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arXiv:2203.05188 · Optics Express

Transfer and evolution of structured polarization in a double-V atomic system

Zhenzhu Li, Sonja Franke‐Arnold, Thomas W. Clark, Jinwen Wang, Dawei Zhang, Chunfang Wang

Published May 11, 2022• 11 citations
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Abstract

We numerically investigate the transfer of optical information from a vector-vortex control beam to an unstructured probe beam, as mediated by an atomic vapour. The right and left circular components of these beams drive the atomic transitions of a double-V system, with the atoms acting as a spatially varying circular birefringent medium. Modeling the propagation of the light fields, we find that, for short distances, the vectorial light structure is transferred from the control field to the probe. However, for larger propagation lengths, diffraction causes the circular components of the probe field to spatially separate. We model this system for the D1 line of cold rubidium atoms and demonstrate that four wave mixing can lead to correlations between the optical polarization structure and the diffraction of light, generating coupled dynamics of the internal and external degrees of freedom.

DOI
10.1364/oe.457368

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We numerically investigate the transfer of optical information from a vector-vortex control beam to an unstructured probe beam, as mediated by an atomic vapour. The right and left circular components of these beams drive the atomic transitions of a double-V system, with the atoms acting as a spatially varying circular birefringent medium. Modeling the propagation of the light fields, we find that, for short distances, the vectorial light structure is transferred from the control field to the probe. However, for larger propagation lengths, diffraction causes the circular components of the probe field to spatially separate. We model this system for the D1 line of cold rubidium atoms and demonstrate that four wave mixing can lead to correlations between the optical polarization structure and the diffraction of light, generating coupled dynamics of the internal and external degrees of freedom.
We consider the optical rotation of the polarization of a linearly polarized probe field passing through an M-type atomic system by using the interaction between two vortex control fields and optical transitions. We investigate theoretically to generate the spatially dependent structured light with the atoms acting as a spatially varying circular birefringent medium. We show that the polarization and intensity distributions of the vector beam spatially vary by changing the orbital angular momentum (OAM) of the vortex control field.
We investigate the propagation of an optical vector vortex beam in an atomic medium featuring four-level tripod transitions, where ground-state coherence is mediated by a transverse magnetic field. The vector beam consists of left- and right-circularly polarized components, each carrying an optical vortex with opposite orbital angular momentum (OAM). We study the linear response of the medium to the vector beam in order to determine the evolution of the beam's intensity and polarization profile. We find that the beam structure undergoes significant transformations as it propagates: the transverse intensity evolves from a ring-shaped profile to a petal-like structure, while the polarization transitions between left-circular, linear, and right-circular polarizations. Furthermore, when only the right-circular polarization component (a scalar vortex) enters the medium, it parametrically generates a left-circular polarization component, transferring its OAM to the generated field. This process converts the initial vortex beam into a superposition of left- and right-circular components, forming a scalar vortex beam where both polarization components carry the same OAM.
We demonstrate a pump-probe scheme in which an atomic vapor is optically pumped with circularly polarized light and probed with a vector vortex beam. The pump induces a macroscopic magnetization in the medium, which gives rise to frequency-dependent circular dichroism and birefringence. The vortex probe, characterized by spatially varying polarization, maps this optical activity onto the spatial structure of the transmitted light, thereby generating correlations between the frequency, polarization, and spatial degrees of freedom. Measuring the intensity profile in a suitable polarization component then allows us to perform spatially resolved polarization spectroscopy. We demonstrate the translation of frequency shifts into an image rotation, observing on resonance a rotation in the order of 98 mrad per MHz. These findings may find applications in high-precision spectroscopy, magnetometry, and the generation of hybrid entanglement.
We investigate the propagation of optical vector vortices of slow light in a coherently prepared four-level tripod atomic system. The vector vortex consists of superposed pulse pairs with opposite circular polarizations and orbital angular momentum (OAM) charges ±l\pm l±l, weakly interacting with an atomic medium initially prepared in a coherent superposition of two ground states. A third unoccupied state is coupled to a stronger control laser without OAM, creating a phase-dependent configuration. In the linear regime, the vortex OAM is mapped onto the medium, producing symmetrical azimuthally structured absorption patterns, with losses significantly reduced by the control field. For small detunings, complementary spatially dependent amplification and absorption occur for the two circular polarization components. This OAM-structured coherence induces a dynamical anisotropy, affecting both the intensity and polarization of the slow-light vortex. Polarization states evolve periodically between left-circular, linear, and right-circular polarizations during propagation. Once the beam reaches a stationary regime, the ring-shaped intensity transforms into a petal-like structure, and the final polarization states stabilize according to the initial superposition. The rate of polarization transitions is tunable via the control field strength, demonstrating flexible control over slow-light vector vortex dynamics.
We investigate the propagation of an optical vector vortex weakly interacting with a coherently prepared atomic medium (phaseonium) in a three-level ΛΛΛ configuration. The vector beam consists of vortex pulse pairs with right- and left-circular polarizations, corresponding to opposite spin angular momentum (SAM), and carrying opposite orbital angular momentum (OAM) charges ±l\pm l±l. We show that during the propagation of the vortex pairs, analytically obtained in the linear regime, the medium inherits the topology of the vortex pair, mapping the OAM onto a spatially structured atomic coherence. This mapping produces 2∣l∣−2|l|-2∣l∣−fold azimuthal transparency structures that reshape the beam intensity from a ring into a petal-like pattern. The OAM-structured atomic coherence induces a corresponding optical anisotropy within the medium, which feeds back into the propagating vector beam, resulting in optical spin-orbit coupling manifested as SAM exchange, rotation, and evolution of polarization textures. Depending on the initial ground-state population of the phaseonium, the polarization state evolves between left-circular, linear, and right-circular polarizations.
We show that optical activity in atomic media can generate multidimensional correlations in frequency, polarization and spatial degrees of freedom, allowing us to observe frequency shifts as image rotations. Specifically, we demonstrate a pump-probe scheme, where optical pumping with circularly polarized light generates macroscopic magnetization in an atomic vapor, associated with frequency-dependent circular dichroism and birefringence. A vortex probe beam, characterized by spatially varying polarization, maps this optical activity onto the spatial structure of the transmitted light. Measuring the intensity profile in a suitable polarization component then allows us to perform spatially resolved polarization spectroscopy. On resonance we observe a rotation with a slope in the order of 98 mrad per MHz. These findings may find applications in image-based laser-locking, high-precision spectroscopy, magnetometry, and the generation of hybrid entanglement.