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arXiv:2404.08378 · Physical Review Letters

On-Chip Quantum Interference between Independent Lithium Niobate-on-Insulator Photon-Pair Sources

Robert J. Chapman, Tristan Kuttner, Jost Kellner, Alessandra Sabatti, Andreas Maeder, Giovanni Finco, Fabian Kaufmann, Rachel Grange

Published May 12, 2025• 18 citations
arXivHTMLPDF

Abstract

Generating and interfering nonclassical states of light is fundamental to optical quantum information science and technology. Quantum photonic integrated circuits provide one pathway towards scalability by combining nonlinear sources of nonclassical light and programmable circuits in centimeter-scale devices. The key requirements for quantum applications include efficient generation of indistinguishable photon-pairs and high-visibility programmable quantum interference. Here, we demonstrate a lithium niobate-on-insulator (LNOI) integrated photonic circuit that generates a two-photon path-entangled state, and a programmable interferometer for quantum interference. We generate entangled photons with ∼2.3×10^{8} pairs/s/mW brightness and perform quantum interference experiments on the chip with 96.8±3.6% visibility. LNOI is an emerging photonics technology that has revolutionized high-speed modulators and efficient frequency conversion. Our results provide a path towards large-scale integrated quantum photonics including efficient photon-pair generation and programmable circuits for applications such as boson sampling and quantum communications.

