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Heralded quantum interference in integrated lithium niobate nanophotonics

Tristan Kuttner, Alessandra Sabatti, Jost Kellner, Rachel Grange, Robert J. Chapman

Published Apr 25, 2026• 0 citations
Publisher

Abstract

Photonics has emerged as one of the leading platforms for the implementation of real-world-applicable quantum technologies, enabling secure communication, enhanced sensing capabilities, as well as resolving previously intractable computational challenges. However, to harness the full potential of the photonics platform, several engineering feats need to be accomplished; among those is the quest for a scalable source of pure single photons. While single photon sources can be implemented in a variety of different ways, integrated lithium niobate stands out as a prime contender for a monolithic quantum photonics platform, given its second-order nonlinearity and proven classical scalability. Despite the extensive effort put into developing the platform, integrating suitable photon pair sources remains a hurdle limiting the scalability of quantum photonic systems in lithium niobate. We engineer three-wave-mixing in a nanophotonic lithium niobate device, integrating multiple near-perfect spectrally separable heralded single photon sources. By mixing photons generated via the developed sources, we show bosonic interference between indistinguishable photons—a crucial interaction for many photonic quantum computing protocols. This demonstration of proof-of-principle heralded multi-source interference in integrated lithium niobate contributes towards a scalable quantum photonics platform.

