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Acta Physica Polonica A

Squeezing and Sub-Poissonian Effects of Light in Third Harmonic Generation

R. Pratap, Dilip Kumar Giri, A. Prasad

Published May 1, 2014• 3 citations
Publisher

Abstract

The squeezing and sub-Poissonian eects of light in third harmonic generation are investigated based on the fully quantum mechanical approach up to the rst order Hamiltonian interaction in gt, where g is the coupling constant between the modes per second and t is the interaction time between the waves during the process in a nonlinear medium.The coupled Heisenberg equations of motion involving real and imaginary parts of the quadrature operators are established.The occurrence of amplitude squeezing eects in both the quadratures of the radiation eld in the fundamental mode is investigated and found to be dependent on the selective phase values of the eld amplitude.The photon statistics of the pump mode in this process have also been investigated and found to be sub-Poissonian in nature.It is shown that for particular phase values the amplitude squeezing and sub-Poissonian photon statistics of light occur simultaneously.It is observed that there is no possibility to produce squeezed light in the harmonic mode up to rst-order interaction in gt.Further, it is found that the normal squeezing in the harmonic mode directly depends upon the amplitude-cubed squeezing of the initial pump eld to the case of second-order interaction in gt.This gives a method of converting higher-order (amplitude-cubed) squeezing of the fundamental mode into normal squeezing of the harmonic mode and vice versa.

