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Spin-stripe state of a dipolar Bose-Einstein condensate

Au-Chen Lee

Published Aug 30, 2024• 0 citations
OpenAlex

Abstract

This work concerns a theoretical study of a two-component ultra-cold bosonic gas of polarised magnetic dipolar atoms. The atoms interact by short-ranged contact interactions and long-ranged dipole-dipole interactions. The two components can correspond to two different spin-states of a single atomic species or two different atomic species, as realised in recent experiments. Here, we develop a general theory for the ground states and excitations of a two-component dipolar Bose-Einstein condensate. The ground states are described by dipolar Gross-Pitaevskii equations and Bogoliubov-de Gennes equations describe the excitations. We apply these theories to systems in 3D harmonic traps and a uniform planar potential. Specialised numerical methods are developed to provide accurate solutions of these equations, and to deal with the singular dipole-dipole interaction kernel. These methods involve spectral representations based on plane waves and Bessel functions. We also discuss the methods we used for obtaining ground state solutions of the nonlinear Gross-Pitaevskii energy functional. Dipole-dipole interactions can favour spatial structure, as demonstrated in the recent observation of supersolid states of matter in a single-component dipolar gas. In the two-component system these interactions can also favour a ground state with a periodic order in the pseudo-spin density. A two-component system can be either miscible (components overlap) or immiscible (components are separated). Our focus here is in the spin-stripe state, which occurs in a flattened trap geometry and involves an immiscible stripe pattern along one of the weakly trapped or untrapped directions. We examine the dynamical stability conditions of the uniform miscible state in planar confinement, and produce an associated stability phase diagram. We identify the various instabilities and analytical criteria for estimating these. We focus on the occurrence of, and conditions that favour, density-roton or spin-roton excitations, anticipating that the softening of these excitations will lead to structured ground states. To characterize these excitations we introduce density and spin dynamical structure factors, which can be measured in experiments using Bragg spectroscopy. Building on the stability phase diagram we compute ground states where the immiscible state is unstable to spin-rotons, finding triangular and stripe immiscible states with a length scale set by the confinement and interactions. We find that the transition to the stripe state is continuous and coincides with the spin-roton softening in the uniform miscible state. We study the excitations of the spin stripe state which exhibits three gapless excitation branches arising from the spontaneous broken symmetries. We identify a balanced parameter regime, where the excitations exhibit a nonsymmorphic symmetry (a symmetry is nonsymmorphic when it is a combination of point-group operations with nonprimitive lattice translations, i.e. not an integer multiple of lattice constants), which is revealed in the density and spin dynamical structure factors. We also consider the dynamics of the system following a quench from the uniform to immiscible stripe states. In the early time dynamics, a spin-stripe state is formed in a such way that the stripe order only extends over small domains. In subsequent dynamics, these domain sizes grow as the system phase-orders towards its equilibrium state. We identify the relevant topological defects such as disclinations, dislocations and grain boundaries. Using ensembles of large scale simulations we show that dynamical scaling holds for the growth of order.

