We study quantum phases and transitions in ultra-cold quantum gases, beyond the scope of conventional condensed matter systems. The study focuses on three major thrusts. The first thrust is the study of cold ensembles of bosonic or fermionic atoms in the higher orbital bands of optical lattices. Orbital and topological quantum physics is systematically explored for various lattice geometries, to be outlined below. The second is the low dimensional spin-imbalanced fermions in the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase. We analyze its thermal instability towards Berezinsky-Kosterlitz-Thouless (BKT) phase transitions driven by different topological defects at finite temperature. The third is the theoretical search for a mechanism to achieve a Bose-Einstein crystal phase for bosons in the ground state. A new class of two-body interactions characterized by strong momentum-dependence is found to give rise to such a quantum state. It is different than but related to the long-debated concept of supersolidity. The first thrust forms the main part of the dissertation. Meta-stable phases of high orbital bosons and fermions have been explored for different lattice geometries such as square and bipartite lattices. Exotic Mott and superfluid phases are studied in both one and two dimensions. Quantum and thermal phase transitions, associated with time reversal symmetry breaking and their experimental signatures are discussed. In particular a quantum ``disordered" superfluid phase, beyond the mean field description, is found in one dimension. The challenging problem of probing time reversal symmetry breaking is solved. Besides, a one-dimensional fermionic optical ladder with coupled s- and p-orbitals is shown to mimic spin-orbit interactions and exhibit topological insulator and topological superconducting phases. Charge fractionalization is shown to be realizable in such an sp-orbital ladder.
We study quantum phases and transitions in ultra-cold quantum gases, beyond the scope of conventional condensed matter systems. The study focuses on three major thrusts. The first thrust is the study of cold ensembles of bosonic or fermionic atoms in the higher orbital bands of optical lattices. Orbital and topological quantum physics is systematically explored for various lattice geometries, to be outlined below. The second is the low dimensional spin-imbalanced fermions in the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase. We analyze its thermal instability towards Berezinsky-Kosterlitz-Thouless (BKT) phase transitions driven by different topological defects at finite temperature. The third is the theoretical search for a mechanism to achieve a Bose-Einstein crystal phase for bosons in the ground state. A new class of two-body interactions characterized by strong momentum-dependence is found to give rise to such a quantum state. It is different than but related to the long-debated concept of supersolidity. The first thrust forms the main part of the dissertation. Meta-stable phases of high orbital bosons and fermions have been explored for different lattice geometries such as square and bipartite lattices. Exotic Mott and superfluid phases are studied in both one and two dimensions. Quantum and thermal phase transitions, associated with time reversal symmetry breaking and their experimental signatures are discussed. In particular a quantum ``disordered" superfluid phase, beyond the mean field description, is found in one dimension. The challenging problem of probing time reversal symmetry breaking is solved. Besides, a one-dimensional fermionic optical ladder with coupled s- and p-orbitals is shown to mimic spin-orbit interactions and exhibit topological insulator and topological superconducting phases. Charge fractionalization is shown to be realizable in such an sp-orbital ladder.
In this thesis, we discuss ultracold quantum gases both in continuum and optical lattices. For the continuum Fermi gases in BCS-BEC crossover, we present an effective field theory study on the recently discovered puzzling damping phenomena on the BCS side of the crossover. We find that in contrast to the previous proposed pair-breaking mechanism of damping, the damping process is due to the interaction between superfluid phonons and thermally excited fermionic quasi particles. Results from our effective field theory are compared quantitatively with experiments, showing a good agreement. For the ultracold fermionic atoms in optical lattices, we propose two novel quantum phases. Firstly, we show that a novel superconducting pairing occurs for spin-imbalanced Fermi gases with the spin up and down Fermi levels lying within the px- and s- orbital bands of a quasi-one-dimensional optical lattice. The pairs condense at a finite momentum equal to the sum of the two Fermi momenta of spin up and down fermions, and form a p-orbital condensate. The phase diagram shows that the p-orbital pair condensate occurs in a wide range of fillings. Secondly, we study instabilities of single-species fermionic atoms in the p-orbital bands in two-dimensional square optical lattices. From the nearly-perfect nesting Fermi surfaces, charge density wave and orbital density wave orderings with stripe or checkerboard patterns are found for attractive and repulsive interactions, respectively. The superconducting phase, usually expected of attractively interacting fermions, is strongly suppressed. We also use field theory to analyze the possible liquid crystal phases in our system. For bosons, we study ultracold bosonic atoms loaded in a one-dimensional optical lattice of two-fold p-orbital degeneracy at each site, and find an anti-ferro-orbital, a homogeneous px Mott insulator phase and two kinds of superfluid phases distinguished by the orbital ordering.
