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Optical atomic magnetometer

Dmitry Budker

Published Jan 23, 2023• 0 citations
OpenAlex

Abstract

An optical atomic magnetometers is provided operating on the principles of nonlinear magneto-optical rotation. An atomic vapor is optically pumped using linearly polarized modulated light. The vapor is then probed using a non-modulated linearly polarized light beam. The resulting modulation in polarization angle of the probe light is detected and used in a feedback loop to induce self-oscillation at the resonant frequency.

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Introduction Shortly after the inception of atomic magnetometry, alkali-vapor magnetometers were being used to measure the Earth's magnetic field to unprecedented precision. During the same era, Bell and Bloom first demonstrated all-optical atomic magnetometry through synchronous optical pumping [1] (see Chapters 1 and 6). In this approach, optical-pumping light is frequency- or amplitude-modulated at harmonics of the Larmor frequency ω L to generate a precessing spin polarization within an alkali vapor at finite magnetic field [2, 3]. Although this technique received considerable attention from the atomic physics community for its applicability to optical pumping experiments, Earth's-field alkali-vapor atomic magnetometers continued to rely on radiofrequency (RF) field excitation for several decades (see Chapter 4). Upon the advent of diode lasers addressing alkali and metastable helium transitions, synchronously pumped magnetometers experienced a revival beginning in the late 1980s. In recent years, such magnetometers have found applications in nuclear magnetic resonance detection [4] (see also Chapter 14), quantum control experiments [5], and chip-scale devices intended for spacecraft use [6] (see also Chapters 7 and 15). All-optical magnetometers possess several advantages over devices that employ RF coils. RF-driven magnetometers can suffer from cross-talk if two sensors are placed in close proximity, since the AC magnetic field driving resonance in one vapor cell can adversely affect the other. All-optical magnetometers are free from such interference. When operated in self-oscillating mode [7], RF-driven magnetometers require an added ±90° electronic phase shift in the feedback loop to counter the intrinsic phase shift between the RF field and the probe-beam modulation.

Cambridge University Press eBooks•Mar 7, 2013•0 citations

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D. C. Hovde, Eric Corsini

A method has been developed to mechanically implement the optical phase shift by adjusting the polarization of the pump and probe beams in an NMOR (nonlinear magneto-optical rotation) magnetometer as the proper phase shift is necessary to induce self-oscillation. This innovation consists of mounting the pump beam on a ring that surrounds the atomic vapor sample. The propagation of the probe beam is perpendicular to that of the pump beam. The probe beam can be considered as defining the axis of a cylinder, while the pump beam is directed radially. The magnetic field to be measured defines a third vector, but it is also taken to lie along the cylinder axis. Both the pump and probe beams are polarized such that their electric field vectors are substantially perpendicular to the magnet field. By rotation of the ring supporting the pump beam, its direction can be varied relative to the plane defined by the probe electric field and the magnetic field to be measured.

