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Implementation of Double Quantum Magnetometry to Continuously Excited Ramsey Method

裕太 荒木, Yuta Araki, 伊久哉 藤崎, Ikuya Fujisaki, 雄治 波多野, Yuji Hatano, 孝之 岩崎, Takayuki Iwasaki, 睦子 波多野, Takayuki Iwasaki, Mutsuko Hatano

Published Nov 1, 2022• 0 citations
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Quantum magnetic sensors based on nitrogen vacancy (NV) centers are expected to be used for various biological and medical applications. Continuously excited (CE) Ramsey magnetometry is one of the most sensitive measurement protocols and has the potential to improve the sensitivity of sensors using additional quantum manipulations to extend the spin dephasing time. In a typical ensemble NV measurement, the spin dephasing time is limited by inhomogeneous coupling. To overcome this limitation, a magnetometry that extends the CE Ramsey protocol with a double‐quantum (DQ) Ramsey sequence and spin bath driving is developed. It is demonstrated that the electric noise due to the spatial inhomogeneity of the crystal strain is cancelled out by the DQ Ramsey, and the magnetic noise due to the P1 centers was suppressed by spin bath driving. Compared to the conventional CE Ramsey, the CE‐DQ Ramsey with spin bath driving effectively doubles the gyromagnetic ratio and yields a twofold extension of , corresponding to a fourfold enhancement of the photon‐shot‐noise limited sensitivity.
We developed a highly sensitive and long-term stable diamond quantum magnetometer by integrating a dual-feedback system that compensates for common- and differential-mode frequency shifts in double-quantum (DQ) 4-Ramsey interferometry. Detecting extremely weak magnetic-field signals requires extensive signal accumulation to enhance the signal-to-noise ratio. However, deviations from the optimal operating frequencies caused by thermal drift or environmental magnetic noise severely hinder the long-term stability of such a sensing system. To overcome the limitation, we first derived analytical solutions for the signal response to common- and differential-mode detunings based on a detuning-inclusive Hamiltonian to theoretically clarify the robustness limit in DQ 4-Ramsey sensing. Guided by this theoretical model, we introduced synchronized frequency modulation and a dual-feedback scheme to independently track and compensate for these frequency shifts while maintaining an optimal magnetic-field response. The proposed method enabled stable continuous operation against temperature variations of 2.8 K. By maintaining a magnetic field sensitivity of 7.0 pT/Hz^1/2 in the frequency range of 5-100 Hz for a prolonged duration of 4 hours, we achieved an extremely low noise floor of 64 fT/Hz^1/2. During prolonged continuous sensing, the system exhibited the expected 1/T^1/2 scaling with integration time T, and prevented both the underestimation of amplitude and waveform distortion. These results establish a robust approach for long-term DQ 4-Ramsey diamond magnetometry and demonstrate its potential for detecting weak biomagnetic signals.