This thesis addresses four key contributions. First, we investigated how tem-poral correlations and dephasing in a quantum dot photon-pair source affecttwo-photon interference, analyzing these effects through multiple approaches,including the sensor method, temporal post-selection, and temperature varia-tion under constant temporal correlations. Second, we implemented a methodbased on low-quality factor micropillar cavities to enhance collection effi-ciency for photon pairs. This approach is based on relatively simple fabrica-tion method and achieves high collection efficiency without solely relying onstrong Purcell enhancement, in contrast to conventional concept. Third, wepresented non-Gaussianity criteria that explicitly account for optical losses,enabling reliable characterization of photon states, and we experimentally ver-ified the presence of non-Gaussianity using a quantum dot photon-pair source.Finally, we introduced a deep-learning-based super-resolution imaging tech-nique that accurately reconstructs images of quantum dots with high resolu-tion without prior system knowledge, even in high-density and noisy environ-ments.Together, these results offer practical solutions for advancing quantum dotphoton sources suitable for emerging quantum technologies.
This thesis addresses four key contributions. First, we investigated how tem-poral correlations and dephasing in a quantum dot photon-pair source affecttwo-photon interference, analyzing these effects through multiple approaches,including the sensor method, temporal post-selection, and temperature varia-tion under constant temporal correlations. Second, we implemented a methodbased on low-quality factor micropillar cavities to enhance collection effi-ciency for photon pairs. This approach is based on relatively simple fabrica-tion method and achieves high collection efficiency without solely relying onstrong Purcell enhancement, in contrast to conventional concept. Third, wepresented non-Gaussianity criteria that explicitly account for optical losses,enabling reliable characterization of photon states, and we experimentally ver-ified the presence of non-Gaussianity using a quantum dot photon-pair source.Finally, we introduced a deep-learning-based super-resolution imaging tech-nique that accurately reconstructs images of quantum dots with high resolu-tion without prior system knowledge, even in high-density and noisy environ-ments.Together, these results offer practical solutions for advancing quantum dotphoton sources suitable for emerging quantum technologies.
The quick development of quantum technologies and quantum communication demands a continuous search for more efficient and with higher performance quantum sources and devices. In particular, quantum dots are firmly established sources of single photon emitters and entangled photon pairs, with entanglement of photons emitted by a single quantum dot probed in polarization[1], time-bin[2] and hyperentanglement[3]. Although spontaneous parametric down conversion sources (SPDC) are widely used as entangled photon sources with the highest values of entanglement[4], are being reached by quantum dot devices[5]. With similar quality as SPDC sources, QDs however stand out as sources with sub-Poissonian statistics, essential for safe quantum communication. Still, most of the quantum dots devices exhibit low extraction efficiencies. Attempts to maximize the extraction efficiency involve sophisticated engineered photonic systems[6,7]. Furthermore, the accurate alignment of the quantum dot-cavity system is crucial for an effective quantum dotcavity coupling and hence an emission enhancement into free space[8]. All of this implies the need of intricated nanofabrication processes. Here we present a simple, scalable photonic device that grants efficient creation of entangled photon pairs from InAs quantum dots. The device, spontaneously formed during the growth process, is based on pairs of bottom/top distributed bragg reflectors (DBRs). A propagating deformation in the DBRs, leads to the formation of self-aligned dimples on top of the QDs, resulting in a self-aligned quantum-dot cavity system[9]. Therefore, costly and complex deterministic nanofabrication techniques are not required. In this work, the device performance was characterized, showing experimental collection efficiencies of 0.17, with theoretically pair extraction efficiencies above 0.45. Furthermore, a Purcell enhancement up to 1.7 was obtained. Finally, the device potential to generate time-bin entangled photons was investigated performing state tomography measurements. The subsequent reconstruction of the density matrix yields a concurrence of 0.70(10) and a fidelity of 0.84(5).
