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Ultracold atoms in optical lattices with long-range interactions and periodic driving

O. Tieleman

Published Mar 8, 2013• 0 citations
Publisher

Abstract

This thesis contains theoretical research on ultracold quantum gases in spatially periodic potentials, featuring high-frequency periodic driving, long-range interactions, or both. The largest part features deep potentials where the behaviour of the gas is well-described by quantum lattice models. The periodic driving is then integrated out to obtain effective time-independent descriptions. One project investigates emergent long-range interactions in a stationary, weak, spatially periodic potential, where a lattice theory is not appropriate.In two short introductory chapters, the topics of ultracold atoms, optical lattice potentials, periodic driving, and long-range interactions, are sketched, without attempting to give a complete overview. Some experimentally relevant length and energy scales are given, but the main focus is on deriving and constructing theoretical descriptions of ultracold gases in various spatially and/or temporally periodic potentials.The first project presented, is focused on how the single-particle spectrum of a Bose gas in a non-separable two-dimensional square lattice is affected by high-frequency periodic driving; the most striking conclusion is that under suitable circumstances, it develops two inequivalent minima, leading to finite-momentum Bose-Einstein condensation. Perturbative calculations indicate that local interactions induce spontaneous time-reversal symmetry breaking (TRSB) in such a system.The second project investigates the interplay between kinetic frustration and long-range interactions in fermionic gases. Both a mean-field approximation and exact diagonalisations predict that such a system, studied in the more specific realisation of a weakly interacting dipolar fermionic gas in a 2D triangular lattice, also leads to spontaneous TRSB. Furthermore, a density wave could form at quarter filling, where the Fermi surface is perfectly nested. Perhaps more interesting yet, a spatially inhomogeneous TRSB pattern is predicted, confined to the low-density sublattice that emerges in the density wave.The third project revolves around the question of supersolidity in the presence of a gauge field. Applying the Bogolyubov approximation to a variation of the extended Bose-Hubbard model, indicates that combining an artificial staggered magnetic field in a 2D square lattice with nearest-neighbour density-density interactions, not only leads to a supersolid with staggered vortices, but also induces an inhomogeneous distribution of the associated currents around the elementary plaquette.In the fourth project, a one-dimensional Bose gas with strong local interactions in a weak lattice at incommensurate densities is shown to feature excitations corresponding to excess or deficit particles. The excitations interact repulsively at long distances, in spite of the fact that the underlying atoms themselves do not. As a consequence, the incommensurability of the density with the lattice can drive a transition to a density wave and even a supersolid.The four above-mentioned research projects combine bosonic and fermionic gases, weak and strong interactions, perturbative and mean-field approximations, effective field theories and exact diagonalisations. The main overall conclusion is that long-range interactions and high-frequency periodic driving lead to a very diverse range of fascinating phenomena in ultracold lattice gases.

DOI
10.5821/dissertation-2117-94906

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This thesis contains theoretical research on ultracold quantum gases in spatially periodic potentials, featuring high-frequency periodic driving, long-range interactions, or both. The largest part features deep potentials where the behaviour of the gas is well-described by quantum lattice models. The periodic driving is then integrated out to obtain effective time-independent descriptions. One project investigates emergent long-range interactions in a stationary, weak, spatially periodic potential, where a lattice theory is not appropriate.In two short introductory chapters, the topics of ultracold atoms, optical lattice potentials, periodic driving, and long-range interactions, are sketched, without attempting to give a complete overview. Some experimentally relevant length and energy scales are given, but the main focus is on deriving and constructing theoretical descriptions of ultracold gases in various spatially and/or temporally periodic potentials.The first project presented, is focused on how the single-particle spectrum of a Bose gas in a non-separable two-dimensional square lattice is affected by high-frequency periodic driving; the most striking conclusion is that under suitable circumstances, it develops two inequivalent minima, leading to finite-momentum Bose-Einstein condensation. Perturbative calculations indicate that local interactions induce spontaneous time-reversal symmetry breaking (TRSB) in such a system.The second project investigates the interplay between kinetic frustration and long-range interactions in fermionic gases. Both a mean-field approximation and exact diagonalisations predict that such a system, studied in the more specific realisation of a weakly interacting dipolar fermionic gas in a 2D triangular lattice, also leads to spontaneous TRSB. Furthermore, a density wave could form at quarter filling, where the Fermi surface is perfectly nested. Perhaps more interesting yet, a spatially inhomogeneous TRSB pattern is predicted, confined to the low-density sublattice that emerges in the density wave.The third project revolves around the question of supersolidity in the presence of a gauge field. Applying the Bogolyubov approximation to a variation of the extended Bose-Hubbard model, indicates that combining an artificial staggered magnetic field in a 2D square lattice with nearest-neighbour density-density interactions, not only leads to a supersolid with staggered vortices, but also induces an inhomogeneous distribution of the associated currents around the elementary plaquette.In the fourth project, a one-dimensional Bose gas with strong local interactions in a weak lattice at incommensurate densities is shown to feature excitations corresponding to excess or deficit particles. The excitations interact repulsively at long distances, in spite of the fact that the underlying atoms themselves do not. As a consequence, the incommensurability of the density with the lattice can drive a transition to a density wave and even a supersolid.The four above-mentioned research projects combine bosonic and fermionic gases, weak and strong interactions, perturbative and mean-field approximations, effective field theories and exact diagonalisations. The main overall conclusion is that long-range interactions and high-frequency periodic driving lead to a very diverse range of fascinating phenomena in ultracold lattice gases.
