Ultracold atoms are used to study various fundamental physics, including many-body system, nonequilibrium dynamics, and find many applications in quantum computing and quantum sensing. In this thesis, we studied the dynamics of ultracold atom gases with controllable two-body interactions. One of the major concerns is to manipulate the atomic states with electromagnetic fields. Here, we will show four projects associated with this topic. The first project is about the Sagnac interferometer based on trapped Bose-Einstein condensate. We explored the dynamics of the atoms and their relation to the sensitivity. We came up with an optimised driving field, and the performance is examined with interactions taken into consideration. The second project is about the quantum dynamics of bosonic atoms in an optical lattice with long-range interactions by Rydberg-dressing. It has been widely studied due to its controllable strength, length and anisotropy, which paves the new approach to engineering exotic quantum states and improving the performance of quantum devices. We found that phase transitions of Mott-insulator, superfluid supersolid, and density wave during a quench process. The correlation of the atoms is studied which reveals the properties of long-range interactions. The third project shows new designs of the magneto-optical trap for atom cooling. They are proposed to be manufactured by 3D printing technology. We simulated their performance and optimised the geometric parameters. The time-response and impedance have also been analysed. The fourth project studies the ground state of Rydberg-dressed fermions from the perspective of Fermi surface deformation. We calculated the deformation manifested by the aspect ratio and the appearance of Cooper pairs. The power-law scaling relations have been found with respect to the laser field, atom density and the quantum number of Rydberg states.
Ultracold atoms are used to study various fundamental physics, including many-body system, nonequilibrium dynamics, and find many applications in quantum computing and quantum sensing. In this thesis, we studied the dynamics of ultracold atom gases with controllable two-body interactions. One of the major concerns is to manipulate the atomic states with electromagnetic fields. Here, we will show four projects associated with this topic. The first project is about the Sagnac interferometer based on trapped Bose-Einstein condensate. We explored the dynamics of the atoms and their relation to the sensitivity. We came up with an optimised driving field, and the performance is examined with interactions taken into consideration. The second project is about the quantum dynamics of bosonic atoms in an optical lattice with long-range interactions by Rydberg-dressing. It has been widely studied due to its controllable strength, length and anisotropy, which paves the new approach to engineering exotic quantum states and improving the performance of quantum devices. We found that phase transitions of Mott-insulator, superfluid supersolid, and density wave during a quench process. The correlation of the atoms is studied which reveals the properties of long-range interactions. The third project shows new designs of the magneto-optical trap for atom cooling. They are proposed to be manufactured by 3D printing technology. We simulated their performance and optimised the geometric parameters. The time-response and impedance have also been analysed. The fourth project studies the ground state of Rydberg-dressed fermions from the perspective of Fermi surface deformation. We calculated the deformation manifested by the aspect ratio and the appearance of Cooper pairs. The power-law scaling relations have been found with respect to the laser field, atom density and the quantum number of Rydberg states.
Rydberg-dressed ground state atoms are atoms with an electron off-resonantly excited to a very high energy state, i.e., a state of high principal quantum number n ≫ 1. This thesis investigates the quantum dynamics of interacting Rydberg-dressed ground state atoms trapped in several multi-well potential traps. Rydberg atoms are atoms with exaggerated properties. One of their most interesting properties is that they exhibit a strong and long-ranged interaction that can be tuned leading to a variety of different quantum behaviours. My work focuses on studying the effects of these interacting atoms when loaded in multi-well potential traps. Generally, multi-well systems are considered as the simplest example of a finite optical lattice structure. For this reason, this thesis covers three research topics that examine the effects of long-range interaction on Rydberg-dressed atoms trapped in several potential confinements. I begin, in the introduction, by discussing the theoretical background of relevance to this work. It starts with presenting the physics of Bose-Einstein condensate. Then, the fundamentals of the interaction between two-level atom and light are analytically studied. This study has the purpose of understanding both; the dressed interacting atoms and optical lattices. The definition, characteristics, and the nature of the interaction between Rydberg atoms are analysed afterwards. The second chapter examines the dynamics of an ensemble of interacting Rydberg- dressed atoms trapped in static, i.e., time-independent, multi-well potentials using a mean-field theoretical approach. I choose one-dimensional double- and triple-well in addition to a two-dimensional quadruple-well potentials. The time-dependent non-linear Gross-Pitaevskii equation is used to numerically explore the ensemble’s quantum dynamics. Solving the dynamical differential equations along with tuning the strength of the applied long-range interaction shows that the behaviour of non-interacting Rydberg-dressed atoms does not differ conceptually according to the geometry of the trapping potential. However, this changes when the interactions are switched on where the shape of the confinement leads to interesting outcomes especially in the non-linear interacting limit, such as macroscopic quantum self-trapping. After investigating an ensemble of interacting Rydberg-dressed atoms in static multi-well potential traps, the second research topic examines the dynamical evolution of these atoms when loaded in a finite optical lattice using the extended Bose-Hubbard model. In this chapter, the atoms ensemble is assumed to be in a superfluid state where I investigate both, the order parameter when the Rydberg excitation laser is applied and the interference pattern of the condensates in different dimensions. The study shows the emerging long-range interactions lead to a rapid collapse of the superfluid order parameter and in general allow only for partial revivals. In addition, the interference experiments can directly reveal the interaction between Rydberg-dressed atoms. In the fourth chapter, the dynamics of Rydberg-dressed atoms trapped in a dynamical, i.e., time-dependent, potential confinement is presented. The dynamical trap is constructed such that it begins as a harmonic oscillator and ends as a double- well potential. The analysis investigates an ensemble of contact-interacting atoms via the time-dependent non-linear GP equation.
