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Письма в Журнал экспериментальной и теоретической физики

Observation of the Strong Magneto-Optical Rotation of the Polarization of Light in Rubidium Vapor for Applications in Atomic Magnetometry

A. O Makarov, Denis V. Brazhnikov, Andrei Goncharov

Published Apr 15, 2023• 1 citation
Publisher

Abstract

Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.

DOI
10.31857/s1234567823070054

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Observation of the Strong Magneto-Optical Rotation of the Polarization of Light in Rubidium Vapor for Applications in Atomic Magnetometry

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Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.

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Rubidium atomic magnetometer based on pump-probe nonlinear magneto-optical rotation

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We report a rubidium atomic magnetometer based on pump-probe nonlinear magneto-optical rotation. The rubidium vapor cell is placed in a five-layer magnetic shield with inner coils that can generate uniform magnetic fields along the direction of pump beam, and the cell is also placed in the center of a Helmholtz coil that can generate an oscillating magnetic field perpendicular to the direction of pump beam. The atoms are optically pumped by circularly polarized pump beam along a constant magnetic field in a period of time, then the pump beam is turned off and a /2 pulse of oscillating magnetic field for 87Rb atoms is applied. After the above process, the individual atomic magnetic moments become phase coherent, resulting in a transverse magnetization vector precessing at the Larmor frequency in the magnetic field. The linearly polarized probing beam is perpendicular to the direction of magnetic field, and can be seen as a superposition of the left and right circularly polarized light. Because of the different absorptions and dispersions of the left and right circularly polarized light by rubidium atoms, the polarization direction of probing beam rotates when probing beam passes through rubidium vapor cell. The rotation of the polarization is subsequently converted into an electric signal through a polarizing beam splitter. Finally, the decay signal related to the transverse magnetization vector is measured. The Larmor frequency proportional to magnetic field is obtained by the Fourier transform of the decay signal. The value of magnetic field is calculated from the formula:B=(2/) f, where and f are the gyromagnetic ratio and Larmor frequency, respectively. In order to measure the magnetic field in a wide range, the tracking lock mode is proposed and tested. The atomic magnetometer can track the magnetic field jump of 1000 nT or 10000 nT, indicating that the atomic magnetometer has strong locking ability and can be easily locked after start-up. The main performances in different magnetic fields are tested. The results show that the measurement range of the atomic magnetometer is from 100 nT to 100000 nT, the extreme sensitivity is 0.2 pT/Hz1/2, and the magnetic field resolution is 0.1 pT. The transverse relaxation times of the transverse magnetization vector in different magnetic fields are obtained, and the relaxation time decreases with the increase of the magnetic field. When the measurement range is from 5000 nT to 100000 nT, the magnetic field sampling rate of the atomic magnetometer can be adjusted in a range from 1 Hz to 1000 Hz. The atomic magnetometer in high sampling rate can measure weak alternating magnetic field at low frequency. This paper provides an important reference for developing the atomic magnetometer with large measurement range, high sensitivity and high sampling rate.