This thesis studies bosonic and fermionic quantum gases. In the first part, a variational many-body theory is used to explain a Bragg scattering experiment carried out on a bosonic quantum gas [S.B. Papp et al. Bragg Spectroscopy of a Strongly Interacting 85Rb Bose-Einstein Condensate. Phys. Rev. Lett. 101, 135301 (2008)]. A key feature in the experiment was the use of a Feshbach resonance, which made large values of the scattering length accessible. Due to the large values of the scattering length, existing models such as the Beliaev model could not be used to explain the observations, and therefore the experiment was a particularly interesting one to analyze. In our first approach, we constructed ad hoc potentials that fitted the observed excitation spectrum, and later we improved our approach by using T-matrix formalism to describe the Feshbach resonant system. All in all, the phenomenological model we developed fits the observed excitation spectrum and yields correct molecular Feshbach resonance state energies in certain cases. The second part of this thesis studies fermionic quantum gases. We focus on studying a gas of spin-1/2 particles confined to a spin-dependent optical lattice. The lattice geometry is such that the up-spin component is loaded in a honeycomb lattice, and the down-spin component is confined to the underlying triangular lattice. We considered attractive on-site and nearest-neighbor interactions, and formulated the nearest-neighbor interaction term in such a way that it takes into account the possibility of spontaneous time-reversal symmetry breaking. Furthermore, we took into account the possibility of Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase, which breaks spatial symmetry. Within a mean-field approximation, we showed that the FFLO state is the ground state of the system in many instances. In addition, we found out that the system spontaneously breaks time-reversal symmetry if the nearest-neighbor interaction strength is large. Due to the time-reversal symmetry breaking, the system has topologically non-trivial phases characterized by nonzero Chern numbers. Finally, there were also cases where the time-reversal symmetry was broken in the FFLO phase, and thus we found a phase where spatial and time-reversal symmetries are simultaneously broken.
Ultracold atoms are used to study various fundamental physics, including many-body system, nonequilibrium dynamics, and find many applications in quantum computing and quantum sensing. In this thesis, we studied the dynamics of ultracold atom gases with controllable two-body interactions. One of the major concerns is to manipulate the atomic states with electromagnetic fields. Here, we will show four projects associated with this topic. The first project is about the Sagnac interferometer based on trapped Bose-Einstein condensate. We explored the dynamics of the atoms and their relation to the sensitivity. We came up with an optimised driving field, and the performance is examined with interactions taken into consideration. The second project is about the quantum dynamics of bosonic atoms in an optical lattice with long-range interactions by Rydberg-dressing. It has been widely studied due to its controllable strength, length and anisotropy, which paves the new approach to engineering exotic quantum states and improving the performance of quantum devices. We found that phase transitions of Mott-insulator, superfluid supersolid, and density wave during a quench process. The correlation of the atoms is studied which reveals the properties of long-range interactions. The third project shows new designs of the magneto-optical trap for atom cooling. They are proposed to be manufactured by 3D printing technology. We simulated their performance and optimised the geometric parameters. The time-response and impedance have also been analysed. The fourth project studies the ground state of Rydberg-dressed fermions from the perspective of Fermi surface deformation. We calculated the deformation manifested by the aspect ratio and the appearance of Cooper pairs. The power-law scaling relations have been found with respect to the laser field, atom density and the quantum number of Rydberg states.
