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Large Nonlinear Absorption under Weak Continuous Incoherent Light using Long-lived Room Temperature Excitons

修造 平田, Shuzo Hirata

Published Jun 1, 2015• 0 citations
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Optical bistability and bright and dark resonator solitons exist in semiconductor resonator at room temperature [C.O. Weis and Ye. Larionova, Rep. Prog. Phys. 70 (2007) 255-335], with the usual semiconductor nonlinearity. At low temperature in the strong coupling regime between quantum well excitons and the optical field in a semiconductor microcavity the nonlinearities are strong and based on “polariton nonlinearity”. The strong coupling results in a quasi-particle “exciton-polariton” which gives access to positive and negative reactive and dissipative optical nonlinearities, as opposed to the usual room temperature semiconductor nonlinearities possessing essentially only one sign. The type of nonlinearity and the properties of solitons can be varied widely by the detuning between the photon- and exciton resonances. We show for the first time experimentally the existence of patterns, bright and dark solitons based on polariton nonlinearity. 1. INTRODUCTION Bright and dark spatial solitons were shown to exist in such microresonators with and without population inversion [1-3]. At room temperature the nonlinearity which is at the origin of the soliton existence is the usual mixed absorptive/refractive semiconductor nonlinearity which can have transverse effects (e.g. self-focusing) and longitudinal effects such as nonlinear resonance, both ingredients for soliton stability. At low temperature (or at large exciton binding energies) the exciton, which merges with the absorption band at room temperature, is well separated spectrally from the absorption band so that the nonlinearity becomes that of a 2-level system. If the exciton resonance is strongly coupled with the field inside a resonator the exciton- and the photon resonances mix. At coincidence of the two resonance frequencies, the photon- and the exciton resonances hybridize in an avoided crossing and the two hybrid resonances are ascribed to a quasi-particle, the excitonpolariton. This quasi-particle has unusual optical properties. E.g. is the photon nonlinearity determined by exciton collisions. That the exciton-polariton system has interesting nonlinearities (e.g. induced absorption as opposed to the usual saturable absorption) has been shown previously [4]. It was realized that semiconductor microresonators in the strong field-exciton coupling regime might show optical bistability and first experimental proofs for bistability were given recently [5]. As optical bistability of a resonator is a precondition for the existence of spatial resonator solitons, the question arises whether semiconductor microresonators with polariton nonlinearity can support spatial resonator solitons, which, as a consequence of the large nonlinearity of the polaritons, could be expected to exist at rather small light intensities, as it is of importance for all applications. 2. EXPERIMENTAL ARRANGEMENT AND RESULTS The cooled resonator sample (4 K) is illuminated by light at the polariton resonance wavelengths, and the light reflected from the resonator is observed. The light source is a Ar

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H. Yokoyama

An analysis of static room-temperature-operation characteristics of a reflection-mode semiconductor multiple-quantum well etalon by a simplified two-level system formula of optical nonlinear properties and a computer simulation is presented. In the calculation for a GaAs/AlGaAs multiple-quantum-well etalon using the parameters reported in experimental measurement, it is shown that the very large excitonic optical nonlinearity is not effectively utilized for the optical bistable operation. This occurs because the effective positive-feedback mechanism which increases the etalon internal light intensity is suppressed when a hardly saturable background interband absorption tail is larger than a few thousand cm/sup -1/ at a wavelength where the large excitonic dispersive nonlinearity is observed.>

IEEE Journal of Quantum Electronics•Jun 1, 1989•13 citations
Optical bistability and bright and dark resonator solitons exist in semiconductor resonator at room temperature [C.O. Weis and Ye. Larionova, Rep. Prog. Phys. 70 (2007) 255-335], with the usual semiconductor nonlinearity. At low temperature in the strong coupling regime between quantum well excitons and the optical field in a semiconductor microcavity the nonlinearities are strong and based on “polariton nonlinearity”. The strong coupling results in a quasi-particle “exciton-polariton” which gives access to positive and negative reactive and dissipative optical nonlinearities, as opposed to the usual room temperature semiconductor nonlinearities possessing essentially only one sign. The type of nonlinearity and the properties of solitons can be varied widely by the detuning between the photon- and exciton resonances. We show for the first time experimentally the existence of patterns, bright and dark solitons based on polariton nonlinearity. 1. INTRODUCTION Bright and dark spatial solitons were shown to exist in such microresonators with and without population inversion [1-3]. At room temperature the nonlinearity which is at the origin of the soliton existence is the usual mixed absorptive/refractive semiconductor nonlinearity which can have transverse effects (e.g. self-focusing) and longitudinal effects such as nonlinear resonance, both ingredients for soliton stability. At low temperature (or at large exciton binding energies) the exciton, which merges with the absorption band at room temperature, is well separated spectrally from the absorption band so that the nonlinearity becomes that of a 2-level system. If the exciton resonance is strongly coupled with the field inside a resonator the exciton- and the photon resonances mix. At coincidence of the two resonance frequencies, the photon- and the exciton resonances hybridize in an avoided crossing and the two hybrid resonances are ascribed to a quasi-particle, the excitonpolariton. This quasi-particle has unusual optical properties. E.g. is the photon nonlinearity determined by exciton collisions. That the exciton-polariton system has interesting nonlinearities (e.g. induced absorption as opposed to the usual saturable absorption) has been shown previously [4]. It was realized that semiconductor microresonators in the strong field-exciton coupling regime might show optical bistability and first experimental proofs for bistability were given recently [5]. As optical bistability of a resonator is a precondition for the existence of spatial resonator solitons, the question arises whether semiconductor microresonators with polariton nonlinearity can support spatial resonator solitons, which, as a consequence of the large nonlinearity of the polaritons, could be expected to exist at rather small light intensities, as it is of importance for all applications. 2. EXPERIMENTAL ARRANGEMENT AND RESULTS The cooled resonator sample (4 K) is illuminated by light at the polariton resonance wavelengths, and the light reflected from the resonator is observed. The light source is a Ar
We review the nonlinear-optical effects observed at room temperature in semiconductor quantum-well structures photoexcited near the band gap. A comprehensive discussion of optical transitions in these microstructures is given, including excitonic effects and the specific features of room-temperature exciton resonances. Experimental investigations using continuous-wave, picosecond-, and femtosecond-laser sources are presented. They show extremely efficient nonlinear processes. In the case of excitations that are long compared with the exciton-ionization time, the induced changes in absorption and refraction do not depend on the wavelength or on the duration of excitation. These changes depend only on the density of absorbed photons and are interpreted in terms of electron–hole plasma screening and band filling. In contrast, for ultrashort excitation, nonlinear processes depend critically on the excitation wavelength. The selective generation of excitons is found to produce effects larger than a plasma of the same density. This unexpected result is shown to arise from the low temperature of the exciton gas before it interacts with the lattice and from the decrease of screening that is the reduced dimensionality of quantum-well structures.
An analysis of static room-temperature-operation characteristics of a reflection-mode semiconductor multiple-quantum well etalon by a simplified two-level system formula of optical nonlinear properties and a computer simulation is presented. In the calculation for a GaAs/AlGaAs multiple-quantum-well etalon using the parameters reported in experimental measurement, it is shown that the very large excitonic optical nonlinearity is not effectively utilized for the optical bistable operation. This occurs because the effective positive-feedback mechanism which increases the etalon internal light intensity is suppressed when a hardly saturable background interband absorption tail is larger than a few thousand cm/sup -1/ at a wavelength where the large excitonic dispersive nonlinearity is observed.>