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Strong correlations and topological order in one-dimensional systems

Wade DeGottardi

Published Aug 1, 2012• 0 citations
OpenAlex

Abstract

This thesis presents theoretical studies of strongly correlated systems as well as topologically ordered systems in 1D. Non-Fermi liquid behavior characteristic of interacting 1D electron systems is investigated with an emphasis on experimentally relevant setups and observables. The existence of end Majorana fermions in a 1D p-wave superconductor subject to periodic, incommensurate and disordered potentials is studied. The Tomonaga-Luttinger liquid (TLL), a model of interacting electrons in one spatial dimension, is considered in the context of two systems of experimental interest. First, a study of the electronic properties of single-walled armchair carbon nanotubes in the presence of transverse electric and magnetic fields is presented. As a result of their effect on the band structure and electron wave functions, fields alter the nature of the (effective) Coulomb interaction in tubes. In particular, it is found that fields couple to nanotube bands (or valleys), a quantum degree of freedom inherited from the underlying graphene lattice. As revealed by a detailed TLL calculation, it is predicted that fields induce electrons to disperse into their spin, band, and charge components. Fields also provide a means of tuning the shell-filling behavior associated with short tubes. The phenomenon of charge fractionalization is investigated in a one-dimensional ring. TLL theory predicts that momentum-resolved electrons injected into the ring will fractionalize into clockwise- and counterclockwise-moving quasiparticles. As a complement to transport measurements in quantum wires connected to leads, non-invasive measures involving the magnetic field profiles around the ring are proposed. Topological aspects of 1D p-wave superconductors are explored. The intimate connection between non-trivial topology (fermions) and spontaneous symmetry breaking (spins) in one-dimension is investigated. Building on this connection, a spin ladder system endowed with vortex degrees of freedom is proposed in order to study the effects that inhomogeneous potentials have on the topological phase diagram. Periodic vortex patterns yield a rich parameter space for tuning into a topologically non-trivial phase. This analysis hinges on the development of a topological invariant based on the wave function of Majorana fermions which inhabit the ends of the system and are robust to disorder. The method is generalized to aperiodic and disordered potentials. The topological phase diagram of such systems is studied; numerical and analytic results are found to be in close agreement.

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This thesis presents theoretical studies of strongly correlated systems as well as topologically ordered systems in 1D. Non-Fermi liquid behavior characteristic of interacting 1D electron systems is investigated with an emphasis on experimentally relevant setups and observables. The existence of end Majorana fermions in a 1D p-wave superconductor subject to periodic, incommensurate and disordered potentials is studied. The Tomonaga-Luttinger liquid (TLL), a model of interacting electrons in one spatial dimension, is considered in the context of two systems of experimental interest. First, a study of the electronic properties of single-walled armchair carbon nanotubes in the presence of transverse electric and magnetic fields is presented. As a result of their effect on the band structure and electron wave functions, fields alter the nature of the (effective) Coulomb interaction in tubes. In particular, it is found that fields couple to nanotube bands (or valleys), a quantum degree of freedom inherited from the underlying graphene lattice. As revealed by a detailed TLL calculation, it is predicted that fields induce electrons to disperse into their spin, band, and charge components. Fields also provide a means of tuning the shell-filling behavior associated with short tubes. The phenomenon of charge fractionalization is investigated in a one-dimensional ring. TLL theory predicts that momentum-resolved electrons injected into the ring will fractionalize into clockwise- and counterclockwise-moving quasiparticles. As a complement to transport measurements in quantum wires connected to leads, non-invasive measures involving the magnetic field profiles around the ring are proposed. Topological aspects of 1D p-wave superconductors are explored. The intimate connection between non-trivial topology (fermions) and spontaneous symmetry breaking (spins) in one-dimension is investigated. Building on this connection, a spin ladder system endowed with vortex degrees of freedom is proposed in order to study the effects that inhomogeneous potentials have on the topological phase diagram. Periodic vortex patterns yield a rich parameter space for tuning into a topologically non-trivial phase. This analysis hinges on the development of a topological invariant based on the wave function of Majorana fermions which inhabit the ends of the system and are robust to disorder. The method is generalized to aperiodic and disordered potentials. The topological phase diagram of such systems is studied; numerical and analytic results are found to be in close agreement.