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The study of out-of-equilibrium dynamics in ultra-cold gases is a new and exciting field, driven largely by the recent experimental advances in controlling and imaging cold clouds. The experimental and theoretical work thus far has been somewhat exploratory and largely numerical in nature, as the very paradigms for thinking about these systems are not well established. In this thesis I consider several different scenarios of ultra-cold bosonic and fermionic gases driven out of equilibrium and study their properties. In Chapter 1, I provide an overview of the phenomenology of ultra-cold gases, highlighting the timescales governing these systems and how the experimentalist can tune them. I discuss how cold gases can be cooled and trapped and discuss the basic physics behind optical lattices. I also discuss experimental probes of these gases, in particular the new high resolution imaging techniques developed recently at Chicago, Munich and Harvard. In Chapter 2, I discuss an early experiment (circa. 2008) which observed long lived spin dynamics in a thermal spin-1/2 Fermi gas. This experiment is an nice illustration of interesting physics resulting from the separation of timescales between spin and collisional dynamics. In my opinion, it is an excellent example of why cold gases are naturally suited to studying non-equilibrium dynamics. I simulate the experiment numerically using a collisionless Boltzmann equation and explain the observed spin dynamics both qualitatively and quantitively. In Chapter 3, I continue the discussion of spin waves in thermal gases by extending previous works on spin-1/2 gases to spin-1 Bose gases. In contrast to Chapter 2, the bulk of the work in this Chapter is analytic in nature. In particular, I find a spin wave instability in the thermal spin-1 Bose gas, which is the high temperature analog of the polar to ferromagnetic transition in a spin-1 Bose Einstein condensate. In Chapter 3, I turn my attention to bosonic systems and briefly review the the Bogoliubov mean-field theory. I calculate the momentum distribution and density-density correlation function of an interacting Bose gas within the Bogoliubov framework. Then I consider bosons in an optical lattice, and introduce the Bose Hubbard model. I calculate the mean-field phase diagram of the Bose Hubbard model and then consider fluctuations about the mean field, and derive the excitation spectrum of the lattice gas in the superfluid and insulating regimes. In Chapter 4, I ask what we learn by studying the dynamics of correlation functions following a sudden change in the interactions in a superfluid. Using the Bogoliubov theory developed in Chapter 3, I will show how the underlying excitation spectrum influences the long and short time behavior of the correlation functions. By considering a lattice dispersion, I study the analogous problem in a weak optical lattice and discuss how the lattice dispersion leads to additional features in the correlation functions. I will also discuss the timescale governing the revival of the condensate fraction in a quantum depleted gas. In Chapter 5, I derive equations of motion governing the dynamics of one and two body correlation functions in the single-band Bose Hubbard model, applicable to bosons in deep lattices. I then consider a simple quench from a Mott insulating initial state to a weakly interacting final state and produce analytic expressions describing the dynamics of correlations following such a quench. I discuss the timescale for the development of long range order following such a quench. I study the problem of chapter 4 using an equations of motion approach. This approach complements the Bogoliubov approach of Chapter 4. First, I derive exact expressions for a quench to a non-interacting state. I then consider how interactions redistribute quasi-momentum to first order in perturbation theory in different dimensions. In Chapter 6, I calculate the relevant timescales for local and global dynamics in trapped lattice Bose gases, a work done in collaboration with Dr. Kaden R. A Hazzard. Using a time-dependent Gutzwiller mean-field theory, I show that the timescale for local equilibration in these systems is fast in experimental terms. I then show that due to the spatial inhomogeneities inherent to cold gases, achieving global equilibrium can be quite complicated, sometimes taking longer than the lifetime of the experiment, an issue of practical importance to current day experiments. I continue this discussion in Chapter 7 which is a collaborative work with experimentalists David McKay and Prof. Brian DeMarco from the University of Toronto and the University of Illinois, Urbana Champaign. Using experimental and numerical methods, we show that the rapid timescales for local dynamics in interacting systems invalidates a frequently used cold atom technique for mapping out the momentum distribution of atoms in an optical lattice.