Acta Physica Sinica•Jan 1, 2017•11 citations
Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.
Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.
A new configuration for observation of magneto-optical subnatural-linewidth resonances of electromagnetically induced absorption (EIA) in alkali vapor has been verified experimentally. The configuration includes using two counter-propagating pump and probe light waves with mutually orthogonal linear polarizations, exciting an open optical transition of an alkali atom in the presence of a buffer gas. The main advantage of the novel observation scheme consists in the possibility of obtaining simultaneously high-contrast and quite narrow nonlinear signals. Here a 2.5-cm long rubidium-87 vapor cell filled with Ar buffer gas is used, and the excited optical transition is the Fg_gg​=2 →\to→ Fe_ee​=1 of the D1_11​ line. The signals registered reach a contrast of 57.7% with a FWHM of 7.2 mG. The contrast with respect to a wide Doppler pedestal well exceeds 100%. To our knowledge, to date this is the best result for EIA resonances in terms of contrast-to-width ratio. In general, the results demonstrate that the new magneto-optical scheme has very good prospects for various applications in quantum metrology, nonlinear optics and photonics.
A self-oscillating magnetometer based on nonlinear magneto-optical rotation using amplitude-modulated pump light and unmodulated probe light (AM-NMOR) in 87Rb has been constructed and tested towards a goal of airborne detection of magnetic anomalies. In AM-NMOR, stroboscopic optical pumping via amplitude modulation of the pump beam creates alignment of the ground electronic state of the rubidium atoms. The Larmor precession causes an ac rotation of the polarization of a separate probe beam; the polarization rotation frequency provides a measure of the magnetic field. An anti-relaxation coating on the walls of the atomic vapor cell results in a long lifetime of 56 ms for the alignment, which enables precise measurement of the precession frequency. Light is delivered to the magnetometer by polarization-maintaining optical fibers. Tests of the sensitivity include directly measuring the beat frequency between the magnetometer and a commercial instrument and measurements of Earth's field under magnetically quiet conditions, indicating a sensitivity of at least 5 pT/νHz. Rotating the sensor indicates a heading error of less than 1 nT, limited in part by residual magnetism of the sensor.
Large Faraday rotations can be generated by circular birefringence of atomic samples in an axial magnetic field in the vicinity of atomic resonance lines. More generally, magneto-optical effects in atomic samples include circular dichroism in addition to birefringence, resulting in a modification of the ellipticity as well as the polarization alignment. Usually such effects are investigated for homogeneous linear polarizations, but the mechanisms apply also to polarization structures such as vector vortices. We investigate the effect of optical activity of a rubidium vapor in the hyperfine Paschen–Back regime along the D2 line, for the example of azimuthally polarized input light. We show that for low atomic densities, circular birefringence dominates over dichroism, and azimuthal polarization is rotated toward radial polarization. The rotation angle increases with increasing optical densities. At high vapor temperatures, dichroism becomes more and more relevant, leading to intricate variations of both alignment and ellipticity. Our results shine new light on the interplay between different magneto-optic effects at strong magnetic fields. Their highly sensitive response to detuning may find applications in spectroscopy and quantum sensing.
Nonlinear magneto-optical rotation (NMOR) of linearly polarized light, resonant to the Fg = 2 → Fe = 1 atomic transition of D1 line of 87Rb is investigated experimentally, by applying spatially separated laser fields in the Rb vacuum cell. In our experiment, the probe laser beam propagates through the center of the pump laser beam, which has the shape of a hollow cylinder. We have measured the rotation of the probe laser beam polarization with respect to the incident polarization, as a function of the external magnetic field, parallel to the laser beam propagation. We show substantial narrowing of the resonance if the pump beam, with the same linear polarization, is present. The opposite direction of the probe rotation was obtained when the pump laser beam polarization is orthogonal to the probe laser beam polarization.
We report a rubidium atomic magnetometer based on pump-probe nonlinear magneto-optical rotation. The rubidium vapor cell is placed in a five-layer magnetic shield with inner coils that can generate uniform magnetic fields along the direction of pump beam, and the cell is also placed in the center of a Helmholtz coil that can generate an oscillating magnetic field perpendicular to the direction of pump beam. The atoms are optically pumped by circularly polarized pump beam along a constant magnetic field in a period of time, then the pump beam is turned off and a /2 pulse of oscillating magnetic field for 87Rb atoms is applied. After the above process, the individual atomic magnetic moments become phase coherent, resulting in a transverse magnetization vector precessing at the Larmor frequency in the magnetic field. The linearly polarized probing beam is perpendicular to the direction of magnetic field, and can be seen as a superposition of the left and right circularly polarized light. Because of the different absorptions and dispersions of the left and right circularly polarized light by rubidium atoms, the polarization direction of probing beam rotates when probing beam passes through rubidium vapor cell. The rotation of the polarization is subsequently converted into an electric signal through a polarizing beam splitter. Finally, the decay signal related to the transverse magnetization vector is measured. The Larmor frequency proportional to magnetic field is obtained by the Fourier transform of the decay signal. The value of magnetic field is calculated from the formula:B=(2/) f, where and f are the gyromagnetic ratio and Larmor frequency, respectively. In order to measure the magnetic field in a wide range, the tracking lock mode is proposed and tested. The atomic magnetometer can track the magnetic field jump of 1000 nT or 10000 nT, indicating that the atomic magnetometer has strong locking ability and can be easily locked after start-up. The main performances in different magnetic fields are tested. The results show that the measurement range of the atomic magnetometer is from 100 nT to 100000 nT, the extreme sensitivity is 0.2 pT/Hz1/2, and the magnetic field resolution is 0.1 pT. The transverse relaxation times of the transverse magnetization vector in different magnetic fields are obtained, and the relaxation time decreases with the increase of the magnetic field. When the measurement range is from 5000 nT to 100000 nT, the magnetic field sampling rate of the atomic magnetometer can be adjusted in a range from 1 Hz to 1000 Hz. The atomic magnetometer in high sampling rate can measure weak alternating magnetic field at low frequency. This paper provides an important reference for developing the atomic magnetometer with large measurement range, high sensitivity and high sampling rate.