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Field theories of strongly correlated, two-dimensional metals : phases and criticality

Thomas P. Sheerin

Published Jan 22, 2026• 0 citations
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Abstract

This thesis details quantum-field-theoretical analyses of four distinct strongly correlated metallic systems in two spatial dimensions. It begins by examining two driving mechanisms proposed in the literature for the exotic charge-density-wave phase in monolayer vanadium diselenide. The spectral-function-fitting method used to analyse the first proves quite indeterminate, leading to only speculative conclusions. The second mechanism is tested by producing mean-field phase diagrams of the system, yielding an appreciable region of phase space in which it does drive the charge-density wave. In the next chapter, the square-lattice Hubbard model with first-, second- and third-nearest-neighbour hoppings is considered. Phase diagrams are predicted using the few-patch parquet renormalization group and compared with those produced by a colleague using another method, and with those from another patch scheme in the literature. It is concluded that few-patch parquet-renormalization-group schemes are not sophisticated enough to correctly describe many features of this system, and likely other systems. The second half of the thesis studies non-Fermi liquids. First, the non-Fermi liquid resulting from coupling finite-density fermions to a U(1) gauge field is examined. The functional renormalization group, with a soft frequency regulator for the fermions, is used, and gauge-symmetry constraints are imposed. The resulting bosonic dynamical exponent is z_A = 2, and the fermionic self-energy scales as Σ(ω,k_F) ~ √ω at small frequency. Enforcement of the symmetry constraints leaves the results largely unchanged, but does make the bosonic mass term irrelevant about criticality. In the final research chapter, the non-equilibrium modes of two-dimensional non-Fermi liquids in incipient itinerant ferromagnets are analysed. Linearized quantum Boltzmann equations are solved to find the spectra of charge- and spin-density modes. Whether collective modes are present is found to depend on both universal and non-universal information, in ways previously overlooked. Preliminary results are also given for the spectra when coupling to a classical magnetic field is reincluded.