This dissertation is devoted to theoretical studies of strongly interacting one-dimensional and quasi one-dimensional electron systems. The properties of one-dimensional electron systems can be studied within the bosonization technique, which presents fermions as collective bosonic density excitations. The power of this approach is the ability to treat electron-electron interaction exactly in the low-energy limit. The approach predicts the failure of Fermi liquid and an absence of long-range order in one-dimensions. The low-energy description of one-dimensional interacting systems is called the Tomonaga-Luttinger liquid theory. For example, the edges of quantum Hall systems are one-dimensional and described by a chiral Tomonaga-Luttinger liquid. Another example is a quantum spin Hall system with helical edge states, which are also described by a Tomonaga-Luttinger liquid. In our first work, a study of magnetized edge states of quantum spin-Hall system is presented. A magnetic field dependent signature of such edges is obtained, which can be verified in a Coulomb drag experiment. The second part of the dissertation is devoted to quasi-one dimensional antiferromagnetic lattices. A spatially anisotropic lattice antiferromagnet can be viewed as an array of one dimensional spin chains coupled in a way to match the lattice symmetry. This allows to use the non-Abelian bosonization technique to describe the low-energy physics of spin chains and study the inter-chain interactions perturbatively. The work presented in the dissertation studies the effect of Dzyaloshinskii-Moriya interaction on the magnetic phase diagram of the spatially anisotropic kagome antiferromagnet. We predict a Dzyaloshinskii-Moriya interaction driven phase transition from Neel to Neel+dimer state. In the third work, a novel model of the fractional quantum Hall effect is given. Wave functions of two-dimensional electrons in strong and quantizing magnetic field are essentially one-dimensional. That invites one to use the one-dimensional phenomenological bosonization to describe the density fluctuations of the two-dimensional interacting electrons in magnetic field. Remarkably, the constructed trial bosonized fermion operator describing the electron states with a fixed Landau gauge momentum is effectively two-dimensional.
The interplay among symmetry, topology and condensed matter systems has deepened our understandings of matter and lead to tremendous recent progresses in finding new topological phases of matter such as topological insulators, superconductors and semi-metals. Most examples of the aforementioned topological materials are free fermion systems, in this thesis, however, we focus on their strongly correlated counterparts where electron-electron interactions play a major role. With interactions, exotic topological phases and quantum critical points with fractionalized quantum degrees of freedom emerge. In the first part of this thesis, we study the problem of resonant tunneling through a quantum dot in a spinful Luttinger liquid. It provides the simplest example of a (0+1)d system with symmetry-protected phase transitions. We show that the problem is equivalent to a two channel SU(3) Kondo problem and can be mapped to a quantum Brownian motion model on a Kagome lattice. Utilizing boundary conformal field theory, we find the universal peak conductance and compute the scaling behavior of the resonance line-shape.\nFor the second part, we present a model of interacting Majorana fermions that describes a superconducting phase with a topological order characterized by the Fibonacci topological field theory. Our theory is based on a SO(7)1=SO(7)1/(G2)1 x (G2)1 coset construction and implemented by a solvable two-dimensional network model. In addition, we predict a closely related ''anti-Fibonacci'' phase, whose topological order is characterized by the tricritical Ising model. Finally, we propose an interferometer that generalizes the Z2 Majorana interferometer and directly probes the Fibonacci non-Abelian statistics.\nFor the third part, we argue that a correlated fluid of electrons and holes can exhibit fractional quantum Hall effects at zero magnetic field. We first show that a Chern insulator can be realized as a free fermion model with p-wave(m=1) excitonic pairing. Its ground state wavefunction is then worked out and generalized to m>1. We give several pieces of evidence that this conjectured wavefunction correctly describes a topological phase, dubbed ''fractional excitonic insulator'', within the same universality class as the corresponding Laughlin state at filling 1/m. We present physical arguments that gapless states with higher angular momentum pairing between energy bands are conducive to forming the fractional excitonic insulator in the presence of repulsive interactions. Without interactions, these gapless states appear at topological phase transitions which separate the trivial insulator from a Chern insulator with higher Chern number. Since the nonvanishing density of states at these higher angular momentum band inversion transitions can give rise to interesting many-body effects, we introduce a series of minimal lattice models realizations in two dimensions. We also study the effect of rotational symmetry broken electron-hole exciton condensation in our lattice models using mean field theory.