Optical lattices make it possible to trap and coherently control large ensembles of ultracold atoms. They provide the possibility to create lattice potentials that mimic the structure of solid-state systems, and to control these potentials dynamically. In this thesis, we study how dynamical manipulations of the lattice geometry can be used to perform different tasks, ranging from quantum information processing to the creation of diatomic molecules. We first examine the dynamical properties of ultracold atoms trapped in a lattice whose periodicity is dynamically doubled. We derive a model describing the dynamics of the atoms during this process, and compute the different interaction parameters of this model. We investigate different ways of using this lattice manipulation to optimise the initialisation time of a Mott-insulating state with one atom per site, and provide a scaling law related to the interaction parameters of the system. We go on to show that entangling operations between the spin of adjacent atoms are realisable with optical lattices forming arrays of double-well potentials. We study the creation of a lattice containing a spin-encoded Bell-pair in each double-well, and show that resilient, highly-entangled many-body states are realisable using lattice manipulations. We show that the creation of cluster-like states encoded on Bell-pairs can be achieved using these systems, and we provide measurement networks that allow the execution of quantum algorithms while maintaining intact the resilience of the system. Finally, we investigate the possibility to create a diatomic molecular state and simulate Fermi systems via the excitation to Rydberg levels of ground-state atoms trapped in optical lattices. We develop a method based on symbolical manipulations to compute the interaction parameters between highly-excited electrons, and evaluate them for different electronic configurations. We use these parameters to investigate the existence of diatomic molecular states with equilibrium distances comparable to typical lattice spacings. Considering the possibility to excite atoms trapped in an optical lattice to Rydberg levels such that the electronic cloud of neighbouring atoms overlap, we propose a model describing their interactions and compute its parameters. If such systems were realised, they would allow the simulation of Fermi systems at a temperature much below the Fermi temperature, thus enabling the observation of quantum phenomena hitherto inaccessible with current technology.
In this habilitation-thesis a collection of 14 experiments is presented. In these experiments we have developed and used novel techniques to control ultracold gases on the quantum level. In brief, Bose-Einstein condensates (BEC) and degenerate Fermi gases of laser-cooled alkali atoms are subjected to specially designed optical and magnetic fields. The fields influence in a coherent way the behavior, properties and dynamics of the gases. On this basis we developed tools to prepare, coherently manipulate, and analyze pre-defined quantum states. With this high level of control, it was possible to investigate interesting physics phenomena, and we were able to achieve several breakthroughs in the field of ultracold atoms. Highlights of our experimental results include the demonstration of phase engineering of a BEC wavefunction where we created solitons in a BEC and studied their propagation. In another experiment we constructed a spatially resolved matter wave interferometer with which we mapped out the phase distribution on a condensate. Illuminating the BEC with a periodic pattern, i.e. an optical lattice, allowed us to study solid states physics phenomena. In a second set of experiments we demonstrated optically tuning of the interaction between atoms with optical Feshbach resonances. Employing either magnetically tunable Feshbach resonances or laser radiation, we were able to produce ground state molecules in well defined quantum states. This led to the production of the first molecular BEC. By tuning the coupling of atom pairs in a Fermi gas of atoms, we could for the first time investigate the so-called BEC-BCS crossover which describes the continuous change from a BEC superfluid to a Bardeen-Cooper Schrieffer (BCS) superfluid. Due to the excellent control on the quantum level, the developed cold atom techniques open up intriguing prospects for future applications and experiments. They represent a general tool box to investigate fundamental physical phenomena in a pure and undisturbed environment. In the future, cold atoms might serve as a testing ground for fundamental theories or as quantum simulators for complex systems.