DOI
10.17630/sta/1505

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This thesis details quantum-field-theoretical analyses of four distinct strongly correlated metallic systems in two spatial dimensions. It begins by examining two driving mechanisms proposed in the literature for the exotic charge-density-wave phase in monolayer vanadium diselenide. The spectral-function-fitting method used to analyse the first proves quite indeterminate, leading to only speculative conclusions. The second mechanism is tested by producing mean-field phase diagrams of the system, yielding an appreciable region of phase space in which it does drive the charge-density wave. In the next chapter, the square-lattice Hubbard model with first-, second- and third-nearest-neighbour hoppings is considered. Phase diagrams are predicted using the few-patch parquet renormalization group and compared with those produced by a colleague using another method, and with those from another patch scheme in the literature. It is concluded that few-patch parquet-renormalization-group schemes are not sophisticated enough to correctly describe many features of this system, and likely other systems. The second half of the thesis studies non-Fermi liquids. First, the non-Fermi liquid resulting from coupling finite-density fermions to a U(1) gauge field is examined. The functional renormalization group, with a soft frequency regulator for the fermions, is used, and gauge-symmetry constraints are imposed. The resulting bosonic dynamical exponent is z_A = 2, and the fermionic self-energy scales as Σ(ω,k_F) ~ √ω at small frequency. Enforcement of the symmetry constraints leaves the results largely unchanged, but does make the bosonic mass term irrelevant about criticality. In the final research chapter, the non-equilibrium modes of two-dimensional non-Fermi liquids in incipient itinerant ferromagnets are analysed. Linearized quantum Boltzmann equations are solved to find the spectra of charge- and spin-density modes. Whether collective modes are present is found to depend on both universal and non-universal information, in ways previously overlooked. Preliminary results are also given for the spectra when coupling to a classical magnetic field is reincluded.
The aim of this thesis it to contribute to three open problems in the theory of itinerant electron systems in two spatial dimensions. Firstly, the mechanism for charge density wave formation in the transition metal dichalcogenides is a debated subject. In this thesis it is shown that charge density wave formation is possible via a purely electronic mechanism in monolayer vanadium diselenide. The competition of superconductivity and density wave formation is taken into account using the renormalisation group. As the Fermi surface is tuned to perfect nesting, a charge density wave phase emerges when the Heisenberg exchange interaction is of the order of the contact Coulomb repulsion. Secondly, the search for materials which exhibit topological superconductivity is ongoing. Possible candidates are strongly spin-orbit-coupled metals. In this thesis a square-lattice Hubbard model with strong Rashba spin-orbit coupling and one of the Fermi surfaces close to a Lifshitz transition is examined. The metal is shown to be generically unstable to the formation of mixed-parity superconductivity with a helical triplet component via a renormalisation group analysis. Thirdly, the breakdown of Fermi liquid theory close to a quantum critical point is still not well understood. In this thesis a functional renormalisation group analysis is presented using a soft frequency cutoff, investigating a general class of Pomeranchuk instabilities with 𝑁_𝑏 flavours of boson. At small 𝑁_𝑏 the theory is characterised by weakly non-Fermi-liquid behaviour of the electrons and 𝑧≈2 dynamics for the order parameter fluctuations. For large 𝑁_𝑏, the theory crosses over to 𝑧≈1 scaling and non-Fermi-liquid behaviour.
"Strong electron correlation phenomena are ubiquitous, such as unconventional superconductivity and the metal-insulator transitions. Having a proper understanding of strongly correlated electron systems requires a non-perturbative analysis because Fermi liquid theory inevitably breaks down due to the strong correlation. In this thesis, we will study two non-perturbative approaches to tackle strongly correlated electronic system: 1.) multi-dimensional bosonization and 2.) the AdS/CFT correspondence. Multidimensional bosonization is the generalization of bosonization to spatial dimensions larger than one. The bosonized theory is an effective field theory in terms of the bosonic particle-hole fluctuations in different patches of the Fermi surface. The bosonized theory is quadratic and hence can be solved non-perturbatively. The AdS/CFT correspondence is a conjecture that d-dimensional field theory is dual to a d+1 dimensional quantum gravitational theory. Problems in strongly coupled field theory then have an equivalent description using weakly interacting gravitational theory, allowing a non-perturbative analysis. Chapter 1 will serve as an introduction. We will review several experiments which show a breakdown of Fermi liquid theory. Formalisms for multidimensional bosonization and the AdS/CFT correspondence will then be reviewed. In chapter 2, the two-orbital Hubbard model with degenerate d{xz} and d{yz} orbitals are investigated. We apply multidimensional bosonization to solve this problem exactly and discover a z=3 overdamped collective modes that emerges at the orbital-ordering quantum critical point. These modes modify the single-particle density of states and lead to non-Fermi liquid behavior which can provide a possible explanation for the recently observed zero-bias enhancement in the point contact spectroscopy signal on iron pnictides. Chapters 3, 4 and 5 discuss the applications of the AdS/CFT correspondence to model various condensed matter systems. In chapter 3, We consider an interaction term between a bulk spinor field and a gauge field in the Reissner-Nordstr\""om AdS background. When the Pauli interaction term is large enough, a dynamical gap is generated and spectral weight transfer is observed in the spectral density, mimicking the behavior of the Hubbard model. We further consider the finite temperature case and discover that the ratio between the dynamical gap and the critical temperature has the same order as that of VO^2. The Pauli coupling is also studied in the superconducting background. Chapter 4 consider the propagation of a neutral scalar field in the geometry called the electron star. The electron star has Lifshitz scaling with finite dynamical critical exponent at the interior, which is suitable for the modeling of quantum criticality and quantum phase transition with a neutral order parameter, for example for antiferromagnetism. We find that the quantum phase transition has the Berezinski-Kosterlitz-Thouless characteristic and the dynamical critical exponent can change across the quantum critical point. In chapter 5, we construct a gravity dual of the nematic phase by studying the condensation of a spin-two field in the Schwarzschild-AdS background. The condensation of a spin-two field can distort the rotational symmetry of the Fermi surface as long as the spin-two field is coupled to a probe spinor field in the bulk gravity dual."