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This work concerns a theoretical study of a two-component ultra-cold bosonic gas of polarised magnetic dipolar atoms. The atoms interact by short-ranged contact interactions and long-ranged dipole-dipole interactions. The two components can correspond to two different spin-states of a single atomic species or two different atomic species, as realised in recent experiments. Here, we develop a general theory for the ground states and excitations of a two-component dipolar Bose-Einstein condensate. The ground states are described by dipolar Gross-Pitaevskii equations and Bogoliubov-de Gennes equations describe the excitations. We apply these theories to systems in 3D harmonic traps and a uniform planar potential. Specialised numerical methods are developed to provide accurate solutions of these equations, and to deal with the singular dipole-dipole interaction kernel. These methods involve spectral representations based on plane waves and Bessel functions. We also discuss the methods we used for obtaining ground state solutions of the nonlinear Gross-Pitaevskii energy functional. Dipole-dipole interactions can favour spatial structure, as demonstrated in the recent observation of supersolid states of matter in a single-component dipolar gas. In the two-component system these interactions can also favour a ground state with a periodic order in the pseudo-spin density. A two-component system can be either miscible (components overlap) or immiscible (components are separated). Our focus here is in the spin-stripe state, which occurs in a flattened trap geometry and involves an immiscible stripe pattern along one of the weakly trapped or untrapped directions. We examine the dynamical stability conditions of the uniform miscible state in planar confinement, and produce an associated stability phase diagram. We identify the various instabilities and analytical criteria for estimating these. We focus on the occurrence of, and conditions that favour, density-roton or spin-roton excitations, anticipating that the softening of these excitations will lead to structured ground states. To characterize these excitations we introduce density and spin dynamical structure factors, which can be measured in experiments using Bragg spectroscopy. Building on the stability phase diagram we compute ground states where the immiscible state is unstable to spin-rotons, finding triangular and stripe immiscible states with a length scale set by the confinement and interactions. We find that the transition to the stripe state is continuous and coincides with the spin-roton softening in the uniform miscible state. We study the excitations of the spin stripe state which exhibits three gapless excitation branches arising from the spontaneous broken symmetries. We identify a balanced parameter regime, where the excitations exhibit a nonsymmorphic symmetry (a symmetry is nonsymmorphic when it is a combination of point-group operations with nonprimitive lattice translations, i.e. not an integer multiple of lattice constants), which is revealed in the density and spin dynamical structure factors. We also consider the dynamics of the system following a quench from the uniform to immiscible stripe states. In the early time dynamics, a spin-stripe state is formed in a such way that the stripe order only extends over small domains. In subsequent dynamics, these domain sizes grow as the system phase-orders towards its equilibrium state. We identify the relevant topological defects such as disclinations, dislocations and grain boundaries. Using ensembles of large scale simulations we show that dynamical scaling holds for the growth of order.
The work of this thesis concerns the properties of a Bose gas of polarised dipoles that have long-range and anisotropic interactions. Our work is divided into two parts. First, the stability of a dipolar Bose gas at finite temperature (both above and below the critical Bose-Einstein condensation (BEC) temperature Tc). Second, the fluctuations of a dipolar BEC at zero and small finite temperature (T ≪ Tc) in a regime where rotonic excitations emerge. \n \nPart I: Stability of a Trapped Finite Temperature Dipolar Bose Gas: Above Tc we implement a semiclassical Hartree-Fock theory and characterise the dependence of the stability boundary on temperature, trap geometry and the strength of the dipole-dipole interaction and contact interaction. We find that stability is greatly enhanced above Tc and that trap geometry continues to play a key role. Furthermore, we find that for oblate traps a novel double instability feature emerges. \nTo extend our stability analysis to the low temperature regime, T < Tc, we develop a beyond semiclassical Hartree theory. We use this to characterise the stability boundary as a function of geometry. Interestingly, we find large beyond semiclassical effects above Tc for prolate trapping geometries. We characterise thermal effects on biconcave condensate states. \n \nPart II: Rotons and Fluctuations in a Trapped Dipolar Condensate: To study density fluctuations we implement a numerical scheme to solve the Gross-Pitaevskii equation and the Bogoliubov de Gennes equations. We find that the phonon and roton gases spatially separate and we characterise the role of the anomalous density on the density fluctuations of the thermally activated rotons. We develop a numerical scheme that calculates number fluctuations within cells of various shapes and sizes, and find a strong peak in the fluctuations when the cell size is around half the roton wavelength, which should be detectable by current experiments. By tailoring the cell shape we predict that experiments should be able to detect the effects of individual roton modes. \nFor the study of zero temperature fluctuations we deploy the Gross-Pitaevskii and Bogoliubov de Gennes equations to calculate the dynamic and static structure factors for a highly oblate BEC. We find a clear signature of the roton gas dispersion relation within the structure factors. This signature should be detectible in current experiments using Bragg spectroscopy.