Advances in experiments on dilute ultracold atomic gases have given us access to highly tunable quantum systems. In particular, there have been substantial improvements in achieving different kinds of interaction between atoms. As a result, utracold atomic gases oer an ideal platform to simulate many-body phenomena in condensed matter physics, and engineer other novel phenomena that are a result of the exotic interactions produced between atoms. In this dissertation, I present a series of studies that explore the physics of dilute ultracold atomic gases in different settings. In each setting, I explore a different form of the inter-particle interaction. Motivated by experiments which induce artificial spin-orbit coupling for cold fermions, I explore this system in my first project. In this project, I propose a method to perform universal quantum computation using the excitations of interacting spin-orbit coupled fermions, in which effective p-wave interactions lead to the formation of a topological superfluid. Motivated by experiments which explore the physics of exotic interactions between atoms trapped inside optical cavities, I explore this system in a second project. I calculate the phase diagram of lattice bosons trapped in an optical cavity, where the cavity modes mediates effective global range checkerboard interactions between the atoms. I compare this phase diagram with one that was recently measured experimentally. In two other projects, I explore quantum simulation of condensed matter phenomena due to spin-dependent interactions between particles. I propose a method to produce tunable spin-dependent interactions between atoms, using an optical Feshbach resonance. In one project, I use these spin-dependent interactions in an ultracold Bose-Fermi system, and propose a method to produce the Kondo model. I propose an experiment to directly observe the Kondo effect in this system. In another project, I propose using lattice bosons with a large hyperfine spin, which have Feshbach-induced spin-dependent interactions, to produce a quantum dimer model. I propose an experiment to detect the ground state in this system. In a final project, I develop tools to simulate the dynamics of fermionic superfluids in which fermions interact via a short-range interaction.
Quantum optics and ultracold gases are established fields, but they almost do not overlap: the quantum nature of light is typically neglected in works on ultracold atoms. In our work the quantumness of both light and ultracold matter plays a key role. First, we show that light is a quantum nondemolition (QND) probe of many-body phases: they can be distinguished by correlations and full distribution functions (we consider bosons, fermions, and dipolar molecules). Light is not only sensitive to densities, but also to the matter-field interference. Second, we prove that the measurement backaction constitutes a novel source of competitions in many-body systems, especially, for non-QND cases. This leads to a plethora of new phenomena: oscillations of multipartite entangled modes, protection and break-up of fermion pairs, antiferromagnetic orders, long-range pair tunnelling and entanglement beyond Hubbard models. We prove that feedback control induces phase transitions and tunes their universality class. Third, the quantization of trapping potential (quantum optical lattices) leads to novel phases, including both density orders (supersolids, density waves) and bond orders of matter fields (superfluid and supersolid dimers, trimers). Results beyond ultracold atoms include: We extend the paradigm of feedback control from the state control to control of phase transitions. We present the measurement backaction as a novel source of competitions in many-body physics. We merge quantum Zeno dynamics and non-Hermitian physics and show a novel type of Zeno phenomena with Raman transitions beyond Zeno dynamics. We propose quantum simulators based on collective light-matter interaction. Our models can be applied to arrays of other systems (qubits). In general, quantum measurements and feedback produce new phenomena untypical to both closed unitary systems and open dissipative ones in many-body physics.
This thesis contains theoretical research on ultracold quantum gases in spatially periodic potentials, featuring high-frequency periodic driving, long-range interactions, or both. The largest part features deep potentials where the behaviour of the gas is well-described by quantum lattice models. The periodic driving is then integrated out to obtain effective time-independent descriptions. One project investigates emergent long-range interactions in a stationary, weak, spatially periodic potential, where a lattice theory is not appropriate.In two short introductory chapters, the topics of ultracold atoms, optical lattice potentials, periodic driving, and long-range interactions, are sketched, without attempting to give a complete overview. Some experimentally relevant length and energy scales are given, but the main focus is on deriving and constructing theoretical descriptions of ultracold gases in various spatially and/or temporally periodic potentials.The first project presented, is focused on how the single-particle spectrum of a Bose gas in a non-separable two-dimensional square lattice is affected by high-frequency periodic driving; the most striking conclusion is that under suitable circumstances, it develops two inequivalent minima, leading to finite-momentum Bose-Einstein condensation. Perturbative calculations indicate that local interactions induce spontaneous time-reversal symmetry breaking (TRSB) in such a system.The second project investigates the interplay between kinetic frustration and long-range interactions in fermionic gases. Both a mean-field approximation and exact diagonalisations predict that such a system, studied in the more specific realisation of a weakly interacting dipolar fermionic gas in a 2D triangular lattice, also leads to spontaneous TRSB. Furthermore, a density wave could form at quarter filling, where the Fermi surface is perfectly nested. Perhaps more interesting yet, a spatially inhomogeneous TRSB pattern is predicted, confined to the low-density sublattice that emerges in the density wave.The third project revolves around the question of supersolidity in the presence of a gauge field. Applying the Bogolyubov approximation to a variation of the extended Bose-Hubbard model, indicates that combining an artificial staggered magnetic field in a 2D square lattice with nearest-neighbour density-density interactions, not only leads to a supersolid with staggered vortices, but also induces an inhomogeneous distribution of the associated currents around the elementary plaquette.In the fourth project, a one-dimensional Bose gas with strong local interactions in a weak lattice at incommensurate densities is shown to feature excitations corresponding to excess or deficit particles. The excitations interact repulsively at long distances, in spite of the fact that the underlying atoms themselves do not. As a consequence, the incommensurability of the density with the lattice can drive a transition to a density wave and even a supersolid.The four above-mentioned research projects combine bosonic and fermionic gases, weak and strong interactions, perturbative and mean-field approximations, effective field theories and exact diagonalisations. The main overall conclusion is that long-range interactions and high-frequency periodic driving lead to a very diverse range of fascinating phenomena in ultracold lattice gases.