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Bulgarian Journal of Physics

Antibunching, Sub-Poissonian, and Correlation Functions of Photons in Seventh Harmonic Generation Process

Published Dec 21, 2025• 0 citations
Publisher

Abstract

The study investigates antibunching, sub-Poissonian statistics, and photon correlation functions in the pump and harmonic modes of the seventh harmonic generation process.We investigated various approaches to photon antibunching by solving the generalised interaction Hamiltonian in the Heisenberg picture using short-time approximation.It is inferred that the number of pump photons, coupling of the field strength, and interaction times significantly influence photon antibunching.It is observed that third-order antibunching in the pump mode has greater nonclassicality than second-and first-order antibunching.In the harmonic mode, the nonclassical effect is found to be less pronounced and becomes more evident as the interaction time decreases.The first-order Hamiltonian interaction induces a stronger nonclassical effect than the second-order interaction.The interaction of a coherent pump field with a nonzero harmonic field leads to photon clustering and bunching effects.Finally, photon antibunching appears most pronounced, indicating nonclassicality, as the second-order correlation function decreases.This confirms that antibunching is a fundamental quantum property of light.

DOI
10.55318/bgjp.2025.52.4.330

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The study investigates antibunching, sub-Poissonian statistics, and photon correlation functions in the pump and harmonic modes of the seventh harmonic generation process.We investigated various approaches to photon antibunching by solving the generalised interaction Hamiltonian in the Heisenberg picture using short-time approximation.It is inferred that the number of pump photons, coupling of the field strength, and interaction times significantly influence photon antibunching.It is observed that third-order antibunching in the pump mode has greater nonclassicality than second-and first-order antibunching.In the harmonic mode, the nonclassical effect is found to be less pronounced and becomes more evident as the interaction time decreases.The first-order Hamiltonian interaction induces a stronger nonclassical effect than the second-order interaction.The interaction of a coherent pump field with a nonzero harmonic field leads to photon clustering and bunching effects.Finally, photon antibunching appears most pronounced, indicating nonclassicality, as the second-order correlation function decreases.This confirms that antibunching is a fundamental quantum property of light.
We studied photon antibunching in the pump and the harmonic modes of the sixth harmonic generation process. The generalized interaction Hamiltonian is solved for several particular cases in the Heisenberg picture, and the possibility of observing photon antibunching is investigated using the short-time approximation technique. It is shown that the photon antibunching in the pump field depends on the number of pump photons, the interaction time, and the coupling of the field between the modes. With the same amount of pump photons, we deduced that third-order photon antibunching is more nonclassical than second- and first-order photon antibunching. In this process, the effect of photon antibunching is not seen in the harmonic mode over pump mode. It is shown that photon antibunching is more noticeable with shorter interaction times as the depth of nonclassicality increases and the second-order correlation function decreases. The first-order Hamiltonian interaction, which stimulates both pump and harmonic fields, is demonstrated to be more nonclassical than the second-order Hamiltonian interaction. It is clear that the coherent state, or vacuum state, of a pump field with a nonzero harmonic field creates photon clusters because the pump field causes interaction, which leads to bunching effects. It is interpreted that the degree of photon antibunching is maximum in the regions where the second correlation function is minimum. Photon antibunching has been shown to be one of the quantum properties of light.
This paper aims to study the photons antibunching in the fundamental, Stokes and signal modes of CAHRS (coherent anti-Stokes hyper Raman scattering). The generalized interaction Hamiltonian was calculated for different conditions in the Heisenberg picture under short time approximation to observe photons antibunching in the fundamental, Stokes and signal modes of CAHRS. It has been found that antibunching in the fundamental field is dependent upon interaction time, photons number, and coupling strength of field. Third order photon antibunching is found to be nonclassical to a greater extent than second- and first-order photon antibunching for the identical pump photons count. It has been also observed that the effect of photon antibunching in Stokes and signal modes is less prominent than in the fundamental- mode. Furthermore, it is also found that antibunching will increase at short interaction timeswith the increase of depth of nonclassical behavior. Finally, the extent of photons antibunching peaks precisely where the second correlation function is lowest.
