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Binary quantum droplets and dipolar supersolids

 Joseph Smith

Published Jan 1, 2023• 0 citations
OpenAlex

Abstract

We consider a binary magnetic gas and develop an extended Gross-Pitaevskii theory to study the system. We apply this theory to the regime where the two- body interactions are attractive for some arrangements of the atoms, and mean- field theory predicts mechanical collapse. In this regime quantum droplets of the binary magnetic gas can emerge, stabilised by quantum fluctuations. These quantum droplets can exist in miscible and immiscible regimes, and we characterise their properties over a broad parameter space. Simplified theories are developed to describe the droplets, and benchmarked against the full numerical calculations. The system dynamics are simulated for scenarios involving droplet formation and crossing the miscible-immiscible transition. Three-body loss is modelled in the dynamical simulations to account for the dominant loss process expected in experiments. We also study the supersolidity of a single-component dipolar gas in an infinite tube potential. An accurate computational algorithm is developed to calculate the ground state of the system in a unit cell. This algorithm is used to determine the phase diagram by characterising the crystalline order and superfluid fraction. Our results reveal that a system confined in a radially harmonic trap has a continuous transition for a range of density values, but is discontinuous for densities above and below this range. The theory is used to calculate the crystalline and supersolid states of a binary magnetic gas in a tube potential.

