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Spatio-spectral vector light created by optical activity in rubidium vapor

Richard Aguiar Maduro, Riaan Schmidt, Mustafa Al Khafaji, Craig J. A. Millar, Sphinx J. Svensson, Andrey Surzhykov, Adam Selyem, Sonja Franke‐Arnold

Published May 19, 2026• 0 citations
Publisher

Abstract

We demonstrate a pump-probe scheme in which an atomic vapor is optically pumped with circularly polarized light and probed with a vector vortex beam. The pump induces a macroscopic magnetization in the medium, which gives rise to frequency-dependent circular dichroism and birefringence. The vortex probe, characterized by spatially varying polarization, maps this optical activity onto the spatial structure of the transmitted light, thereby generating correlations between the frequency, polarization, and spatial degrees of freedom. Measuring the intensity profile in a suitable polarization component then allows us to perform spatially resolved polarization spectroscopy. We demonstrate the translation of frequency shifts into an image rotation, observing on resonance a rotation in the order of 98 mrad per MHz. These findings may find applications in high-precision spectroscopy, magnetometry, and the generation of hybrid entanglement.

DOI
10.1364/opticaopen.32316006.v1

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We demonstrate a pump-probe scheme in which an atomic vapor is optically pumped with circularly polarized light and probed with a vector vortex beam. The pump induces a macroscopic magnetization in the medium, which gives rise to frequency-dependent circular dichroism and birefringence. The vortex probe, characterized by spatially varying polarization, maps this optical activity onto the spatial structure of the transmitted light, thereby generating correlations between the frequency, polarization, and spatial degrees of freedom. Measuring the intensity profile in a suitable polarization component then allows us to perform spatially resolved polarization spectroscopy. We demonstrate the translation of frequency shifts into an image rotation, observing on resonance a rotation in the order of 98 mrad per MHz. These findings may find applications in high-precision spectroscopy, magnetometry, and the generation of hybrid entanglement.
We show that optical activity in atomic media can generate multidimensional correlations in frequency, polarization and spatial degrees of freedom, allowing us to observe frequency shifts as image rotations. Specifically, we demonstrate a pump-probe scheme, where optical pumping with circularly polarized light generates macroscopic magnetization in an atomic vapor, associated with frequency-dependent circular dichroism and birefringence. A vortex probe beam, characterized by spatially varying polarization, maps this optical activity onto the spatial structure of the transmitted light. Measuring the intensity profile in a suitable polarization component then allows us to perform spatially resolved polarization spectroscopy. On resonance we observe a rotation with a slope in the order of 98 mrad per MHz. These findings may find applications in image-based laser-locking, high-precision spectroscopy, magnetometry, and the generation of hybrid entanglement.
We show that optical activity in atomic media can generate multidimensional correlations in frequency, polarization and spatial degrees of freedom, allowing us to observe frequency shifts as image rotations. Specifically, we demonstrate a pump-probe scheme, where optical pumping with circularly polarized light generates macroscopic magnetization in an atomic vapor, associated with frequency-dependent circular dichroism and birefringence. A vortex probe beam, characterized by spatially varying polarization, maps this optical activity onto the spatial structure of the transmitted light. Measuring the intensity profile in a suitable polarization component then allows us to perform spatially resolved polarization spectroscopy. On resonance we observe a rotation with a slope in the order of 98 mrad per MHz. These findings may find applications in image-based laser-locking, high-precision spectroscopy, magnetometry, and the generation of hybrid entanglement.
Vector beams with spatially varying polarization distribution in the wavefront plane have received increasing attention in recent years. The manipulation of vector beams both in intensity and polarization distributions is highly desired and under development. In this work, we study the transmission property of vector beams through warm rubidium vapor and realize controllable transmission of vector beams based on atomic dichroism. By utilizing the linearly polarized beam and vector beams as the pump and probe beams in a pump–probe configuration, a spatially-dependent dichroism can be obtained, which leads to spatially varied absorption of the probe beam. The controllable intensity distribution of the probe beam, as a two-petal pattern, can rotate with the variation of the pump beam's polarization states. We experimentally demonstrate the mechanism of dichroism with linear polarization light and provide an explanation based on the optical pumping effect. Alternatively, the varying trend of the probe beam's intensity is also interpreted by utilizing the Jones matrix. Our results are thus beneficial for providing potential applications in optical manipulation in atomic ensembles.
We numerically investigate the transfer of optical information from a vector-vortex control beam to an unstructured probe beam, as mediated by an atomic vapour. The right and left circular components of these beams drive the atomic transitions of a double-V system, with the atoms acting as a spatially varying circular birefringent medium. Modeling the propagation of the light fields, we find that, for short distances, the vectorial light structure is transferred from the control field to the probe. However, for larger propagation lengths, diffraction causes the circular components of the probe field to spatially separate. We model this system for the D1 line of cold rubidium atoms and demonstrate that four wave mixing can lead to correlations between the optical polarization structure and the diffraction of light, generating coupled dynamics of the internal and external degrees of freedom.
Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.
Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.