Far-field optical microscopy beyond the Abbe diffraction limit, making use of nonlinear excitation (e.g. STED), or temporal fluctuations in fluorescence (PALM, STORM, SOFI) is already a reality. In contrast, overcoming the diffraction limit using non-classical properties of light is very difficult to achieve due to the fragility of quantum states of light. Here, we experimentally demonstrate superresolution microscopy based on quantum properties of light naturally emitted by fluorophores used as markers in fluorescence microscopy. Our approach is based on photon antibunching, the tendency of fluorophores to emit photons one by one rather than in bursts. Although a distinctively quantum phenomenon, antibunching is readily observed in most common fluorophores even at room temperature. This nonclassical resource can be utilized directly to enhance the imaging resolution, since the non-classical far-field intensity correlations induced by antibunching carry high spatial frequency information on the spatial distribution of emitters. Detecting photon statistics simultaneously in the entire field of view, we were able to detect non-classical correlations of the second and third order, and reconstructed images with resolution significantly beyond the diffraction limit. Alternatively, we demonstrate the utilization of antibunching for augmenting the capabilities of localization-based superresolution imaging in the presence of multiple emitters, using a novel detector comprised of an array of single photon detectors connected to a densely packed fiber bundle. These features allow us to enhance the spatial and temporal resolution with which multiple emitters can be imaged compared with other techniques that rely on CCD cameras.
In the pursuit of developing a quantum information network, photons appear to be the most convenient carriers to interconnect distant ports. The need to get on-demand single photons that is one and only one photon, with a high reliability, is the main driving force for the development of bright solid-state sources. One important parameter is the brightness defined as the probability that one collected pulse contains a single photon. For some applications like quantum information processing or long distance quantum communications, the emitted single photons must be also indistinguishable, so that can make use of their quantum interference to implement effective photon-photon interactions. To reach the ideal source of single and indistinguishable photons, different systems are explored : defects in diamond (NV centers), trapped atoms or ions, single molecules or semiconductor quantum dots.By coupling a semiconductor quantum dot to an optical cavity, the spontaneous emission of the emitter can be modified to obtain bright single-photon sources. An innovative technique was developed by Pr. Pascale Senellart and her team at the Laboratory of Photonics and Nanostructures (LPN) from CNRS that allows making such sources in a very reproducible way.This work explores the performance of single quantum dot coupled to micropillars. Various techniques are used in order to increase the single photon purity and indistinguishability while keeping a high source brightness. First, the cavity was modified using an adiabatic architecture such that a strong acceleration of the spontaneous emission was implemented. Then, a technique to apply an electric bias on the micropillars has been developed. The combination of the electric bias with a resonant optical excitation of the quantum dot allows to generation purely indistinguishable photons with a high brightness.The results developed in this thesis open a vast field of novel applications in quantum technologies, from quantum cryptography, metrology to quantum imaging.
Quantum technology promises to revolutionize various aspects of information processing, communication, and data security, by surpassing the capabilities of classical systems. Central to these advancements are photons, due to their resilience to external influence and ease of transport in air and glass fibers. However, attenuation in glass fiber cores hinders the realization of a worldwide quantum network. To circumvent this limit, the use of quantum repeaters for long-distance communication is required. Pivotal to the realization of quantum repeaters are entangled photons, enabling the distribution of entanglement across intermediate nodes, eventually extending the range of the envisioned quantum network. Despite the availability of numerous photon sources, stringent requirements–such as deterministic photon generation with high purity, high indistinguishability, high efficiency and a high degree of entanglement–hinder the realization of quantum repeaters, as they need to be fulfilled within the same device. Epitaxial quantum dots have emerged as promising candidates for generating pairs of entangled photons with a high purity and a high degree of entanglement. These semiconductor nanostructures, often referred to as “artificial atoms,” confine charge carriers and discretize energy levels like atoms but in a manipulable solid state environment. They exhibit exceptional emission characteristics owing to their high quantum efficiency and tunability via external fields such as electric, magnetic, and strain fields. Nevertheless, the fact that they are embedded in a semiconductor matrix with