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arXiv:2412.15193 · Physical Review Applied

Quantum frequency conversion of photons with microsecond duration from the visible to the telecommunication C band

Sören Wengerowsky, Stefano Duranti, Lukas Heller, Hugues de Riedmatten

Published Feb 20, 2025• 7 citations
arXivHTMLPDF

Abstract

Quantum frequency conversion is a widely used technique to interface atomic systems with the telecom band in order to facilitate propagation over longer distances in fiber. Here, we demonstrate the difference-frequency conversion from 606 nm to 1552 nm of microsecond-long weak coherent pulses at the single-photon level compatible with $\mathrm{Pr}$${}^{3+}$:$\mathrm{Y}$${}_{2}$$\mathrm{Si}\mathrm{O}$${}_{5}$ quantum memories, with a high signal-to-noise ratio (SNR). We use a single-step difference-frequency-generation process with a continuous-wave pump at 994 nm in a periodically poled lithium niobate ($\mathrm{Mg}\mathrm{O}$:ppLN) waveguide and ultranarrow spectral filtering down to a bandwidth of 12.5 MHz. With this setup, we achieve the conversion of weak coherent pulses of duration up to 13.6 \textmu{}s with a device efficiency of about 25 % and an SNR >460 for 10-$\text{\ensuremath{\mu}}\mathrm{s}$-long pulses containing one photon on average. This SNR is large enough to enable a high-fidelity conversion of qubits emitted from an emissive quantum memory based on $\mathrm{Pr}$${}^{3+}$:$\mathrm{Y}$${}_{2}$$\mathrm{Si}\mathrm{O}$${}_{5}$ and to realize an interface with quantum processing nodes based on narrow-linewidth cavity-enhanced trapped ions.

