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Counter-propagating spontaneous parametric down-conversion source in lithium niobate on insulator

Jost Kellner, Alessandra Sabatt, Tristan Kuttner, Robert J. Chapman, Rachel Grange

Published Apr 25, 2026• 0 citations
Publisher

Abstract

Quantum photonic technologies rely on the ability to generate, manipulate, and interfere indistinguishable single photons on a scalable platform. Among the various approaches, spontaneous parametric down-conversion (SPDC) remains one of the most widely used methods for generating entangled photon pairs and pure heralded single photons. However, most integrated SPDC sources relying on co-propagating geometries have a limited purity of heralded photons or require lossy filtering. Type-2 SPDC processes can produce pure separable photons but typically suffer from lower efficiency and added complexity due to polarization management. Here we show the first integrated counter-propagating photon-pair source on lithium niobate on insulator, where signal and idler photons are generated in opposite directions. The counter-propagating geometry leads to spectrally uncorrelated photon pairs without spectral filtering. The joint spectral intensity measurements and unheralded g(2) correlations yield purities of (92 ± 3)degrees lc. Interference between two independent sources achieves heralded visibilities of (71 ± 3)degrees lc, confirming the scalability of the platform. These results establish anew route towards integrated, high-purity, and tunable photon sources. The demonstrated counter-propagating geometry offers a scalable solution for quantum photonic networks.

DOI
10.3929/ethz-c-000800375

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Recent advances of high-quality lithium niobate (LN) on insulator technology have revitalized the progress of novel chip-integrated LN-based photonic devices and accelerated application research. One of the promising technologies of interest is the generation of entangled photon pairs based on spontaneous parametric down-conversion (SPDC) in LNs. In this paper, we investigated, theoretically and numerically, Type II SPDC in two kinds of LNs—undoped and 5-mol% MgO doped LNs. In each case, both non-poled and periodically poled crystals were considered. The technique is based on the SPDC under Type II extended phase matching, where the phase matching and the group velocity matching are simultaneously achieved between interacting photons. The proposed approach has not yet been reported for LNs. We discussed all factors required to generate photon pairs in LNs, in terms of the beam propagation direction, the spectral position of photons, and the corresponding effective nonlinearities and walk-offs. We showed that the spectral positions of the generated photon pairs fall into the mid-infrared region with high potential for free-space quantum communication, spectroscopy, and high-sensitivity metrology. The joint spectral analyses showed that photon pairs can be generated with high purities of 0.995–0.999 with proper pump filtering.