high refractive index limits their brightness due to challenging light extraction. This PhD thesis investigates the potential of strain-tuned GaAs droplet-etched quantum dots–a system known to generate highly entangled photon pairs–embedded within a photonic cavity, aiming to enhance light extraction efficiency, for an ideal entangled photon source. Device fabrication involves bonding the semiconductor with a micromachined piezoelectric substrate for strain-tuning quantum dots and their deterministic integration with a circular Bragg grating resonator, known as a “bullseye cavity.” Key advancements include cryogenic photoluminescence imaging for precise quantum dot localization, achieving high spatial overlap of the confined excitons with the resonator’s mode volume. Furthermore, postfabrication tuning of the resonator mode via wet chemical etching is employed to optimize spectral overlap. The achievements enable significant Purcell enhancement and high extraction efficiency. Simultaneously, multi-axial strain tuning the quantum dot emission eliminates entanglement degradation caused by the anisotropic exchange interaction of charge carriers. Such an entangled photon source additionally allows to experimentally reveal the limits of entanglement set by the excitation type. Finally, with optimized excitation conditions, a near-ideal entangled photon pair source is realized, which may surpass any other quantum emitter in terms of simultaneous brightness and degree of entanglement. The advancements presented within this PhD thesis represent a significant step towards the integration of quantum dot-based entangled photon sources into real-world quantum technology applications, facilitating the realization of a quantum internet.
The process of image recording is arguably one of the most prevalent technology in modern society and continues to inspire vast swathes of research due to its widespread applications spanning military, medical and consumer spheres. The danger present in a field so broad is that separate niches of research can become isolated with critical advancements struggling to traverse the gulfs between. Unifying the field is the omnipresent drive to acquire an ever increasing quality of images at the lowest possible cost, a goal which warrants continual fundamental research. Quantum entanglement exhibits many intriguing characteristics which make it a suitable tool for such fundamental investigations. The process of spontaneous parametric down- conversion has offered a yet unbeaten strength of photon correlations with the quantum nature of their production providing a reliable and controllable source of single-photons. Arising from these attributes is the technique known as ghost imaging. Though now known to be classically possible, the strength of entanglement generated correlations is yet to be surpassed. This thesis implemented this technique in tandem with the cutting edge detector technology in order to probe the fundamentals of image formation. This form of imaging allowed us to subject an object to a known number of photons whilst acquiring structural information from spatially separate, correlated photons which never interact with the object. The strength of the produced correlations allow us to acquire low background, high resolution images with far less light than traditional techniques and affords many novel benefits. The possibility of incorporating this technique with pre-existent regimes allowed me to draw from advancements made across the landscape of imaging research. Although referred to as “quantum ghost imaging” throughout this work, it should be noted that the intrinsic quantum nature of the correlations was not directly relied upon but provided an ideal source of strongly correlated photons. In order to determine the limits of a traditional imaging system this thesis first sought to answer the question: “can an image of an object be reconstructed from fewer photons than ii pixels in the image?” In chapter 3 I approached this from the perspective of compression, which minimises redundant information within a signal. This lead to the development of an imaging regime capable of imaging with far fewer photons than pixels in the image. By employing assumptions about the sparsity of natural images I was able to reconstruct an image of a biological sample containing an average of less than one photon per image pixel. Having reduced the number of photons necessary to form an image I then considered alternative methods for reducing the optical energy impinging on a sample. I sought to answer the question: “can non-degenerate ghost imaging reduce the optical energy impinged upon an object during imaging”. The photons produced in SPDC need not be of similar wavelengths, however may be chosen far from degeneracy, i.e. non-degenerate. In Chapter 4 I presented a ghost imaging system which illuminated the object with infrared light whilst recording the structural information via entangled visible photons. This allowed for objects opaque to visible light to be imaged in high quality without the need for a spatially resolving infrared detector, the state of the art of which lags behind their silicon based visible counterparts. I presented the systems capabilities by imaging objects which were etched into a gold substrate layered on to silicon, both of which are opaque to visible light. Not