DOI
10.1103/physrevapplied.23.024049

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Quantum frequency conversion is a widely used technique to interface atomic systems with the telecom band in order to facilitate propagation over longer distances in fiber. Here, we demonstrate the difference-frequency conversion from 606 nm to 1552 nm of microsecond-long weak coherent pulses at the single-photon level compatible with \mathrm{Pr}$${}^{3+}:\mathrm{Y}$${}_{2}$$\mathrm{Si}\mathrm{O}$${}_{5} quantum memories, with a high signal-to-noise ratio (SNR). We use a single-step difference-frequency-generation process with a continuous-wave pump at 994 nm in a periodically poled lithium niobate (MgO\mathrm{Mg}\mathrm{O}MgO:ppLN) waveguide and ultranarrow spectral filtering down to a bandwidth of 12.5 MHz. With this setup, we achieve the conversion of weak coherent pulses of duration up to 13.6 \textmu{}s with a device efficiency of about 25 % and an SNR >460 for 10-\ensuremath\mus\text{\ensuremath{\mu}}\mathrm{s}\ensuremath\mus-long pulses containing one photon on average. This SNR is large enough to enable a high-fidelity conversion of qubits emitted from an emissive quantum memory based on \mathrm{Pr}$${}^{3+}:\mathrm{Y}$${}_{2}$$\mathrm{Si}\mathrm{O}$${}_{5} and to realize an interface with quantum processing nodes based on narrow-linewidth cavity-enhanced trapped ions.
We report on quantum frequency conversion of memory-compatible narrow-bandwidth photons at 606 nm to the telecom C-band at 1552 \,nm. The 200 \,ns long photons, compatible with Praseodymium-based solid-state quantum memories are frequency converted using a single-step difference frequency generation process in a periodically poled Lithium Niobate waveguide. We characterize the noise processes involved in the conversion and by applying strong spectral filtering of the noise, we demonstrate high signal-to-noise ratio conversion at the single photon level (SNR$\,>\,100forameaninputphotonnumberperpulseof1).Wefinallyobservethatamemorycompatibleheraldedsinglephotonwithabandwidthof1.8100 for a mean input photon number per pulse of 1). We finally observe that a memory compatible heralded single photon with a bandwidth of 1.8100forameaninputphotonnumberperpulseof1).Wefinallyobservethatamemorycompatibleheraldedsinglephotonwithabandwidthof1.8\,$MHz, obtained from a spontaneous parametric down conversion pair source, still shows a strong non-classical behavior after conversion. We first demonstrate that correlations between heralding and converted heralded photons stay in the non-classical regime. Moreover, we measured the heralded autocorrelation function of the heralded photon using the converter device as a frequency-domain beam splitter, yielding a value of 0.19±0.070.19\pm0.070.19±0.07. The presented work represents a step towards the connection of several quantum memory systems emitting narrow-band visible photons to the telecommunication wavelengths.
We report an experiment demonstrating quantum frequency conversion of weak light pulses compatible with atomic quantum memories to telecommunication wavelengths. We use a PPLN nonlinear waveguide to convert weak coherent states at the single photon level with a duration of 30 ns from a wavelength of 780 nm to 1552 nm. We measure a maximal waveguide internal (external) conversion efficiency η(int) = 0.41 (η(ext) = 0.25), and we show that the signal to noise ratio (SNR) is good enough to reduce the input photon number below 1. In addition, we show that the noise generated by the pump beam in the crystal is proportional to the spectral bandwidth of the device, suggesting that narrower filtering could significantly increase the SNR. Finally, we demonstrate that the quantum frequency converter can operate in the quantum regime by converting a time-bin qubit and measuring the qubit fidelity after conversion.
Signal photons emitted by quantum nodes typically fall outside the low-loss telecom window of optical fibers, leading to severe transmission losses. Quantum frequency conversion (QFC) offers an effective optical interface that bridges quantum nodes with telecom-band channels, enabling long-distance quantum communication. In this work, we demonstrate a compact, fiber-integrated QFC system with low noise and a high signal-to-noise ratio (SNR). Using a periodically poled lithium niobate (PPLN) waveguide, input photons at 637.2 nm are down-converted to telecom photons at 1588.3 nm. Our system achieves a total conversion efficiency of approximately 9%, with pump-induced noise suppressed to 154 Hz. For input photon rates of 32.7, 118.0, and 327.7 kHz, the corresponding SNRs are 12.3, 43.9, and 117.8, respectively. We further develop a theoretical model to simulate the entanglement fidelity between nitrogen-vacancy (NV) center spins and the frequency-converted telecom photons. At the emission rate of an NV center, our QFC system maintains an expected fidelity exceeding 52% over a transmission distance of 100 km. These findings highlight the potential of our QFC system for scalable, long-distance quantum networking.
In this work we experimentally and theoretically characterize the converted signal and the noise level of a quantum frequency conversion (QFC) device implemented for frequency down conversion from the visible to telecommunication wavelengths. This frequency converter is a useful device able to interface quantum memories operating at different wavelengths. We observe that the main noise source is directly induced by the pump via spontaneous parametric down-conversion (SPDC), enhanced by imperfections in the periodic poling structure of the waveguide. We also measure conversion with high signal to noise ratio for microsecond long weak coherent states at the single photon level. Finally, we show theoretically that the converted Stokes/Anti-Stokes non-classical correlations of photon pairs emitted by quantum memories could be largely preserved for pulse durations lower than 4µs.
For quantum information processing (QIP), it is important to have a long-lived quantum memory (QM), coupled to other QMs and quantum processors (QP). However, QM and QP systems demonstrated so far suffer from many limitations, and in the near future a single platform will not have the optimal version of all the components needed for QIP. Thus, it is also important to be able to couple quantum bits in different systems, for example, Rb atoms and NV diamond, preferably using telecom fibres. In this paper, we describe a quantum frequency converter (QFC) that will perform this telecom band qubit conversion. The QFC is based on periodically poled lithium niobate waveguides. For concreteness, we consider specific examples: the conversion of a 780 nm or 795 nm Rb qubit to the telecom band and the conversion of a 637 nm photonic NV diamond qubit to the telecom band, as well as the inverse processes. We show that interface fidelity exceeding 95% should be feasible. Given the storage times ∼1 s already demonstrated in the solid-state systems, and the recent demonstrations of spin-photon entanglement with the NV and entanglement of the NV spin with a superconducting flux qubit operating in the microwave region near 2.88 GHz, such a link would provide the key interface needed to build a quantum internet.
Trapped ions are one of the leading candidates for scalable and long-distance quantum networks because of their long qubit coherence time, high-fidelity single- and two-qubit gates, and their ability to generate photons entangled with the qubit state of the ion. One method for creating ion-photon entanglement is to exploit optical transitions from the 6 P 1/2 to 6 S 1/2 levels, which naturally emit spin-photon entangled states. But these optical transitions typically lie in the ultraviolet and visible wavelength regions of the spectrum. These wavelengths exhibit significant fiber-optic propagation loss, thereby limiting the transfer of quantum information to tens of meters. Quantum frequency conversion is essential to convert these photons to telecom wavelengths so that they can propagate over long distances in fiber-based networks, as well as for compatibility with the vast number of telecom-based optoelectronic components. Here, we generate O-band telecom photons via a low-noise quantum frequency conversion scheme from photons emitted from the 6 P 1/2 to 6 S 1/2 dipole transition of a trapped barium ion. We use a two-stage quantum frequency conversion scheme to achieve a frequency shift of 375.4 THz between the input visible photon and the output telecom photon, achieving a conversion efficiency of 11%. We attain a signal-to-background ratio of over 100 for the converted O-band telecom photon with background noise of less than 15 counts/s. These results are an important step toward achieving trapped ion quantum networks over long distances for distributed quantum computing and quantum communication.