenomenon which has recently been observed. The paper is devoted to the problem of the cooperative spontaneous emission of atomic samples with linear dimensions much smaller than the wavelength of the emitted light. The treatment, which is based on a fully quantum mechanical description of the problem, corroborates the results obtained in a semiclassical treatment by Friedberg and Hartmann (1974). Starting from a master equation describing both the cooperative spontaneous emission and the dipole-dipole interaction, a statistical treatment of the latter is introduced and the corresponding symmetry relaxation is studied. The evolution of the atoms is described in three typical cases that correspond to different sample geometries and/or atomic distributions. In one of these cases, in particular, the symmetry is first conserved and the atoms follow Dicke's predictions for a time. A 'retarded' symmetry breaking then occurs suddenly, near the zero value of the collective energy, as in Friedberg and Hartmann's calculations for a small sphere. With regard to the further evolution of the atoms in this case, which cannot be studied in a semiclassical model, it is shown that the decay rate quickly becomes much smaller than the incoherent decay rate. An unquestionable subradiance phenomenon is thus predicted in this case.
Abstract The electrodynamics of active continuous media is applied to theoretically examine collective spontaneous emission regimes of dipole oscillator ensembles. Recent experiments in which the superfluorescence phenomenon has been observed are reviewed. The focus is on propagation and interaction effects experienced by the inhomogeneous waves of active center polarization and electromagnetic fields. The superradiant laser dynamics is examined and prospects for the realization of superradiant lasers using low-Q cavities are discussed.
Abstract The electrodynamics of active continuous media is applied to theoretically examine collective spontaneous emission regimes of dipole oscillator ensembles. Recent experiments in which the superfluorescence phenomenon has been observed are reviewed. The focus is on propagation and interaction effects experienced by the inhomogeneous waves of active center polarization and electromagnetic fields. The superradiant laser dynamics is examined and prospects for the realization of superradiant lasers using low- Q cavities are discussed.