This thesis explores certain extraordinary phenomena that occur when a gas of neutral atoms is cooled to the coldest temperatures in the universe --- much colder, in fact, than the electromagnetic radiation that permeates the vacuum of interstellar space. At those extreme temperatures, quantum effects dominate and the collective behaviour of the atoms can have unexpected consequences. For example, Bose-Einstein condensation may occur where the atoms lose their individual identities to coalesce into a macroscopic quantum particle. Although such ultracold atomic gases are interesting in their own right, much of the excitement generated in this field is due to the possibility that studying these gases could shed light on intractable problems in other areas of physics. This is predominantly due to the uniquely high degree of control over various physical parameters that ultracold atomic gases afford to experimentalists. Recent technological advances exploit this advantage to study quantum phenomena in a detail that would not be possible in other systems. For instance, atoms can be made to attract or repel each other, the strength of this interaction can be set to almost any value, and external potentials of various geometries and periodicities can be introduced. In this way, atoms can be used to model phenomena as diverse as the quark-gluon plasmas arising in high-energy particle physics, the colour superfluids conjectured to exist in the core of neutron stars, and the high-temperature superconductivity exhibited by electrons on the ion lattice of certain compounds. Indeed, ultracold atomic gases also have a demonstrated applicability to quantum information and computation. Due to a subtle interplay between electronic and nuclear spins known as the hyperfine interaction, atoms can have either an integer or half-integer total spin quantum number, making them either bosonic or fermionic at low temperatures, respectively. With the exception of chapter 7, the work presented here concerns fermionic atoms in periodic potential formed by interfering laser beams. Indeed, the standing light wave created by the interfering beams gives rise to a lattice potential because of the Stark effect which couples the electronic energy levels of the atoms to the spatially undulating electric field. Furthermore, fermionic atoms can be prepared in two different hyperfine states corresponding to the the \\spin-up" and \\spin-down" quantum states, and as such mimic electrons moving in the lattice structure of solids. This system is well described by the famous Hubbard model which we introduce in chapter 2 and, under certain conditions, undergoes a phase transition into the N eel state which believed to be a precursor to superconductivity in certain high-temperature superconductors. In chapter 3, we calculate precisely how the N eel state may be achieved in an ultracold fermionic atom gas. When the number of spin-up and spin-down atoms is unequal the system becomes spin-canted and exhibits both ferro- and antiferromagnetic characteristics, as we show in chapter 4. We also nd there are topological excitations present in the quantum spin texture known as merons which have never unambiguously been observed before. In order to form a Bose-Einstein condensate, fermionic atoms must rst form pairs, and can do so in two contrasting ways. The relationship between these two qualitatively di erent forms of pairing is described in chapter 5, and we examine how these two types of pairs transform into one another in an optical lattice in chapter 6. Finally, chapter 7 is a detailed eld-theoretic study of pairing as it occurs in an ultracold Bose gas. There, we nd there is an intriguing bosonic analogy of the two forms of fermion pairing and explore the properties of these pairs.
The monograph is devoted to the main aspects of theoretical description of quantum many-body systems with Bose-Einstein or Fermi-Dirac statistics. We provide a review of modern methods of theoretical research, both analytical and numerical, as well as experimental realizations of unique effects and phenomena in quantum systems. The main attention is given to the theoretical study of exotic states in degenerate gases of atoms and quasiparticles. We develop a methology to accurately determine chemical potentials and other thermodynamic characteristics of ideal Bose and Fermi gases. These allow us to describe the ultraslow-light phenomenon in ultracold atomic gases in the framework of the microscopic approach that accounts for the internal degrees of freedom of bound states. The formalism relies on the linear response theory applied for the case of weak perturbation by the external elecromagnetic field. We also study Bose-Einstein condensation of photons in ideal atomic gases in different regimes of degeneracy of atomic and photonic components. A special attention is given to the Bogoliubov method of quasiaverages and related theory of a weakly interacting Bose gas with condensate. We extend the Bogoliubov theory to examine the spinor condensate and its magnetic states, as well as the condensate of heteronuclear Fermi-Fermi molecules. We also study a spatially periodic state of Bose-Einstein condensate, which can serve as a model for supersolid state of matter and develop the hydrodynamic theory of the latter. We outline the main statements of the Fermi liquid theory including the Pomeranchuk stability conditions of the normal state. It is shown that the violation of stability conditions results in certain phase transitions associated with the breaking of translational symmetry and rotational symmetry in the momentum space. We review a progress in the theoretical description of ultracold Fermi gases consisting of neutral atoms in the presence of the optical lattice spatial modulation. In case of multicomponent systems, a number of unique magnetically-ordered states are theoretically studied and predicted. We also develop a theory of highly dispersive spinful excitons in cobaltite compounds that explains certain unusual magnetic properties and effects in the resonant inelastic X-ray scattering on these materials.