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Time-resolved FT spectra of neon Rydberg states

Petr Kubelík, Adam Pastorek, Svatopluk Civiš

Published Jan 1, 2014• 0 citations
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The one- and two-colour spectra of Neon Rydberg states have been recorded in the energy region below the first ionization threshold. Access to this region is achieved by recording the yield of Ne2+ ions formed in an associative ionization process between atoms in the Rydberg states formed in the photonic excitation and ground state neutral atoms. The one-colour spectra permit a study of the AI process as a function of the principal quantum number of the photo-excited Rydberg state while the two-colour spectra give access to Rydberg series previously unobserved using photon excitation.
We report extensive new data on the single-colour two-photon optogalvanic spectra of neon in the visible region. The experimental method enables us to record a pure two-photon spectrum in a region which is full of one-photon transitions. A large number of two-photon transitions originating from two metastable 3s(3/2) 2 , 3s'( 1/2 ) 0 states and one non-metastable 3s(3/2) I state of the 2p 5 3s configuration of neon have been recorded and arranged into 19 Rydberg series. The interchannel interactions among the overlapping Rydberg series have been studied using the multichannel quantum defect theory.