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Acta Sinica Quantum Optica

The Spin Manipulation of the High Density of NV Centers in Diamond

赵敏 ZHAO Min, 秦丽 QIN Li, Ma Zong-min, 王芳 WANG Fang, 张少文 ZHANG Shao-wen, Lin Chaodong, Jun Liu

Published Jan 1, 2016• 0 citations
Publisher
DOI
10.3788/asqo20162204.0379

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Electron and nuclear spins of diamond nitrogen-vacancy (NV) centers are good candidates for quantum information processing as they have long coherence time and can be initialized and read out optically. However, creating a large number of coherently coupled and individually addressable NV centers for quantum computing has been a big challenge. Here we propose methods to use high-density diamond NV centers coupled by spin-spin interaction with an average separation on the order of 10 nm for quantum computing. We propose to use a strain gradient to encode the position information of each NV center in the energy level of its excited electron orbital state, which causes a shift of its optical transition frequency. With such strain encoding, more than 100 closely-packed NV centers below optical diffraction limit can be read out individually by resonant optical excitation. A magnetic gradient will be used to shift the electron spin resonant (ESR) frequencies of NV centers. Therefore, the spin state of each NV center can be individually manipulated and different NV centers can be selectively coupled. A universal set of quantum operations for two-qubit and three-qubit system is introduced by careful design of external drives. Moreover, entangled states with multiple qubits can be created by this protocol, which is a major step towards quantum information processing with solid-state spins.
The nitrogen-vacancy (NV) center is one of the major platforms in the evolving field of quantum technologies. The inertial surveying technology based on NV centers in diamond is a developing field with both scientific and technological importance. Quantum measurement using the solid-state spin of the NV center has demonstrated potential in both high-precision and small-volume low-cost devices. In terms of rotation measurement, the optically detected magnetic resonance has provided a perspective of the rotation measurement mechanism via the solid-state spin of the NV center. A new type of gyroscope based on the solid-state spin in diamond according to the theory has attracted considerable attention. In addition, combined with the ingenious quantum mechanics manipulation and coupling mechanism, acceleration measurement can be achieved through an efficient quantum detection technology of the NV center. This review summarizes the recent research progress in diamond-based inertial measurement, including sensitivity optimization methods for inertial measurement systems based on the NV center.
Selective alignment of nitrogen-vacancy (NV) centers in diamond is an important technique towards its applications. Quantification of the alignment ratio is necessary to design the optimized diamond samples. However, this is not a straightforward problem for dense ensemble of the NV centers. We estimate the alignment ratio of ensemble NV centers along the [111] direction in (111) diamond by optically detected magnetic resonance measurements. Diamond films deposited by N2 doped chemical vapor deposition have NV center densities over 1 × 1015 cm−3 and alignment ratios over 75%. Although spin coherence time (T2) is limited to a few μs by electron spins of nitrogen impurities, the combination of the selective alignment and the high density can be a possible way to optimize NV-containing diamond samples for the sensing applications.