In this thesis we study the scaling properties of unconventional metals that arise at quantum critical points using low-energy effective field theories. Due to high rate of scatterings between electrons and critical fluctuations of the order parameter associated with spontaneous symmetry breaking, Landau’s Fermi liquid theory breaks down at the critical points. The theories that describe these critical points generally flow into strong coupling regimes at low energy in two space dimensions. Here we develop and utilize renormalization group methods that are suitable for the interacting non-Fermi liquids. We focus on the critical points arising at excitonic, and commensurate spin and charge density wave transitions. By controlled analyses we find stable non-Fermi liquid and marginal Fermi liquid states, and extract the scaling behaviour. The field theories for the non-Fermi liquids are characterized by symmetry groups, local curvature of the Fermi surface, the dispersion of the order parameter fluctuations, and dimensions of space and Fermi surface.
The primary subject of this thesis is the two-dimensional Hubbard model. Using the functional renormalization Group in static approximation we will present the phase diagram of the 2D-Hubbard model and refine it by including frequency dependencies and full self-energy effects. The focus will fall on the vicinity of the quantum critical point, where the system shows a non-Fermi-liquid-like behavior. In mean-field calculations, we show that the frequency dependence of the self-energy has a substantial impact on the ground state. Furthermore, we investigate the relation between the density-density interaction and the quasiparticle lifetime. During the course of our study, we will develop a saddle-point formulation of Schwinger-Dyson equations and present a new renormalization group scheme which is valid for all fermionic systems.
We present a field-theoretic renormalization group analysis of Abanov and Chubukov's model of the spin density wave transition in two dimensional metals. We identify the independent field scale and coupling constant renormalizations in a local field theory and argue that the damping constant of spin density wave fluctuations tracks the renormalization of the local couplings. The divergences at two-loop order overdetermine the renormalization constants and are shown to be consistent with our renormalization scheme. We describe the physical consequences of our renormalization-group equations, including the breakdown of Fermi liquid behavior near the ``hot spots'' on the Fermi surface. In particular, we find that the dynamical critical exponent zzz receives corrections to its mean-field value z=2z=2z=2. At higher orders in the loop expansion, we find infrared singularities similar to those found by Lee [Phys. Rev. B 80, 165102 (2009)] for the problem of a Fermi surface coupled to a gauge field. A treatment of these singularities implies that an expansion in 1∕N1∕N1∕N (where NNN is the number of fermion flavors) fails for the present problem. We also discuss the renormalization of the pairing vertex and find an enhancement which scales as logarithm squared of the energy scale. A similar enhancement is also found for a modulated bond order which is locally an Ising-nematic order.
The physics of strongly interacting particles is often extraordinarily rich, leading to the \textit{emergence} of fundamentally new phases and phenomena that cannot exist in the absence of correlations. This thesis is devoted to the study of different classes of quantum systems with such strong correlations. Programmable quantum simulators based on Rydberg atom arrays have recently emerged as versatile platforms to probe quantum many-body phases and their dynamics. In Chapter 2, we start with theories of quantum phase transitions (QPTs) in one-dimensional chains of Rydberg atoms. We demonstrate the existence of a novel QPT in the universality class of the Z3\mathbb{Z}^{}_3Z3​ chiral clock model, calculate its critical exponents, and discuss their measurement with the quantum Kibble-Zurek mechanism. Proceeding to two dimensions, Chapter 3 describes the zero-temperature phase diagram of a square-lattice Rydberg atom array, revealing several experimentally realizable density-wave-ordered phases and QPTs. For a different geometry, namely, the kagome lattice studied in Chapter 4, we identify a regime that constitutes a likely candidate for hosting a phase with long-range quantum entanglement and topological order. Based on mappings to dimer models and gauge theories, we argue for the existence of a quantum spin liquid phase that has proved elusive in solid-state materials. In the next part of this thesis, we focus on similarly strongly correlated phases in the realm of quantum materials. Motivated by recent observations of an enhanced thermal Hall response in the high-temperature cuprate superconductors, in Chapter 5, we study the thermal Hall conductivity, κxy\kappa^{}_{xy}κxy​, of chiral spin-liquid ans\"{a}tze on the square lattice, focusing on the contribution from neutral (bosonic or fermionic) spinons. Thereafter, going beyond mean-field theory, we consider the corrections due to emergent gauge fields, which yield a response of opposite sign to that of the fermionic matter. We additionally consider the contribution of phonons to κxy\kappa^{}_{xy}κxy​ and establish its relation to the spinon Hall viscosity. Thermal Hall measurements also leave intriguing fingerprints in Kitaev materials like α\alphaα-RuCl3_33​, and in this context, Chapter 6 investigates the unquantized κxy\kappa_{xy}κxy​ obtained in a gapless spinon Fermi surface state.