With the discovery of the integer quantum Hall effect by von Klitzing and collaborators in 1980, the mathematical field of topology entered the world of condensed matter physics. Almost three decades later, this eventually led to the theoretical prediction and the experimental realization of many intriguing topological materials and topology-based devices. In this Ph.D. thesis, we will study the interplay between topology and another key topic in condensed matter physics, namely the study of inter-particle interactions in many-body systems. This interplay is analyzed from two different perspectives. Firstly, we studied how the presence of electron-electron interactions affects single-electron injection into a couple of counter-propagating one-dimensional edge channels. The latter appear at the edges of topologically non-trivial systems in the quantum spin Hall regime and they can also be engineered by exploiting the integer quantum Hall effect. Because of inter-channel interactions, the injected electron splits up into a couple of counter-propagating fractional excitations. Here, we carefully study and discuss their properties by means of an analytical approach based on the Luttinger liquid theory and the bosonization method. Our results are quite relevant in the context of the so-called electron quantum optics, a fast developing field which deeply exploits the topological protection of one-dimensional edge states to study the coherent propagation of electrons in solid-state devices. As an aside, we also showed that similar analytical techniques can also be used to study the time-resolved dynamics of a Luttinger liquid subject to a sudden change of the interaction strength, a protocol known as quantum quench which is gaining more and more attention, especially within the cold-atoms community. Secondly, we study how inter-particle interactions can enhance the topological properties of strictly one-dimensional fermionic systems. More precisely, the starting point is the seminal Kitaev chain, a free-fermionic lattice model which hosts exotic Majorana zero-energy modes at its ends. The latter are extremely relevant in the context of topological quantum computation because of their non-Abelian anyonic exchange statistics. Here we show that, by properly adding electron-electron interactions to the Kitaev chain, it is possible to obtain lattice models which feature zero-energy parafermionic modes, an even more intriguing generalization of Majoranas. To this end, we develop at first an exact mapping between Z4 parafermions and ordinary fermions on a lattice. We subsequently exploit this mapping to analytically obtain an exactly solvable fermionic model hosting zero-energy parafermions. We study their properties and numerically investigate their signatures and robustness even when parameters are tuned away from the exactly solvable point.
This thesis is devoted to the study of strongly correlated phases of quantum matter in two spatial dimensions. In presence of strong interactions, the electron can split up into separate spin and charge degrees of freedom. The diagnosis of such fractionalized excitations in recent experiments, as well as finding new probes for their detection, comprise the two major themes of this thesis.\nThe first part of the thesis, comprising chapters 2-6, discusses the relevance of fractionalization to the pseudogap phase of the underdoped high Tc cuprate superconductors. This is motivated by transport experiments that show a violation of Luttinger's theorem, possible only in the presence of topological order that can arise naturally as a consequence of fractionalization. Chapters 2 and 3 focus on phenomenological models with bosonic charge carriers and fermionic spin carriers, and investigate transport properties as well as various confinement transitions to symmetry broken phases. Chapters 4, 5 and 6 deal with a different framework of electron fractionalization, where the charge carriers are fermionic and spin carriers are bosonic. We find that these models can better explain the thermal and electrical transport properties in chapter 5. In chapters 6 and 7, we show how such models arise naturally from quantum fluctuations of antiferromagnetism, and can simultaneously intertwine the anti-nodal spectral gap with the discrete broken symmetries that are observed in the cuprates. \nThe second part of the thesis, comprising chapters 7 and 8, proposes new experimental probes to study the behavior of insulating two dimensional quantum magnets. Aided by geometric frustration and strong quantum fluctuations, they may realize a spin liquid ground state which can be extremely difficult to detect via conventional probes. Chapter 7 discusses how novel spin-transport probes from the spintronics community can be used to detect fractionalized excitations in a quantum spin liquid. Chapter 8 studies how the temperature dependent anisotropy of in-plane versus out-of-plane thermal conductivities can serve as an explicit signature of fractionalization in layered two-dimensional materials.
