Many schemes for implementing quantum information processing require that the atomic states used have a nonzero magnetic moment; however, such magnetically sensitive states of an atom are vulnerable to decoherence due to fluctuating magnetic fields. Dressing an atom with external fields is a powerful method of reducing such decoherence [N. Timoney et al., Nature (London) 476, 185 (2011)]. We introduce an experimentally simpler method of manipulating such a dressed-state qubit, which allows the implementation of general rotations of the qubit, and demonstrate this method using a trapped ytterbium ion.
Scalability is a challenging yet key aspect required for large scale quantum computing and simulation using ions trapped in radio-frequency (rf) Paul traps. In this thesis 171Yb+ ions are used to demonstrate a magnetic field insensitive qubit which has a measured coherence time of 1.5 s, making it an ideal candidate to use for storing quantum information. A magnetic field sensitive qubit is also characterised which can be used for the implementation of multi-qubit gates using a potentially very scalable scheme based on microwaves in conjunction with a static magnetic field gradient instead of using lasers. However, the measured coherence time is limited by magnetic field fluctuations and will prohibit high fidelity gate operations from being performed. To address this issue, the preparation of a dressed-state qubit using a microwave based stimulated rapid adiabatic passage (STIRAP) pulse sequence will be presented. This qubit is protected against the noisy environment making it less sensitive to magnetic field fluctuations. The lifetime of this qubit is measured to demonstrate its suitability for storing quantum information. A powerful method for manipulating the dressed-state qubit will be presented and is used to measure a coherence time of the qubit of 500 ms which is two orders of magnitude longer compared to the magnetic field sensitive qubit. It will also be shown that our method allows for the implementation of arbitrary rotations of the dressed-state qubit on the Bloch sphere using only a single rf field. This substantially simplifies the experimental setup for single and multi-qubit gates. Furthermore, this thesis will present a experimental setup capable of successfully operating microfabricated surface ion traps. This setup is then used to operate and characterise the first two-dimensional (2D) lattice of ion traps on a microchip. A unique feature of the microfabrication technique used for this device is the extremely large voltage that can be applied which allows long ion lifetimes along with large secular frequencies to be measured, demonstrating the robustness of this device. Rudimentary shuttling between neighbouring lattice sites will be shown which could be used as part of a efficient scheme to load a large lattice of ions. One of the many applications of a 2D lattice of ions lies in the field of quantum simulations where many-body systems such as quantum magnetism, high temperature superconductivity, the fractional quantum hall effect and synthetic gauge fields can be simulated. It will be shown how making only minor modifications to the microchip the ion-ion separation can be reduced sufficiently to offer an exciting platform for the successful implementation of 2D quantum simulations. A theoretical investigation on the optimal 2D ion trap lattice geometry will also be presented with the aim to maximise the ratio of ion-ion coupling strength to decoherence from motional heating of the ions and to laser induced off-resonant coupling.
In this thesis, I discuss coherent manipulation of a trapped ytterbium ion using long wavelength radiation and the results of experiments towards the performance of a two-ion entanglement gate using a static magnetic field gradient of 23.3(6) T/m to create coupling between an ion's internal state and its motion. After using these experiments to explain the requirements for high-fidelity entanglement operations, I continue by examining existing methods for creating this gradient, the current limiting factor in producing the highest fidelity operations. This includes a full characterisation of the gradients produced by symmetric scheme permanent magnets and buried current carrying wires including development of scaling laws in order to create optimum gradients for a given trap geometry. I continue by proposing a new method by which extremely high gradients over 100 T/m can be created for planar chip traps with minimal modification to an existing experiment. These gradients are tailored for axial as well as radial entanglement schemes and aim to show that the technology exists in order to produce a two-qubit gate over the fault tolerant threshold. Subsequently, I discuss the implementation of this new scheme in an experiment before constructing the apparatus to accurately align a chip with these magnets and documenting their installation into two new experimental setups. This includes a preliminary measurement of the gradient produced by an imperfect setup outside of vacuum which verifies those simulated at ~ 110 T/m. Lastly, I discuss the prospects of on-chip magnetic materials and propose a new method which when sufficiently developed should allow for high magnetic field gradients to be produced on-chip at higher ion heights than when solely using current carrying wires. Additionally this scheme should allow for switchable gradients with maximised stability in geometries previously not possible to create.