•Jan 1, 2011•0 citations
An optical atomic magnetometers is provided operating on the principles of nonlinear magneto-optical rotation. An atomic vapor is optically pumped using linearly polarized modulated light. The vapor is then probed using a non-modulated linearly polarized light beam. The resulting modulation in polarization angle of the probe light is detected and used in a feedback loop to induce self-oscillation at the resonant frequency.
A self-oscillating magnetometer based on nonlinear magneto-optical rotation using amplitude-modulated pump light and unmodulated probe light (AM-NMOR) in 87Rb has been constructed and tested towards a goal of airborne detection of magnetic anomalies. In AM-NMOR, stroboscopic optical pumping via amplitude modulation of the pump beam creates alignment of the ground electronic state of the rubidium atoms. The Larmor precession causes an ac rotation of the polarization of a separate probe beam; the polarization rotation frequency provides a measure of the magnetic field. An anti-relaxation coating on the walls of the atomic vapor cell results in a long lifetime of 56 ms for the alignment, which enables precise measurement of the precession frequency. Light is delivered to the magnetometer by polarization-maintaining optical fibers. Tests of the sensitivity include directly measuring the beat frequency between the magnetometer and a commercial instrument and measurements of Earth's field under magnetically quiet conditions, indicating a sensitivity of at least 5 pT/νHz. Rotating the sensor indicates a heading error of less than 1 nT, limited in part by residual magnetism of the sensor.
The detection of nonlinear magneto-optical rotation (NMOR) of polarized light through alkali atomic vapor is a highly sensitive technique for measuring magnetic fields. We demonstrate that when using frequency modulated light to excite the NMOR resonance, it is possible to cause the system to self-oscillate. The NMOR signal is not a simple replica of the sine wave modulation of the light, but rather contains many higher harmonics of the modulation frequency, and we implement two ways of processing the signal to recover the fundamental modulation frequency in the feedback loop and induce self-oscillation. Self-oscillation simplifies and reduces the power consumption of the electronics required to operate a magnetometer, making the NMOR technique attractive for commercialized magnetic sensors.
Introduction Shortly after the inception of atomic magnetometry, alkali-vapor magnetometers were being used to measure the Earth's magnetic field to unprecedented precision. During the same era, Bell and Bloom first demonstrated all-optical atomic magnetometry through synchronous optical pumping [1] (see Chapters 1 and 6). In this approach, optical-pumping light is frequency- or amplitude-modulated at harmonics of the Larmor frequency ω L to generate a precessing spin polarization within an alkali vapor at finite magnetic field [2, 3]. Although this technique received considerable attention from the atomic physics community for its applicability to optical pumping experiments, Earth's-field alkali-vapor atomic magnetometers continued to rely on radiofrequency (RF) field excitation for several decades (see Chapter 4). Upon the advent of diode lasers addressing alkali and metastable helium transitions, synchronously pumped magnetometers experienced a revival beginning in the late 1980s. In recent years, such magnetometers have found applications in nuclear magnetic resonance detection [4] (see also Chapter 14), quantum control experiments [5], and chip-scale devices intended for spacecraft use [6] (see also Chapters 7 and 15). All-optical magnetometers possess several advantages over devices that employ RF coils. RF-driven magnetometers can suffer from cross-talk if two sensors are placed in close proximity, since the AC magnetic field driving resonance in one vapor cell can adversely affect the other. All-optical magnetometers are free from such interference. When operated in self-oscillating mode [7], RF-driven magnetometers require an added ±90° electronic phase shift in the feedback loop to counter the intrinsic phase shift between the RF field and the probe-beam modulation.
Specific types of atomic coherences between Zeeman sublevels can be generated and detected using a method based on nonlinear magneto-optical rotation with frequency-modulated light. Linearly polarized, frequency-modulated light is employed to selectively generate ground-state coherences between Zeeman sublevels for which $\mathrm{\ensuremath{\Delta}}m=2$ and $\mathrm{\ensuremath{\Delta}}m=4$ in 85Rb^{85}\mathrm{Rb}85Rb and 87Rb^{87}\mathrm{Rb}87Rb atoms, and additionally $\mathrm{\ensuremath{\Delta}}m=6$ in 85Rb^{85}\mathrm{Rb}85Rb. The atomic coherences are detected with a separate, unmodulated probe light beam. Separation of the pump and probe beams enables independent investigation of the processes of creation and detection of the atomic coherences. With the present technique the transfer of the Zeeman coherences, including high-order coherences, from excited to ground state by spontaneous emission has been observed.
A method has been developed to mechanically implement the optical phase shift by adjusting the polarization of the pump and probe beams in an NMOR (nonlinear magneto-optical rotation) magnetometer as the proper phase shift is necessary to induce self-oscillation. This innovation consists of mounting the pump beam on a ring that surrounds the atomic vapor sample. The propagation of the probe beam is perpendicular to that of the pump beam. The probe beam can be considered as defining the axis of a cylinder, while the pump beam is directed radially. The magnetic field to be measured defines a third vector, but it is also taken to lie along the cylinder axis. Both the pump and probe beams are polarized such that their electric field vectors are substantially perpendicular to the magnet field. By rotation of the ring supporting the pump beam, its direction can be varied relative to the plane defined by the probe electric field and the magnetic field to be measured.