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Quantum photonic technologies rely on the ability to generate, manipulate, and interfere indistinguishable single photons on a scalable platform. Among the various approaches, spontaneous parametric down-conversion (SPDC) remains one of the most widely used methods for generating entangled photon pairs and pure heralded single photons. However, most integrated SPDC sources relying on co-propagating geometries have a limited purity of heralded photons or require lossy filtering. Type-2 SPDC processes can produce pure separable photons but typically suffer from lower efficiency and added complexity due to polarization management. Here we show the first integrated counter-propagating photon-pair source on lithium niobate on insulator, where signal and idler photons are generated in opposite directions. The counter-propagating geometry leads to spectrally uncorrelated photon pairs without spectral filtering. The joint spectral intensity measurements and unheralded g(2) correlations yield purities of (92 ± 3)degrees lc. Interference between two independent sources achieves heralded visibilities of (71 ± 3)degrees lc, confirming the scalability of the platform. These results establish anew route towards integrated, high-purity, and tunable photon sources. The demonstrated counter-propagating geometry offers a scalable solution for quantum photonic networks.
Quantum photonic technologies rely on the ability to generate, manipulate, and interfere indistinguishable single photons on a scalable platform. Among the various approaches, spontaneous parametric down-conversion (SPDC) remains one of the most widely used methods for generating entangled photon pairs and pure heralded single photons. However, most integrated SPDC sources relying on co-propagating geometries have a limited purity of heralded photons or require lossy filtering. Type-2 SPDC processes can produce pure separable photons but typically suffer from lower efficiency and added complexity due to polarization management. Here we show the first integrated counter-propagating photon-pair source on lithium niobate on insulator, where signal and idler photons are generated in opposite directions. The counter-propagating geometry leads to spectrally uncorrelated photon pairs without spectral filtering. The joint spectral intensity measurements and unheralded g (2) correlations yield purities of (92 ± 3)%. Interference between two independent sources achieves heralded visibilities of (71 ± 3)%, confirming the scalability of the platform. These results establish a new route towards integrated, high-purity, and tunable photon sources. The demonstrated counter-propagating geometry offers a scalable solution for quantum photonic networks.
On-chip generation of high-purity single photons is essential for scalable photonic quantum technologies. Spontaneous parametric down-conversion (SPDC) is widely used to generate photon pairs for heralded single-photon sources, but intrinsic spectral correlations of the pairs often limit the purity and interference visibility of the heralded photons. Existing approaches to suppress these correlations rely on narrowband spectral filtering, which introduces loss, or exploiting different polarizations, which complicates on-chip integration. Here, we demonstrate a new strategy for generating spectrally separable photon pairs in thin-film lithium niobate nanophotonic circuits by harnessing higher-order spatial modes, with all interacting fields residing in the same polarization. Spectral separability is achieved by engineering group-velocity matching using higher-order transverse-electric modes, combined with a Gaussian-apodized poling profile to further suppress residual correlations inherent to standard periodic poling. Subsequent on-chip mode conversion with efficiency exceeding 95\% maps the higher-order mode to the fundamental mode and routes the photons into distinct output channels. The resulting heralded photons exhibit spectral purities exceeding 94\% inferred from joint-spectral intensity and 89\% from unheralded g(2)g^{(2)}g(2) measurement. This approach enables flexible spectral and temporal engineering of on-chip quantum light sources for quantum computing and quantum networking.
Lithium niobate on insulator is a promising platform for integrated quantum photonics. Its strong nonlinear coefficient and electro-optic effect allow the integration of photon pair sources and fast reconfigurable interferometers for many applications like boson sampling, QKD and quantum state generation. The photons are generated via Spontaneous Parametric Down-Conversion (SPDC). Two key aspects of the photon pairs are their bandwidth and the possibility to split them deterministically. Here we present a new source type where the generated photons travel in opposite directions and feature a narrow bandwidth of 5 nm in the forward and 20nm in the backward propagation. The reduction of bandwidth and the separability are big advantages over the type-0-SPDC sources. Compared to the well-known type-2-SPDC sources we achieve a 3.6 times higher efficiency with similar bandwidths.
Existing nonlinear-optic implementations of pure, unfiltered heralded single-photon sources do not offer the scalability required for densely integrated quantum networks. Additionally, lithium niobate has hitherto been unsuitable for such use due to its material dispersion. We engineer the dispersion and the quasi-phasematching conditions of a waveguide in the rapidly emerging thin-film lithium niobate platform to generate spectrally separable photon pairs in the telecommunications band. Such photon pairs can be used as spectrally pure heralded single-photon sources in quantum networks. We estimate a heralded-state spectral purity of >94% based on joint spectral intensity measurements. Further, a joint spectral phase-sensitive measurement of the unheralded time-integrated second-order correlation function yields a heralded-state purity of ( 86 ± 5 ) % .
Joint spectral characterization of SPDC photon pairs near 2 μμμm in (Al)GaAs-on-insulator waveguides
Integrated photon-pair sources are a core component of chip-based quantum computing, communication, and metrology. Although such sources have been demonstrated at conventional telecom wavelengths, the 2 μμμm band remains comparatively less explored, despite offering advantages for free-space quantum communication, low-loss transmission in emerging fiber networks, and integration with silicon photonic platforms. In this paper, we demonstrate spontaneous parametric down-conversion (SPDC) in straight GaAs- and AlGaAs-on-insulator waveguides. This platform offers strong second-order nonlinearity and geometry-tunable dispersion, which are advantageous for efficient on-chip pair generation. Measurements of the joint spectral intensity and heralded second-order correlation function show broadband emission around 2 μμμm with strong spectral anti-correlations. To our knowledge, this is the first direct joint-spectral characterization of an integrated SPDC source in this wavelength regime.
Recent advances of high-quality lithium niobate (LN) on insulator technology have revitalized the progress of novel chip-integrated LN-based photonic devices and accelerated application research. One of the promising technologies of interest is the generation of entangled photon pairs based on spontaneous parametric down-conversion (SPDC) in LNs. In this paper, we investigated, theoretically and numerically, Type II SPDC in two kinds of LNs—undoped and 5-mol% MgO doped LNs. In each case, both non-poled and periodically poled crystals were considered. The technique is based on the SPDC under Type II extended phase matching, where the phase matching and the group velocity matching are simultaneously achieved between interacting photons. The proposed approach has not yet been reported for LNs. We discussed all factors required to generate photon pairs in LNs, in terms of the beam propagation direction, the spectral position of photons, and the corresponding effective nonlinearities and walk-offs. We showed that the spectral positions of the generated photon pairs fall into the mid-infrared region with high potential for free-space quantum communication, spectroscopy, and high-sensitivity metrology. The joint spectral analyses showed that photon pairs can be generated with high purities of 0.995–0.999 with proper pump filtering.