We have studied non-classical effects, i.e. higher order photon antibunching (HOA) and higher order sub-Poissonian photon number statistics (HOSPS) in various non-linear optical processes like second harmonic generation, fourth harmonic generation, coherent anti-Stokes Raman scattering (CARS) and coherent anti-Stokes hyper-Raman scattering (CAHRS) using short time interaction techniques.The non-classical effects directly depend on number of photons prior to interaction with non-linear medium has already been studied but we have found that non-linear processes involving equal number of pump photons have same higher order photo antibunching (HOA) and higher order sub-Poissonian photon number statistics (HOSPS) independent of the non-linear process involved.KEYWORDS Higher order sub-Poissonian photon number statistics, higher order photon antibunching, optical processes.FOR CITATION Priyanka, Savita Gill Pump photons present in a non-linear process as a witnesses of nonclassicality of a system.
We analyze the most popular approaches to photon antibunching as exemplified in a sim-ple model of second-harmonic generation. We find the exact evolution of the fundamental and harmonic fields for initial Fock states with small photon numbers. We show explicitly that definitions of photon antibunching based on the unnormalized, G(2)(t, t′), and normal-ized, g(2)(t, t′), two-time correlation functions describe distinct phenomena for nonstationary fields. For completeness, we also compare antibunching effects defined by the two-time and single-time correlations. 1 Photon antibunching Photon antibunching and sub-Poisson photon statistics (also called antibunching) reveal the quan-tum nature of light and therefore have received a great deal of attention during the last decades. The first detection of antibunched light by Kimble, Dagenais and Mandel [1] and first detection of sub-Poisson light by Short and Mandel [2] are regarded as milestones in the progress in quantum optics. In spite of many experimental and theoretical achievements, a deeper analysis of these effects seems to be necessary, particularly in the case of nonstationary fields. We shall clarify some of these aspects by referring to an example of second-harmonic generation. There are several commonly used definitions of photon antibunching for a single-mode radiation field (e.g., Refs. [1]–[9]): Definition I: The photon antibunching (see, e.g., Ref. [3]) occurs if the two-time light intensity correlation function G(2)(t, t+ τ) increases from its initial value at τ = 0,
We have examined non classical effect i.e. higher order single mode antibunching and intermodel antibunching and higher order sub-poissonian photon statistics (HOSPS) in fifth harmonic generation non linear optical process using short time interaction technique.We have found that nonclassical effects directly depend on number of photons prior to interaction with non linear medium.The higher the number of photons present prior to an interaction, the higher will be the nonclassicality in the system.It is additionally found that stoke mode doesn't fulfill the condition of single mode antibunching and HOSPS in fifth harmonic generation process.To examine the optical nonlinearity of nanoparticles, there are significant research efforts concerning the estimation of higher order nonlinear susceptibility which can be utilized as a source for the generation of higher order harmonic generation nonlinear optical processes [19].
The squeezing and sub-Poissonian eects of light in third harmonic generation are investigated based on the fully quantum mechanical approach up to the rst order Hamiltonian interaction in gt, where g is the coupling constant between the modes per second and t is the interaction time between the waves during the process in a nonlinear medium.The coupled Heisenberg equations of motion involving real and imaginary parts of the quadrature operators are established.The occurrence of amplitude squeezing eects in both the quadratures of the radiation eld in the fundamental mode is investigated and found to be dependent on the selective phase values of the eld amplitude.The photon statistics of the pump mode in this process have also been investigated and found to be sub-Poissonian in nature.It is shown that for particular phase values the amplitude squeezing and sub-Poissonian photon statistics of light occur simultaneously.It is observed that there is no possibility to produce squeezed light in the harmonic mode up to rst-order interaction in gt.Further, it is found that the normal squeezing in the harmonic mode directly depends upon the amplitude-cubed squeezing of the initial pump eld to the case of second-order interaction in gt.This gives a method of converting higher-order (amplitude-cubed) squeezing of the fundamental mode into normal squeezing of the harmonic mode and vice versa.