We consider the ground states, excitations, and dynamics of a quasi-two-dimensional binary dipolar Bose-Einstein condensate. Our focus is on the transition to a spin-stripe ground state in which the translational invariance is spontaneously broken by a striped immiscible pattern of the alternating components. We develop a ground-state phase diagram showing the parameter regime where the spin-stripe state occurs. Using Bogoliubov theory, we calculate the excitation spectrum and structure factors. We identify a balanced regime where the system has a Z2{\mathbb{Z}}_{2}Z2​ symmetry, and in the spin-stripe state this yields a nonsymmorphic symmetry. We consider the evolution of the system following a quench from the uniform to spin-stripe state, revealing ordering dynamics involving defects of the stripe order. Using an order parameter to characterize the orientational order of the stripes, we show that the phase ordering exhibits dynamic scaling.
We investigate the crystalline stationary states of a dipolar Bose-Einstein condensate in a planar trapping geometry. Our focus is on the ground state phase diagram in the thermodynamic limit, where triangular, honeycomb and stripe phases occur. We introduce a rigorous method to quantify the superfluidity of these states by analysing their nonclassical translational inertia, which allows us to identify favourable parameter regimes for observing supersolid ground states. The resulting superfluid fraction is a rank-2 tensor which is isotropic for the triangular and honeycomb states but anisotropic for the stripe case. We develop two simplified theories to approximately describe the ground states, and consider the relationship to roton softening in the uniform ground state. This also allows us to extend the phase diagram to the low density regime.
We characterize the immiscibility-miscibility transition (IMT) of a two-component Bose-Einstein condensate (BEC) with dipole-dipole interactions. In particular, we consider the quasi-two-dimensional geometry, where a strong trapping potential admits only zero-point motion in the trap direction, while the atoms are more free to move in the transverse directions. We employ the Bogoliubov treatment of the two-component system to identify both the well-known long-wavelength IMT in addition to a rotonlike IMT, where the transition occurs at finite-wave number and is reminiscent of the roton softening in the single-component dipolar BEC. Additionally, we verify the existence of the roton IMT in the fully trapped, finite systems by direct numerical simulation of the two-component coupled nonlocal Gross-Pitaevskii equations.
We develop a theory for a two-component miscible dipolar condensate in a planar trap. Using numerical solutions and a variational theory we solve for the excitation spectrum and identify regimes where density- and spin-roton excitations are favored. We characterize the various instabilities that can emerge in this system over a wide parameter regime and present results for the stability phase diagram. Importantly this allows us to identify the parameter regimes where a novel roton-immiscibility transition can occur, driven by the softening of the spin-roton excitation.
We consider a binary magnetic gas and develop an extended Gross-Pitaevskii theory to study the system. We apply this theory to the regime where the two- body interactions are attractive for some arrangements of the atoms, and mean- field theory predicts mechanical collapse. In this regime quantum droplets of the binary magnetic gas can emerge, stabilised by quantum fluctuations. These quantum droplets can exist in miscible and immiscible regimes, and we characterise their properties over a broad parameter space. Simplified theories are developed to describe the droplets, and benchmarked against the full numerical calculations. The system dynamics are simulated for scenarios involving droplet formation and crossing the miscible-immiscible transition. Three-body loss is modelled in the dynamical simulations to account for the dominant loss process expected in experiments. We also study the supersolidity of a single-component dipolar gas in an infinite tube potential. An accurate computational algorithm is developed to calculate the ground state of the system in a unit cell. This algorithm is used to determine the phase diagram by characterising the crystalline order and superfluid fraction. Our results reveal that a system confined in a radially harmonic trap has a continuous transition for a range of density values, but is discontinuous for densities above and below this range. The theory is used to calculate the crystalline and supersolid states of a binary magnetic gas in a tube potential.