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Simultaneous Frequency Conversion and Spectral-Temporal Shaping of Single-Photon Pulses

Michał Mikołajczyk, Ali Golestani, Rex H. S. Bannerman, James C. Gates, Peter G. R. Smith, Michał Karpiński

Published Sep 22, 2025• 0 citations
Publisher

Abstract

We demonstrate a quantum interface that simultaneously converts the wavelength, bandwidth, and duration of single-photon-level pulses, enabling compatibility between disparate quantum systems. Using difference frequency generation in a lithium niobate waveguide driven by a highly chirped pump, we transform pulses from 798 nm, 5 GHz, 150 ps (quantum dot-like) to 1300 nm, 35 GHz, < 25 ps (telecom standard). This nonlinear optical time lens achieves over 80% internal conversion efficiency and compresses output pulses below detector resolution. The device offers a compact solution for integrating quantum emitters, memories, and telecom networks, with potential for further pulse shape control.

DOI
10.1051/epjconf/202533506011/pdf

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We demonstrate a quantum interface that simultaneously converts the wavelength, bandwidth, and duration of single-photon-level pulses, enabling compatibility between disparate quantum systems. Using difference frequency generation in a lithium niobate waveguide driven by a highly chirped pump, we transform pulses from 798 nm, 5 GHz, 150 ps (quantum dot-like) to 1300 nm, 35 GHz, < 25 ps (telecom standard). This nonlinear optical time lens achieves over 80% internal conversion efficiency and compresses output pulses below detector resolution. The device offers a compact solution for integrating quantum emitters, memories, and telecom networks, with potential for further pulse shape control.
We demonstrate a quantum interface that simultaneously converts the wavelength, bandwidth, and duration of single-photon-level pulses, enabling compatibility between disparate quantum systems. Using difference frequency generation in a lithium niobate waveguide driven by a highly chirped pump, we transform pulses from 798 nm, 5 GHz, 150 ps (quantum dot-like) to 1300 nm, 35 GHz, < 25 ps (telecom standard). This nonlinear optical time lens achieves over 80% internal conversion efficiency and compresses output pulses below detector resolution. The device offers a compact solution for integrating quantum emitters, memories, and telecom networks, with potential for further pulse shape control.
We experimentally demonstrate spectral broadening and shaping of exponentially-decaying nanosecond pulses via nonlinear mixing with a phase-modulated pump in a periodically poled lithium niobate (PPLN) waveguide. 1550 nm pump light is imprinted with a temporal phase and used to upconvert a weak 980 nm pulse to 600 nm while simultaneously broadening the spectrum to that of a Lorentzian pulse up to 10 times shorter. While the current experimental demonstration is for spectral shaping, we also provide a numerical study showing the feasibility of subsequent spectral phase correction to achieve temporal compression and reshaping of a 1 ns mono-exponentially decaying pulse to a 250 ps Lorentzian, which would constitute a complete spectrotemporal waveform shaping protocol. This method, which uses quantum frequency conversion in PPLN with >100:1 signal-to-noise ratio, is compatible with single photon states of light.
Hybrid quantum networks rely on efficient interfacing of dissimilar quantum nodes, as elements based on parametric downconversion sources, quantum dots, colour centres or atoms are fundamentally different in their frequencies and bandwidths. Although pulse manipulation has been demonstrated in very different systems, to date no interface exists that provides both an efficient bandwidth compression and a substantial frequency translation at the same time. Here we demonstrate an engineered sum-frequency-conversion process in lithium niobate that achieves both goals. We convert pure photons at telecom wavelengths to the visible range while compressing the bandwidth by a factor of 7.47 under preservation of non-classical photon-number statistics. We achieve internal conversion efficiencies of 61.5%, significantly outperforming spectral filtering for bandwidth compression. Our system thus makes the connection between previously incompatible quantum systems as a step towards usable quantum networks.
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Abstract Quantum networks typically operate in the telecom wavelengths to take advantage of low-loss transmission in optical fibres. However, bright quantum dots (QDs) emitting highly indistinguishable quantum states of light, such as InGaAs QDs, often emit photons in the near infrared thus necessitating frequency conversion (FC) to the telecom band. Furthermore, the signal quality of quantum emissions is crucial for the effective performance of these networks. In this work we report a method for simultaneously implementing spectral purification and frequency shifting of single photons from QD sources to the c-band in a periodically poled lithium niobate waveguide. We consider difference frequency generation in the counter-propagating configuration to implement FC with the output emission bandwidth in units of GHz. Our approach establishes a clear path to integrating high-performance single-emitter sources in a hybrid quantum network.
Quantum frequency converters are key enabling technologies in photonic quantum information science to bridge the gap between quantum emitters and telecom photons. Here, we report a coherent frequency converter scheme combining a fiber-coupled nonlinear optical lithium niobate waveguide with a fiber-pigtailed single-photon source based on semiconductor quantum dots. Single and indistinguishable photons are converted from 925.7 nm to the telecommunication C-band, with a 48.4% end-to-end efficiency and full preservation of single-photon purity and indistinguishability. The integration of the two fiber-based modules achieving top-level performance represents an important step toward the practical interconnection of future quantum information processing systems operating at different wavelengths.