This thesis describes experimental work in which the spin and motional states of one and two trapped atomic ions are manipulated with long-wavelength radiation in the microwave and radio frequency (RF) regime. This allows single- and two-qubit quantum logic gates to be implemented with long-wavelength radiation, in contrast to laser frequency radiation used in the majority of work to date. The two-qubit gate scheme developed represents a significant advance towards a large scale quantum computing architecture in which laser light is not needed for coherent manipulation. An experimental setup is built in which a macroscopic linear Paul trap is fitted with permanent magnets to create a strong axial magnetic field gradient. This addition allows the spin and motional states of the ions to be coupled using long-wavelength radiation. The coherence time of qubits that are sensitive to the magnetic field gradient is increased by nearly three orders of magnitude with the use of dressed states and the lifetime and coherence time are measured to be T1 = 0.63(4) s and T2 = 0.65(5) s, respectively. Using the dressed-state qubit, sideband cooling of a single ion to the motional ground state is demonstrated, and the final mean phonon number after cooling is measured to be \bar{n} = 0.13(4). Finally, a two-qubit gate is demonstrated using the dressed-state qubits in conjunction with the magnetic field gradient, and a Bell state fidelity of F = 0.985(12) is determined. This is a significant increase in fidelity for a two-qubit gate based on long-wavelength radiation compared to previous work. The errors are analysed and it is shown that with the next generation of microfabricated traps being developed in the group, the gate fidelity using this scheme can be pushed far into the fault tolerant regime. This makes this scheme promising as an integral part of a large scale quantum computing architecture.
This thesis describes experimental work on implementing single and two qubit gates in ¹7¹Yb+ ions using methods suitable for a large scale quantum computer. By combining a magnetic field gradient with microwave and radiofrequency radiation, the spin and motional states of the ions are coupled which allows multi-qubit operations to be performed, as well as providing individual addressing of ions in frequency space. A dressed state qubit is used which exhibits an increase of over two orders of magnitude in the coherence time for a qubit that it is sensitive to the magnetic field gradient. Using this system, single qubit gates are characterised using the technique of randomised benchmarking, resulting in a measured average error per gate of 9(3)x10¯4. A new type of two qubit gate is experimentally demonstrated, which in comparison to a standard two qubit gate shows significantly increased resilience to two major sources of gate infidelity: heating of the motional mode of the ions during gate operations, and incorrectly set gate field frequencies. These types of errors are expected to become increasingly important with the move towards quantum processors with large numbers of qubits. Using this same technique, a two qubit gate is also demonstrated at a higher initial temperature with a significantly improved fidelity compared to standard methods. These gate techniques are used to demonstrate work towards implementing positiondependent quantum logic, a method which could remove the correlation between the number of ions and the number of gate fields required in a large scale quantum computing architecture. A method to move the dressed state qubit through a magnetic field gradient while preserving quantum information is demonstrated, as well as a method to optimise the phase of a two qubit gate of unknown phase in order to implement a CNOT logic gate. This provides a path forwards to demonstrating a CNOT gate using position-dependent quantum logic.
The highly popular ytterbium-171 (
171mathrmYb+) ion is commonly employed in quantum information research as a qubit whose excellent coherence time and fast, simple state preparation has allowed cutting edge work in quantum computation and simulation. Despite these large benefits, the demonstrated measurement fidelity of this ion has lagged the state preparation and gate fidelity achieved to date.In this thesis we investigate and realize methods of increasing the measurement fidelity of
171mathrmYb+ in a scaleable way for large quantum systems. Using methods of coherent control, we implement a pulsed state detection scheme using a mode-locked laser to perform background-free spectroscopy of the ``bright'' state of the qubit. The small hyperfine splitting of the ion necessitates the use of multiple (two) pulses to manipulate time dynamics of the ion to excite a single transition. A Mach-Zehnder interferometer is constructed to control these pulse separations both coarsely (
sim 237 ps) and on a fine sub-femtosecond scale. These pulses cause destructive/constructive interference of the electron wave packet of a single ion levitated in vacuum and are engineered to state-selectively excite the qubit. This allows measurement of the qubit whose transition frequency is much smaller than the bandwidth of the interrogation laser.During this spectroscopy, mechanical forces from the mode-locked laser frequency comb can drive the ion into large coherent states of motion. This motion has been dubbed ``phonon lasing''. We investigate the phonon lasing affect and how the ion interacts with multiple comb teeth. The large number of teeth leads to a protection mechanism from runaway energy gain by near-by blue detuned teeth, allowing ions to be trapped and cooled by the mode-locked laser, regardless of its detuning. We further explore these discrete amplitude coherent states by injecting energy into the ion's motion and exciting higher-order oscillations.We, for the first time, implement an ``electron shelving'' of the hyperfine qubit, and incoherently transfer the bright state population in the extremely long-lived ($\\approx$5 yr)
2F
7/2 state of
171Yb
+, functionally disconnected state. This is accomplished via narrow-band optical pumping on the
2S
1/2 to the
2D
5/2 quadrupole which has a leaky dipole channel into the
2F
7/2. Narrow-band optical pumping is again used to rescue the ion at the end of the experiment with the aid of a 760 nm E2 transition back into the cooling cycle. Measurement with this scheme is no longer limited by off-resonant effects from the main cycling transition. Limits of this novel technique, as well as further directions using the F state as a utility for quantum information are explored. Finally, we combine the pulsed background-free spectroscopy with shelving and demonstrate high-fidelity, background free detection of a single trapped
171mathrmYb+ qubit.