Motivated by rapid experimental progress in the fields of ultracold atoms and quantum optics, I present a series of theoretical studies which explore collective phenomena in quantum gases of atoms and photons. In Chapter 1, I highlight the major developments in the research field and identify the overarching themes and motivations. I also provide a roadmap for the rest of the thesis and summarize the main results. The remaining eight chapters contain original studies, organized along three broad motifs. In Chapters 2 through 5, I investigate how the nature of collective excitations and quasiparticles can be explored in modern experiments. More specifically, I model the dynamics of a spin impurity in a Bose lattice gas, develop a protocol for observing fractionalized excitations or anyons in an optical cavity, and characterize the collective dynamics of Bogoliubov quasiparticles and domain walls in a Fermi superfluid. In Chapters 6 and 7, I examine unconventional superfluid phases in spin-imbalanced Fermi gases. In particular, I propose a novel technique for engineering the long-sought-after Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase and study the relative stability of exotic phases across a dimensional crossover. Finally, Chapters 8 and 9 are devoted to studies of kinetics in out-of-equilibrium systems. I model the formation of a Bose-Einstein condensate in a dimple trap and characterize the approach to thermal equilibrium in quasi-one-dimensional geometries.
This thesis studies bosonic and fermionic quantum gases. In the first part, a variational many-body theory is used to explain a Bragg scattering experiment carried out on a bosonic quantum gas [S.B. Papp et al. Bragg Spectroscopy of a Strongly Interacting 85Rb Bose-Einstein Condensate. Phys. Rev. Lett. 101, 135301 (2008)]. A key feature in the experiment was the use of a Feshbach resonance, which made large values of the scattering length accessible. Due to the large values of the scattering length, existing models such as the Beliaev model could not be used to explain the observations, and therefore the experiment was a particularly interesting one to analyze. In our first approach, we constructed ad hoc potentials that fitted the observed excitation spectrum, and later we improved our approach by using T-matrix formalism to describe the Feshbach resonant system. All in all, the phenomenological model we developed fits the observed excitation spectrum and yields correct molecular Feshbach resonance state energies in certain cases. The second part of this thesis studies fermionic quantum gases. We focus on studying a gas of spin-1/2 particles confined to a spin-dependent optical lattice. The lattice geometry is such that the up-spin component is loaded in a honeycomb lattice, and the down-spin component is confined to the underlying triangular lattice. We considered attractive on-site and nearest-neighbor interactions, and formulated the nearest-neighbor interaction term in such a way that it takes into account the possibility of spontaneous time-reversal symmetry breaking. Furthermore, we took into account the possibility of Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase, which breaks spatial symmetry. Within a mean-field approximation, we showed that the FFLO state is the ground state of the system in many instances. In addition, we found out that the system spontaneously breaks time-reversal symmetry if the nearest-neighbor interaction strength is large. Due to the time-reversal symmetry breaking, the system has topologically non-trivial phases characterized by nonzero Chern numbers. Finally, there were also cases where the time-reversal symmetry was broken in the FFLO phase, and thus we found a phase where spatial and time-reversal symmetries are simultaneously broken.
Cold atoms with laser-induced spin-orbit (SO) interactions provide promising platforms to explore novel quantum physics, in particular the exotic topological phases, beyond natural conditions of solids. The past several years have witnessed important progresses in both theory and experiment in the study of SO coupling and novel quantum states for ultracold atoms. Here we review the physics of the SO coupled quantum gases, focusing on the latest theoretical and experimental progresses of realizing SO couplings beyond one-dimension (1D), and the further investigation of novel topological quantum phases in such systems, including the topological insulating phases and topological superfluids. A pedagogical introduction to the SO coupling for ultracold atoms and topological quantum phases is presented. We show that the so-called optical Raman lattice schemes, which combine the creation of the conventional optical lattice and Raman lattice with topological stability, can provide minimal methods with high experimental feasibility to realize 1D to 3D SO couplings. The optical Raman lattices exhibit novel intrinsic symmetries, which enable the natural realization of topological phases belonging to different symmetry classes, with the topology being detectable through minimal measurement strategies. We introduce how the non-Abelian Majorana modes emerge in the SO coupled superfluid phases which can be topologically nontrivial or trivial, for which a few fundamental theorems are presented and discussed. The experimental schemes for achieving non-Abelian superfluid phases are given. Finally, we point out the future important issues in this rapidly growing research field.