The eect of electronic many-body interactions in one-dimensional (1D) systems is drastically enhanced compared to higher dimensions due to the restricted phasespace, often leading to strong electronic correlations. It can be shown that due to a breakdown of the Fermi liquid theory, the ground state at low temperatures becomes a Tomonaga-Luttinger liquid (TLL). In a TLL, the strength of electronic correlations is characterized by the Luttinger parameter K, ranging between K = 0 and K = 1, where K = 1 describes non-interacting electrons. Various systems, such as single-walled carbon nanotubes, 1D atomic metal chains, and MoS 2 mirror twin boundaries, have been reported to host TLLs, in which spin-degeneracy is intact.
The properties of fermions in one dimension are markedly different from those in higher dimensions. In two or three dimensions, the many-body behaviour of fermions is described by the Fermi liquid model, whose most prominent result is that, instead of studying the behaviour of individual particles, it is better to describe the emergent phenomena of the whole system, known as quasiparticles. These are collective modes of excitations born out of particle-particle interactions, which resemble the constituent single particles, albeit with renormalised mass. In one dimension, however, the formation of such a correlated state is unfavourable and the quasiparticles are completely absent. Instead, 1D fermions are described by a model known as the Tomonaga-Luttinger liquid. Central to this model is the process of bosonisation, a mathematical technique which maps the excitation of fermions to bosonic modes of spin-density and charge-density waves. As a prerequisite of the bosonisation technique, the fermionic single-particle dispersion is approximated as a linear function. Consequently, the Luttinger liquid model is limited in its scope of applicability. Specifically, it is valid only in the vicinity of the Fermi points, where the excitation energy is low. Recent advancement in the theoretical field has expanded our understanding of 1D interacting fermions beyond the limit of linearity. The mobile-impurity model, proposed by L. Glazman and his co-authors, is a generalised model of 1D fermions which extends the scope of applicability of the Tomanaga-Luttinger model, accounting for the curvature of single-particle dispersion relations. It extends the region of validity of the tradition TLL theory from the neighbourhood of the Fermi points to a band which follows the single-particle dispersion. This thesis presents the results of an experimental work which provides direct evidence of non-linear behaviour predicted by the new model. It revolves around the measurement of the spectral function of electrons in surface-gate-defined quantum wires on a double-quantum-well, GaAs/AlGaAs device, and the comparison and fitting of the result to the non-linear theory. The spectral function is a theoretical concept frequently used in discussions on many-body problems. Its physical interpretation makes it closely related to experimental observables, such as the tunnelling current between the double quantum wells in this work. This thesis consists of three parts. Part one concerns the theories of the various many-body models and the experimental technique: Chapter 1 briefly introduces the concept of Fermi liquid, before focusing on a detailed account of the Luttinger-liquid model. The mobile-impurity model will be introduced in the framework of the Luttinger liquid model afterwards, followed by a review of experimental works reported in the literature on the study of TLL physics. In Chapter 2, the principles of the experimental tunnelling spectroscopy technique are described. The second part of the thesis details the structure of the test device used in the experiment and its fabrication. In particular, we will discuss the intricacies of the three-dimensional EBL fabrication process developed specifically for this project. The setup and running of the measurement circuit will also be discussed in this part of the thesis, in the context of a prerequisite sample characterisation measurement. In the final part of the work, data from the main experiment will be presented and analysed, in search for the electron-electron interaction effects which are predicted by the theoretical discussions in the first chapter.