DOI
10.3929/ethz-c-000799503

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Photonics has emerged as one of the leading platforms for the implementation of real-world-applicable quantum technologies, enabling secure communication, enhanced sensing capabilities, as well as resolving previously intractable computational challenges. However, to harness the full potential of the photonics platform, several engineering feats need to be accomplished; among those is the quest for a scalable source of pure single photons. While single photon sources can be implemented in a variety of different ways, integrated lithium niobate stands out as a prime contender for a monolithic quantum photonics platform, given its second-order nonlinearity and proven classical scalability. Despite the extensive effort put into developing the platform, integrating suitable photon pair sources remains a hurdle limiting the scalability of quantum photonic systems in lithium niobate. We engineer three-wave-mixing in a nanophotonic lithium niobate device, integrating multiple near-perfect spectrally separable heralded single photon sources. By mixing photons generated via the developed sources, we show bosonic interference between indistinguishable photons—a crucial interaction for many photonic quantum computing protocols. This demonstration of proof-of-principle heralded multi-source interference in integrated lithium niobate contributes towards a scalable quantum photonics platform.
Photonics has emerged as one of the leading platforms for the implementation of real-world-applicable quantum technologies, enabling secure communication, enhanced sensing capabilities, as well as resolving previously intractable computational challenges. However, to harness the full potential of the photonics platform, several engineering feats need to be accomplished; among those is the quest for a scalable source of pure single photons. While single photon sources can be implemented in a variety of different ways, integrated lithium niobate stands out as a prime contender for a monolithic quantum photonics platform, given its second-order nonlinearity and proven classical scalability. Despite the extensive effort put into developing the platform, integrating suitable photon pair sources remains a hurdle limiting the scalability of quantum photonic systems in lithium niobate. We engineer three-wave-mixing in a nanophotonic lithium niobate device, integrating multiple near-perfect spectrally separable heralded single photon sources. By mixing photons generated via the developed sources, we show bosonic interference between indistinguishable photons—a crucial interaction for many photonic quantum computing protocols. This demonstration of proof-of-principle heralded multi-source interference in integrated lithium niobate contributes towards a scalable quantum photonics platform.
Quantum technologies have surpassed classical systems by leveraging the unique properties of superposition and entanglement in photons and matter. Recent advancements in integrated quantum photonics, especially in silicon-based and lithium niobate platforms, are pushing the technology toward greater scalability and functionality. Silicon circuits have progressed from centimeter-scale, dual-photon systems to millimeter-scale, high-density devices that integrate thousands of components, enabling sophisticated programmable manipulation of multi-photon states. Meanwhile, lithium niobate, thanks to its wide optical transmission window, outstanding nonlinear and electro-optic coefficients, and chemical stability, has emerged as an optimal substrate for fully integrated photonic quantum chips. Devices made from this material exhibit high efficiency in in generating, manipulating, converting, storing, and detecting photon states, thereby establishing a basis for deterministic multi-photon generation and single-photon quantum interactions, as well as comprehensive frequency-state control. This review explores the development of integrated photonic quantum technologies based on both silicon and lithium niobate, highlighting invaluable insights gained from silicon-based systems that can assist the scaling of lithium niobate technologies. It examines the functional integration mechanisms of lithium niobate in electro-optic tuning and nonlinear energy conversion, showcasing its transformative impact throughout the photonic quantum computing process. Looking ahead, we speculate on the developmental pathways for lithium niobate platforms and their potential to revolutionize areas such as quantum communication, complex system simulation, quantum sampling, and optical quantum computing paradigms.
Existing nonlinear-optic implementations of pure, unfiltered heralded single-photon sources do not offer the scalability required for densely integrated quantum networks. Additionally, lithium niobate has hitherto been unsuitable for such use due to its material dispersion. We engineer the dispersion and the quasi-phasematching conditions of a waveguide in the rapidly emerging thin-film lithium niobate platform to generate spectrally separable photon pairs in the telecommunications band. Such photon pairs can be used as spectrally pure heralded single-photon sources in quantum networks. We estimate a heralded-state spectral purity of >94% based on joint spectral intensity measurements. Further, a joint spectral phase-sensitive measurement of the unheralded time-integrated second-order correlation function yields a heralded-state purity of ( 86 ± 5 ) % .
Quantum photonic technologies rely on the ability to generate, manipulate, and interfere indistinguishable single photons on a scalable platform. Among the various approaches, spontaneous parametric down-conversion (SPDC) remains one of the most widely used methods for generating entangled photon pairs and pure heralded single photons. However, most integrated SPDC sources relying on co-propagating geometries have a limited purity of heralded photons or require lossy filtering. Type-2 SPDC processes can produce pure separable photons but typically suffer from lower efficiency and added complexity due to polarization management. Here we show the first integrated counter-propagating photon-pair source on lithium niobate on insulator, where signal and idler photons are generated in opposite directions. The counter-propagating geometry leads to spectrally uncorrelated photon pairs without spectral filtering. The joint spectral intensity measurements and unheralded g (2) correlations yield purities of (92 ± 3)%. Interference between two independent sources achieves heralded visibilities of (71 ± 3)%, confirming the scalability of the platform. These results establish a new route towards integrated, high-purity, and tunable photon sources. The demonstrated counter-propagating geometry offers a scalable solution for quantum photonic networks.
Generating and interfering nonclassical states of light is fundamental to optical quantum information science and technology. Quantum photonic integrated circuits provide one pathway towards scalability by combining nonlinear sources of nonclassical light and programmable circuits in centimeter-scale devices. The key requirements for quantum applications include efficient generation of indistinguishable photon-pairs and high-visibility programmable quantum interference. Here, we demonstrate a lithium niobate-on-insulator (LNOI) integrated photonic circuit that generates a two-photon path-entangled state, and a programmable interferometer for quantum interference. We generate entangled photons with ∼2.3×10^{8} pairs/s/mW brightness and perform quantum interference experiments on the chip with 96.8±3.6% visibility. LNOI is an emerging photonics technology that has revolutionized high-speed modulators and efficient frequency conversion. Our results provide a path towards large-scale integrated quantum photonics including efficient photon-pair generation and programmable circuits for applications such as boson sampling and quantum communications.
Quantum photonic technologies rely on the ability to generate, manipulate, and interfere indistinguishable single photons on a scalable platform. Among the various approaches, spontaneous parametric down-conversion (SPDC) remains one of the most widely used methods for generating entangled photon pairs and pure heralded single photons. However, most integrated SPDC sources relying on co-propagating geometries have a limited purity of heralded photons or require lossy filtering. Type-2 SPDC processes can produce pure separable photons but typically suffer from lower efficiency and added complexity due to polarization management. Here we show the first integrated counter-propagating photon-pair source on lithium niobate on insulator, where signal and idler photons are generated in opposite directions. The counter-propagating geometry leads to spectrally uncorrelated photon pairs without spectral filtering. The joint spectral intensity measurements and unheralded g(2) correlations yield purities of (92 ± 3)degrees lc. Interference between two independent sources achieves heralded visibilities of (71 ± 3)degrees lc, confirming the scalability of the platform. These results establish anew route towards integrated, high-purity, and tunable photon sources. The demonstrated counter-propagating geometry offers a scalable solution for quantum photonic networks.