Advances in experiments on dilute ultracold atomic gases have given us access to highly tunable quantum systems. In particular, there have been substantial improvements in achieving different kinds of interaction between atoms. As a result, utracold atomic gases oer an ideal platform to simulate many-body phenomena in condensed matter physics, and engineer other novel phenomena that are a result of the exotic interactions produced between atoms. In this dissertation, I present a series of studies that explore the physics of dilute ultracold atomic gases in different settings. In each setting, I explore a different form of the inter-particle interaction. Motivated by experiments which induce artificial spin-orbit coupling for cold fermions, I explore this system in my first project. In this project, I propose a method to perform universal quantum computation using the excitations of interacting spin-orbit coupled fermions, in which effective p-wave interactions lead to the formation of a topological superfluid. Motivated by experiments which explore the physics of exotic interactions between atoms trapped inside optical cavities, I explore this system in a second project. I calculate the phase diagram of lattice bosons trapped in an optical cavity, where the cavity modes mediates effective global range checkerboard interactions between the atoms. I compare this phase diagram with one that was recently measured experimentally. In two other projects, I explore quantum simulation of condensed matter phenomena due to spin-dependent interactions between particles. I propose a method to produce tunable spin-dependent interactions between atoms, using an optical Feshbach resonance. In one project, I use these spin-dependent interactions in an ultracold Bose-Fermi system, and propose a method to produce the Kondo model. I propose an experiment to directly observe the Kondo effect in this system. In another project, I propose using lattice bosons with a large hyperfine spin, which have Feshbach-induced spin-dependent interactions, to produce a quantum dimer model. I propose an experiment to detect the ground state in this system. In a final project, I develop tools to simulate the dynamics of fermionic superfluids in which fermions interact via a short-range interaction.
The study of out-of-equilibrium dynamics in ultra-cold gases is a new and exciting field, driven largely by the recent experimental advances in controlling and imaging cold clouds. The experimental and theoretical work thus far has been somewhat exploratory and largely numerical in nature, as the very paradigms for thinking about these systems are not well established. In this thesis I consider several different scenarios of ultra-cold bosonic and fermionic gases driven out of equilibrium and study their properties. In Chapter 1, I provide an overview of the phenomenology of ultra-cold gases, highlighting the timescales governing these systems and how the experimentalist can tune them. I discuss how cold gases can be cooled and trapped and discuss the basic physics behind optical lattices. I also discuss experimental probes of these gases, in particular the new high resolution imaging techniques developed recently at Chicago, Munich and Harvard. In Chapter 2, I discuss an early experiment (circa. 2008) which observed long lived spin dynamics in a thermal spin-1/2 Fermi gas. This experiment is an nice illustration of interesting physics resulting from the separation of timescales between spin and collisional dynamics. In my opinion, it is an excellent example of why cold gases are naturally suited to studying non-equilibrium dynamics. I simulate the experiment numerically using a collisionless Boltzmann equation and explain the observed spin dynamics both qualitatively and quantitively. In Chapter 3, I continue the discussion of spin waves in thermal gases by extending previous works on spin-1/2 gases to spin-1 Bose gases. In contrast to Chapter 2, the bulk of the work in this Chapter is analytic in nature. In particular, I find a spin wave instability in the thermal spin-1 Bose gas, which is the high temperature analog of the polar to ferromagnetic transition in a spin-1 Bose Einstein condensate. In Chapter 3, I turn my attention to bosonic systems and briefly review the the Bogoliubov mean-field theory. I calculate the momentum distribution and density-density correlation function of an interacting Bose gas within the Bogoliubov framework. Then I consider bosons in an optical lattice, and introduce the Bose Hubbard model. I calculate the mean-field phase diagram of the Bose Hubbard model and then consider fluctuations about the mean field, and derive the excitation spectrum of the lattice gas in the superfluid and insulating regimes. In Chapter 4, I ask what we learn by studying the dynamics of correlation functions following a sudden change in the interactions in a superfluid. Using the Bogoliubov theory developed in Chapter 3, I will show how the underlying excitation spectrum influences the long and short time behavior of the correlation functions. By considering a lattice dispersion, I study the analogous problem in a weak optical lattice and discuss how the lattice dispersion leads to additional features in the correlation functions. I will also discuss the timescale governing the revival of the condensate fraction in a quantum depleted gas. In Chapter 5, I derive equations of motion governing the dynamics of one and two body correlation functions in the single-band Bose Hubbard model, applicable to bosons in deep lattices. I then consider a simple quench from a Mott insulating initial state to a weakly interacting final state and produce analytic expressions describing the dynamics of correlations following such a quench. I discuss the timescale for the development of long range order following such a quench. I study the problem of chapter 4 using an equations of motion approach. This approach complements the Bogoliubov approach of Chapter 4. First, I derive exact expressions for a quench to a non-interacting state. I then consider how interactions redistribute quasi-momentum to first order in perturbation theory in different dimensions. In Chapter 6, I calculate the relevant timescales for local and global dynamics in trapped lattice Bose gases, a work done in collaboration with Dr. Kaden R. A Hazzard. Using a time-dependent Gutzwiller mean-field theory, I show that the timescale for local equilibration in these systems is fast in experimental terms. I then show that due to the spatial inhomogeneities inherent to cold gases, achieving global equilibrium can be quite complicated, sometimes taking longer than the lifetime of the experiment, an issue of practical importance to current day experiments. I continue this discussion in Chapter 7 which is a collaborative work with experimentalists David McKay and Prof. Brian DeMarco from the University of Toronto and the University of Illinois, Urbana Champaign. Using experimental and numerical methods, we show that the rapid timescales for local dynamics in interacting systems invalidates a frequently used cold atom technique for mapping out the momentum distribution of atoms in an optical lattice.