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We consider a binary magnetic gas and develop an extended Gross-Pitaevskii theory to study the system. We apply this theory to the regime where the two- body interactions are attractive for some arrangements of the atoms, and mean- field theory predicts mechanical collapse. In this regime quantum droplets of the binary magnetic gas can emerge, stabilised by quantum fluctuations. These quantum droplets can exist in miscible and immiscible regimes, and we characterise their properties over a broad parameter space. Simplified theories are developed to describe the droplets, and benchmarked against the full numerical calculations. The system dynamics are simulated for scenarios involving droplet formation and crossing the miscible-immiscible transition. Three-body loss is modelled in the dynamical simulations to account for the dominant loss process expected in experiments. We also study the supersolidity of a single-component dipolar gas in an infinite tube potential. An accurate computational algorithm is developed to calculate the ground state of the system in a unit cell. This algorithm is used to determine the phase diagram by characterising the crystalline order and superfluid fraction. Our results reveal that a system confined in a radially harmonic trap has a continuous transition for a range of density values, but is discontinuous for densities above and below this range. The theory is used to calculate the crystalline and supersolid states of a binary magnetic gas in a tube potential.
We develop two approximate theories to describe the miscible and immiscible droplets that can occur in a binary mixture of highly magnetic bosonic atoms. In addition to allowing simpler calculations, the approximate theories provide insight into the role of quantum fluctuations in the two regimes. Results are validated by comparison to those from the extended Gross-Pitaevskii equation. As an application, we solve for the ground-state droplets crossing the miscible-immiscible transition as a function of the short-ranged interspecies interaction parameter. We consider regimes where the transition occurs suddenly or as a smooth cross-over. Using dynamical calculations, we show that the character of the transition is revealed in the number of domains produced when ramping the droplet into the immiscible regime.
Quantum droplets can emerge in bosonic binary magnetic gases (BMGs) from the interplay of short- and long-ranged interactions, and quantum fluctuations. We develop an extended mean field theory for this system and use it to predict equilibrium and dynamical properties of BMG droplets. We present a phase diagram and characterize miscible and immiscible droplet states. We also show that a single-component self-bound droplet can bind another magnetic component, which is not in the droplet regime, due to the interspecies dipole-dipole interactions. Our results should be realizable in experiments with mixtures of highly magnetic lanthanide atoms.
The recent realization of a binary dipolar Bose-Einstein condensate [A. Trautmann et al., Phys. Rev. Lett. 121, 213601 (2018)] presents new exciting aspects for studying quantum droplets and supersolids in a binary mixture. Motivated by this experiment, we study the ground-state phases and dynamics of a Dy-Dy mixture. The dipolar bosonic mixture exhibits qualitatively novel and rich physics. Relying on the three-dimensional numerical simulations in the extended Gross-Pitaevskii framework, we unravel the ground-state phase diagrams and characterize their different possible phases. The emergent phases include single-droplet (SD), multiple-droplets (MD), doubly supersolid (SS), and superfluid (SF) states in both miscible and immiscible phases. Intriguing mixed ground states are observed for an imbalanced binary mixture, including a combination of SS-SF, SS-MD, and SS-SS phases. We also explore the dynamics across the phase boundaries by linear quenches of interspecies and intraspecies scattering lengths. During these dynamical processes, we observe an abrupt change in phase which initially results in some instability in the system and forms some metastable states in the intermediate timescale. However, the state produced in long-time evolution is similar to our predicted ground state. Although we demonstrate the possible results for a Dy-Dy mixture and for a specific parameter range of intraspecies and interspecies scattering lengths, our results are in general valid for other dipolar mixtures and may become an important benchmark for future experimental scenarios.
This work concerns a theoretical study of a two-component ultra-cold bosonic gas of polarised magnetic dipolar atoms. The atoms interact by short-ranged contact interactions and long-ranged dipole-dipole interactions. The two components can correspond to two different spin-states of a single atomic species or two different atomic species, as realised in recent experiments. Here, we develop a general theory for the ground states and excitations of a two-component dipolar Bose-Einstein condensate. The ground states are described by dipolar Gross-Pitaevskii equations and Bogoliubov-de Gennes equations describe the excitations. We apply these theories to systems in 3D harmonic traps and a uniform planar potential. Specialised numerical methods are developed to provide accurate solutions of these equations, and to deal with the singular dipole-dipole interaction kernel. These methods involve spectral representations based on plane waves and Bessel functions. We also discuss the methods we used for obtaining ground state solutions of the nonlinear Gross-Pitaevskii energy functional. Dipole-dipole interactions can favour spatial structure, as demonstrated in the recent observation of supersolid states of matter in a single-component dipolar gas. In the two-component system these interactions can also favour a ground state with a periodic order in the pseudo-spin density. A two-component system can be either miscible (components overlap) or immiscible (components are separated). Our focus here is in the spin-stripe state, which occurs in a flattened trap geometry and involves an immiscible stripe pattern along one of the weakly trapped or untrapped directions. We examine the dynamical stability conditions of the uniform miscible state in planar confinement, and produce an associated stability phase diagram. We identify the various instabilities and analytical criteria for estimating these. We focus on the occurrence of, and conditions that favour, density-roton or spin-roton excitations, anticipating that the softening of these excitations will lead to structured ground states. To characterize these excitations we introduce density and spin dynamical structure factors, which can be measured in experiments using Bragg spectroscopy. Building on the stability phase diagram we compute ground states where the immiscible state is unstable to spin-rotons, finding triangular and stripe immiscible states with a length scale set by the confinement and interactions. We find that the transition to the stripe state is continuous and coincides with the spin-roton softening in the uniform miscible state. We study the excitations of the spin stripe state which exhibits three gapless excitation branches arising from the spontaneous broken symmetries. We identify a balanced parameter regime, where the excitations exhibit a nonsymmorphic symmetry (a symmetry is nonsymmorphic when it is a combination of point-group operations with nonprimitive lattice translations, i.e. not an integer multiple of lattice constants), which is revealed in the density and spin dynamical structure factors. We also consider the dynamics of the system following a quench from the uniform to immiscible stripe states. In the early time dynamics, a spin-stripe state is formed in a such way that the stripe order only extends over small domains. In subsequent dynamics, these domain sizes grow as the system phase-orders towards its equilibrium state. We identify the relevant topological defects such as disclinations, dislocations and grain boundaries. Using ensembles of large scale simulations we show that dynamical scaling holds for the growth of order.
The purpose of this paper is to study the dynamics of solutions to an extended Gross–Pitaevskii equation that models the formation of droplets in a dipolar Bose–Einstein condensate (BEC). The formation of these droplets has been recently discovered by driving the BEC into the strongly dipolar regime. Surprisingly, instead of collapsing, the system formed stable droplets. So far, no rigorous mathematical explanation has been proved. To the best of our knowledge, only experimental results have been obtained. The goal of this paper is to validate this breakthrough discovery. Many predictions/ conjectures properties of these droplets have been stated by some research groups in physics and engineering. In particular, it has been claimed that the stability of these droplets is a consequence of the presence of the damping term in the extended Gross–Pitaevskii equation under study. This term describes the three-body loss process. To accurately model the dynamics of formation of these droplets, it is necessary to consider a time-dependent harmonic trapping potential as well as other terms with different types of nonlinearity among them that describe the Lee–Huang–Yang (LHY). This presents some challenges that will be solved in this paper.
We calculate the ground states of a dipolar Bose gas confined in an infinite tube potential. We use the extended Gross-Pitaevskii equation theory and present a numerical method to efficiently obtain solutions. A key feature of this method is an analytic result for a truncated dipole-dipole interaction potential that enables the long-ranged interactions to be accurately evaluated within a unit cell. Our focus is on the transition of the ground state to a crystal driven by dipole-dipole interactions as the short-ranged interaction strength is varied. We find that the transition is continuous or discontinuous depending upon the average system density. These results give deeper insight into the supersolid phase transition observed in recent experiments and validate the utility of the reduced three-dimensional theory developed in [Phys. Rev. Res. 2, 043318 (2020)] for making qualitatively accurate predictions.