DOI
10.1103/n2y3-2bmz

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Generating and interfering nonclassical states of light is fundamental to optical quantum information science and technology. Quantum photonic integrated circuits provide one pathway towards scalability by combining nonlinear sources of nonclassical light and programmable circuits in centimeter-scale devices. The key requirements for quantum applications include efficient generation of indistinguishable photon-pairs and high-visibility programmable quantum interference. Here, we demonstrate a lithium niobate-on-insulator (LNOI) integrated photonic circuit that generates a two-photon path-entangled state, and a programmable interferometer for quantum interference. We generate entangled photons with ∼2.3×10^{8} pairs/s/mW brightness and perform quantum interference experiments on the chip with 96.8±3.6% visibility. LNOI is an emerging photonics technology that has revolutionized high-speed modulators and efficient frequency conversion. Our results provide a path towards large-scale integrated quantum photonics including efficient photon-pair generation and programmable circuits for applications such as boson sampling and quantum communications.
Abstract Entanglement is central to quantum technologies such as cryptography, sensing, and computing. Photon pairs generated via nonlinear optical processes are excellent for preparing entangled states due to their long coherence times and compatibility with fiber optic networks. Steady progress in nanofabrication has positioned lithium niobate-on-insulator (LNOI) as a leading platform for monolithic integration of photon pair sources into optical circuits, leveraging its strong second-order nonlinearity. Here, we present a reconfigurable photonic integrated circuit on LNOI, which combines two on-chip photon pair sources with programmable interferometers, enabling the generation of entangled states. The photon pair sources achieve a source brightness of 26 MHz nm −1 mW −1 while maintaining a coincidence-to-accidental ratio above 100. We successfully interfere the two sources with 99.0 ± 0.7% visibility, demonstrating the indistinguishability required for producing entanglement on-chip. We show the preparation of any of the maximally entangled Bell states with fidelity above 90% verified by quantum state tomography. These results establish LNOI as a compelling, scalable platform to explore integrated quantum photonic technologies enabled by high-brightness sources of entangled quantum states.
Integrated quantum photonic technologies require scalable devices with high-visibility quantum interference. Recent studies have demonstrated that lithium niobate on insulator enables efficient nonlinear interactions, via quasi-phase matching in periodically poled lithium niobate (PPLN) waveguides. However, the on-chip control of two-photon interference utilizing path entanglement remains limited. In this study, we demonstrate on-chip generation of single-photon sources via quantum interference using path-entangled N00N states in two ways. Using the basic structure of a reverse Hong–Ou–Mandel (RHOM) configuration, we directly observe high on-chip visibility of quantum interference. We achieve a visibility of 97.7% ± 1.1% using a dual-PPLN waveguide as the basic RHOM configuration. To improve the compactness, efficiency, and stability of on-chip operation, we further incorporate a PPLN ring resonator with a Sagnac loop. This allows counter-propagating paths to share a single periodically poled waveguide, achieving a visibility of 84.4% ± 1.6%. These results demonstrate that lithium niobate on insulator (LNOI)-based quantum photonic systems provide a robust foundation for the development of future integrated quantum technologies.
Lithium niobate-on-insulator (LNOI) is a leading platform for high-speed optical communication technologies owing to its large electro-optic bandwidth, which enables light modulation above 100 GHz [1]. The wide transparency window is being leveraged to produce photonic integrated circuits operating at different wavelengths, and the strong second-order nonlinearity allows efficient frequency conversion via periodic poling of the crystal on the same waveguide network [2]. LNOI has potential to revolutionise optical communication, and nonlinear conversion processes can be used to generate highly pure quantum states acting as bits of information for the next generation of optical quantum information technologies.
Quantum photonics has advanced rapidly and become a leading approach for developing a broad range of quantum technologies, including quantum communications, quantum information processing, quantum computing, and quantum sensing. Besides, the emerging photonic integrated circuits (PIC) technology has been widely used to implement versatile optical elements advantageous for different quantum applications. For example, PIC-based devices have functioned as building blocks, such as photonic qubit sources, linear optical circuits, modulators, and even single-photon detectors, for realizing highly integrated, large-scale quantum computing schemes. In such a powerful quantum photonic integrated circuits (QPIC) scheme, the creation, manipulation, and testing of quantum entanglement states from the generated qubits via a reconfigurable photonic circuitry are essential. Though the state-of-the-art PIC technology is established based on Si photonics due to its widely mature nanophotonic circuit (waveguide) fabrication technology supported by the existing immense semiconductor industry, Si-based PIC has limitations in implementing efficient and fast active elements that usually demand a quadratic nonlinearity. Lithium niobate (LN), renowned as “the silicon of photonics”, has long been a popular material widely used in integrated-optical and nonlinear-optical applications. A great variety of passive and active photonic elements have been realized in the LN platform. Recently, a novel material based on high-quality single-crystalline films of LN, known as thin-film LN on insulator (LNOI), has been developed and has soon drawn enormous attention for its greatly promising ability to realize nanoscale PIC/QPIC in this iconic optical material platform. In this presentation, we report our recent studies on several key LN PIC building blocks for developing novel quantum photonic sources and circuits, including highly integrated photonic-circuit periodically poled lithium niobate (PPLN) chips for photon-pair generation and manipulation, for high-dimensional frequency-entangled qudit production, for time-frequency grid-state generation, for continuous-variable squeezed vacuum state generation, and their potential applications to quantum computing/communication/sensing technology. Besides, a PP-LNOI electro-optic (EO) polarization mode converter (PMC) useful for demonstrating fast control of quantum polarization states and other LNOI circuit elements as QPIC building blocks will also be presented.
Abstract Programmable interferometric circuits are at the heart of integrated quantum photonic processors. While the lithium niobate-on-insulator platform has the potential to advance integrated quantum photonics due to its strong nonlinearity and tight mode confinement, the demonstration of reconfigurable two-photon interference has not yet been achieved. Here, we design, fabricate and characterize the building block of such interferometric networks in the form of a 2 × 2 Mach–Zehnder Interferometer. We use a thermo-optic phase shifter to achieve stable performance with a power consumption of P π = 44.4 mW and sub-microsecond switching times. We demonstrate the effectiveness of our device for quantum applications by measuring single-photon routing with up to 34 dB extinction ratio. We show Hong-Ou-Mandel interference with fully tunable visibilities reaching a maximum value of 97.4 ± 1.0 % . As part of large scale quantum photonic circuits, this building block will facilitate reconfigurable and tunable photonic processing units integrated alongside non-classical light sources.
Quantum technologies have surpassed classical systems by leveraging the unique properties of superposition and entanglement in photons and matter. Recent advancements in integrated quantum photonics, especially in silicon-based and lithium niobate platforms, are pushing the technology toward greater scalability and functionality. Silicon circuits have progressed from centimeter-scale, dual-photon systems to millimeter-scale, high-density devices that integrate thousands of components, enabling sophisticated programmable manipulation of multi-photon states. Meanwhile, lithium niobate, thanks to its wide optical transmission window, outstanding nonlinear and electro-optic coefficients, and chemical stability, has emerged as an optimal substrate for fully integrated photonic quantum chips. Devices made from this material exhibit high efficiency in in generating, manipulating, converting, storing, and detecting photon states, thereby establishing a basis for deterministic multi-photon generation and single-photon quantum interactions, as well as comprehensive frequency-state control. This review explores the development of integrated photonic quantum technologies based on both silicon and lithium niobate, highlighting invaluable insights gained from silicon-based systems that can assist the scaling of lithium niobate technologies. It examines the functional integration mechanisms of lithium niobate in electro-optic tuning and nonlinear energy conversion, showcasing its transformative impact throughout the photonic quantum computing process. Looking ahead, we speculate on the developmental pathways for lithium niobate platforms and their potential to revolutionize areas such as quantum communication, complex system simulation, quantum sampling, and optical quantum computing paradigms.