only did a reduction in energy deposition arise from the lower energy probe wavelength but applying the reconstruction techniques from the previous chapter brought that down to as low as ≈16 nJcm−2s−1. Seeking to expand the repertoire of applications, the low-light capabilities of my ghost imaging were applied to the technique of phase-contrast microscopy in chapter 5. Typically applied to translucent objects, phase-contrast imaging transfers phase information, i.e. the refractive index changed within the object, into an intensity distribution through the use of a phase-filter. In many of these applications the objects tend to be biological in nature, where high optical exposure can result in bleaching or damage. By applying the phase-filter non- locally, i.e. to the photons correlated to those probing the object, I acquired edge-enhanced images of a phase object whilst illuminating with significantly fewer photons than standard phase-contrast techniques. Having displayed the broad applicability of our low-light ghost imaging system, I then sought to determine the optical resolution in chapter 6. The resolution limits of ghost imaging are not clear at first glance owing to the resolutions dependence upon the strength of spatial correlations. As the length over which the spatial correlations are produced can be brought below the standard diffraction limit, it would seem the resolution of the system could be brought similarly low. To clarify this I artificially restricted the number of spatial modes in each of the correlated beams to uncover the physically realisable resolution. I show that although the resolution of a ghost imaging system to be fundamentally determined by the strength of the correlations, this can never be reached due to the inherent limitations of the intervening imaging system.
Entangled photons are at the heart of experimental quantum physics. They were used for the first fundamental tests of quantum theory, and became a basic building block for many novel quantum protocols, such as quantum cryptography, dense coding or teleportation. Therefore, the efficient generation of entangled photons, as well as their distribution and accurate analysis are of paramount importance, particularly with regard to the practicability of many applications of quantum communication. This thesis deals largely with the problem of efficient generation of photonic entanglement with the principal aim of developing a bright source of polarization-entangled photon pairs, which meets the requirements for reliable and economic operation of quantum communication prototypes and demonstrators. Our approach uses a correlated photon-pair emission in nonlinear process of spontaneous parametric down-conversion pumped by light coming from a compact and cheap blue laser diode. Two alternative source configurations are examined within the thesis. The first makes use of a well established concept of degenerate non-collinear emission from a single type-II nonlinear crystal and the second relies on a novel method where the emissions from two adjacent type-I phase-matched nonlinear crystals operated in collinear non-degenerate regime are coherently overlapped. The latter approach showed to be more effective, yielding a total detected rate of almost 10^6 pairs/s at >98 % quantum interference visibility of polarization correlations. This performance, together with the almost free of alignment operation of the system, suggest that it is an especially promising candidate for many future practical applications, including quantum cryptography, detector calibration or use in undergraduate lab courses. The second issue addressed within the thesis is the simplification and practical implementation of quantum-assisted solutions to multiparty communication tasks. While the recent rapid progress in the development of bright entangled photon-pair sources has been followed with ample experimental reports on two-party quantum communication tasks, the practical implementations of tasks for more than two parties have been held back, so far. This is mainly due to the requirement of multiparty entangled states, which are very difficult to be produced with current methods and moreover suffer from a high noise. We show that entanglement is not the only non-classical resource endowing the quantum multiparty information processing its power. Instead, only the sequential communication and transformation of a single qubit can be sufficient to accomplish certain tasks. This we prove for two distinct communication tasks, secret sharing and communication complexity. Whereas the goal of the first is to split a cryptographic key among several parties in a way that its reconstruction requires their collaboration, the latter aims at reducing the amount of communication during distributed computational tasks. Importantly, our qubit-assisted solutions to the problems are feasible with state-of-the-art technology. This we clearly demonstrate in the laboratory implementation for 6 and 5 parties, respectively, which is to the best of our knowledge the highest number of actively performing parties in a quantum protocol ever implemented. Thus, by successfully solving and implementing a cryptographic task as well as a task originating in computer science, we clearly illustrate the potential to introduce multiparty communication problems into real life.