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Effects of Optical Excitation on the Ramsey Magnetometry of Ensemble NV Centers in Diamond

優征 青木, Yusei Aoki, T. Sekiguchi, 尚 谷口, Takashi Taniguchi, T. Taniguchi, 睦子 波多野, C. Shinei, 孝之 岩崎, S. Saiki, S. Ishii, T. Teraji, T. Ohshima, Mutsuko Hatano, Takayuki Iwasaki

Published Nov 1, 2023• 0 citations
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Nitrogen-vacancy (NV) centers in diamond have found broad applications owing to optical spin initialization and readout as well as long spin coherence time at room temperature.1 Recently, we have reported the construction of a pulsed optically detected magnetic resonance (ODMR) system based on double quantum (DQ) Ramsey magnetometry with lock-in (LI) detection towards DC magnetic field sensitivity sufficient for magnetoencephalography.2 The LI detection of fluorescence allowed reduction of the noise floor, removal of the signal offset, and real-time monitoring of the magnetic field. Beyond the CW-ODMR, where spectral broadening and contrast reduction are induced by high-power excitation, the DQ-Ramsey is expected to have highersensitivity, as it allows extension of spin dephasing time T2 * and increase of contrast and fluorescence rates.2 In practice, however, the magnetic sensitivity depends also on how the optical excitation is applied. In this study, we report the excitation power stabilization by reducing the phase noise and the effect of the excitation power on the fluorescence saturation behavior.

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Spin Squeezing Enhanced Quantum Magnetometry with Nitrogen-Vacancy Center Qutrits

Lea Gassab, Özgür Esat Müstecaplıoğlu

Abstract We explore the utility of quantum spin squeezing in quantum magnetometry, focusing on three-level (qutrit) Nitrogen-Vacancy (NV) centers within diamond, utilizing a standard Ramsey interferometry pulse protocol. Our investigation incorporates the effects of dephasing and relaxation on NV centers' dynamics during Ramsey measurements, modeled via the Lindblad quantum master equation. We conduct a comparative analysis between the metrological capabilities of a single NV center and a pair of NV centers, considering Quantum Fisher Information both with and without spin squeezing. The quantum correlations between NV centers are assessed through the evaluation of the Kitagawa-Ueda spin squeezing parameter within a two-level manifold. Additionally, parallel calculations are conducted using a two-level model (qubit) for NV centers. Our findings reveal that leveraging qutrits and spin squeezing yields enhanced magnetometric precision, albeit constrained by dephasing effects. Nevertheless, even in the absence of dynamical decoupling methods to mitigate environmental dissipation, strategic timing of squeezing and free evolution can sustain the advantages of qutrit-based magnetometry.

arXiv:2406.15324•New Journal of Physics•Aug 6, 2025•4 citations
Nitrogen-vacancy (NV) centers in diamond have found broad applications owing to optical spin initialization and readout as well as long spin coherence time at room temperature.1 Recently, we have reported the construction of a pulsed optically detected magnetic resonance (ODMR) system based on double quantum (DQ) Ramsey magnetometry with lock-in (LI) detection towards DC magnetic field sensitivity sufficient for magnetoencephalography.2 The LI detection of fluorescence allowed reduction of the noise floor, removal of the signal offset, and real-time monitoring of the magnetic field. Beyond the CW-ODMR, where spectral broadening and contrast reduction are induced by high-power excitation, the DQ-Ramsey is expected to have highersensitivity, as it allows extension of spin dephasing time T2 * and increase of contrast and fluorescence rates.2 In practice, however, the magnetic sensitivity depends also on how the optical excitation is applied. In this study, we report the excitation power stabilization by reducing the phase noise and the effect of the excitation power on the fluorescence saturation behavior.
Abstract We explore the utility of quantum spin squeezing in quantum magnetometry, focusing on three-level (qutrit) Nitrogen-Vacancy (NV) centers within diamond, utilizing a standard Ramsey interferometry pulse protocol. Our investigation incorporates the effects of dephasing and relaxation on NV centers' dynamics during Ramsey measurements, modeled via the Lindblad quantum master equation. We conduct a comparative analysis between the metrological capabilities of a single NV center and a pair of NV centers, considering Quantum Fisher Information both with and without spin squeezing. The quantum correlations between NV centers are assessed through the evaluation of the Kitagawa-Ueda spin squeezing parameter within a two-level manifold. Additionally, parallel calculations are conducted using a two-level model (qubit) for NV centers. Our findings reveal that leveraging qutrits and spin squeezing yields enhanced magnetometric precision, albeit constrained by dephasing effects. Nevertheless, even in the absence of dynamical decoupling methods to mitigate environmental dissipation, strategic timing of squeezing and free evolution can sustain the advantages of qutrit-based magnetometry.