DOI
10.12693/aphyspola.125.1126

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The squeezing and sub-Poissonian eects of light in third harmonic generation are investigated based on the fully quantum mechanical approach up to the rst order Hamiltonian interaction in gt, where g is the coupling constant between the modes per second and t is the interaction time between the waves during the process in a nonlinear medium.The coupled Heisenberg equations of motion involving real and imaginary parts of the quadrature operators are established.The occurrence of amplitude squeezing eects in both the quadratures of the radiation eld in the fundamental mode is investigated and found to be dependent on the selective phase values of the eld amplitude.The photon statistics of the pump mode in this process have also been investigated and found to be sub-Poissonian in nature.It is shown that for particular phase values the amplitude squeezing and sub-Poissonian photon statistics of light occur simultaneously.It is observed that there is no possibility to produce squeezed light in the harmonic mode up to rst-order interaction in gt.Further, it is found that the normal squeezing in the harmonic mode directly depends upon the amplitude-cubed squeezing of the initial pump eld to the case of second-order interaction in gt.This gives a method of converting higher-order (amplitude-cubed) squeezing of the fundamental mode into normal squeezing of the harmonic mode and vice versa.
The nonclassical effects of light in the fifth harmonic generation are investigated by quantum mechanically up to the first-order Hamiltonian interaction. The coupled Heisenberg equations of motion involving real and imaginary parts of the quadrature operators are established. The occurrence of amplitude squeezing effects in both quadratures of the radiation field in the fundamental mode is investigated and found to be dependent on the selective phase values of the field amplitude. The photon statistics in the fundamental mode have also been investigated and found to be sub-Poissonian in nature. It is observed that there is no possibility to produce squeezed light in the harmonic mode up to first-order Hamiltonian interaction. Further, we have found that the normal squeezing in the harmonic mode directly depends upon the fifth power of the field amplitude of the initial pump field up to second-order Hamiltonian interaction. This gives a method of converting higher-order squeezing in the fundamental mode into normal squeezing in the harmonic mode and vice versa. The analytic expression of fifth-order squeezing of the fundamental mode in the fifth harmonic generation is established.
Abstract We theoretically investigate the emergence of nonclassical features, two-mode squeezing, sub-Poissonian photon statistics, and bipartite entanglement, in the third harmonic generation (THG) process, employing a first-order interaction Hamiltonian within the short-time approximation. The study reveals that both first- and second-order squeezing exhibit strong dependence on the input field amplitudes, relative phase, and interaction strength. Asymmetric coherent inputs, where the harmonic mode carries greater intensity than the fundamental, enhance the degree of squeezing and lead to deeper nonclassical minima. The squeezing parameters display periodic phase-dependent oscillations, indicating phase-sensitive control of quantum correlations. Sub-Poissonian photon statistics in the fundamental mode further confirm the quantum nature of the generated light. Entanglement is analyzed through the Duan et al. inseparability criterion and the Hillery–Zubairy (HZ) criteria. While the Duan criterion fails to detect entanglement under purely coherent excitation in the short-time regime, both the HZ-1 and HZ-2 criteria confirm entanglement under specific phase conditions, with HZ-2 exhibiting greater sensitivity at elevated field strengths. These results underscore the potential of THG as a viable platform for the controllable generation of nonclassical light, with implications for continuous-variable quantum optics and integrated quantum photonics.
Squeezing of electromagnetic field is investigated in fundamental mode in fourth harmonic generation under a short-time approximation based on quantum mechanical approach. The occurrence of squeezing in field amplitude and amplitude-squared of fundamental mode has been investigated. The degree of squeezing is found to be dependent on interaction time, coupling parameter of interacting waves and phase values of field amplitude of the fundamental mode during the process. The dependence of squeezing on photon number has also been noticed and found that it increases nonlinearly. The photon statistics of the field in the fundamental mode is found to be sub- Poissonian.
Squeezing of the electromagnetic field is a purely quantum mechanical phenomenon and this quantum effect is expected to manifest itself in optical processes in which the nonlinear response of the system to the radiation field plays an important role. It has generated a great deal of interest in view of the possibility of reducing the noise of an optical signal below the vacuum limit i.e. zero-point oscillations. In this paper the concept of nth-order amplitude squeezing is introduced in the fundamental mode in four- and six-wave mixing processes as a generalization of the higher-order squeezing under short-time approximation based on a fully quantum mechanical approach. It established the coupled Heisenberg equations of motion involving real and imaginary parts of the quadrature operators. The condition for occurrence of nth-order squeezing is obtained from which higher-order squeezing upto n=3 are studied. Dependence of squeezing on photon number is also established. The conditions for obtaining maximum and minimum squeezing are obtained. The method of present investigation can be applied to any higher-order non-linear optical processes and the technique can also be extended for studying squeezing in any N-photon process in general. Further, nth-order squeezing of radiation in N-photon process can also be investigated. The results obtained may help in selecting a suitable process to generate optimum squeezing in the radiation field.
We investigate theoretically the generation of squeezed states in spontaneous and stimulated six-wave mixing process quantum mechanically. It has been found that squeezing occurs in field amplitude, amplitude-squared, amplitude-cubed, and fourth power of field amplitude of fundamental mode in the process. It is found to be dependent on coupling parameter “g” (characteristics of higher-order susceptibility tensor) and phase values of the field amplitude under short-time approximation. Six-wave mixing is a process which involves absorption of three pump photons and emission of two probe photons of the same frequency and a signal photon of different frequency. It is shown that squeezing is greater in a stimulated interaction than the corresponding squeezing in spontaneous process. The degree of squeezing depends upon the photon number in first and higher orders of field amplitude. We study the statistical behaviour of quantum field in the fundamental mode and found it to be sub-Poissonian in nature. The signal-to-noise ratio has been studied in different orders. It is found that signal-to-noise ratio is higher in lower orders. This study when supplemented with experimental observations offers possibility of improving performance of many optical devices and optical communication networks.
With the help of second-order nonlinear interactions and hence Hamiltonian, we construct the equations of motion corresponding to pump and signal (second harmonic) fields in a second harmonic generation. The corresponding coupled differential equations involving the non-commuting field operators are not solvable in closed analytical forms. With the help of a perturbation method, we obtain analytical solutions of these field operators up to cubic orders in the interaction constant. In an appropriate limit (truncating the solution up to the second order in the interaction constant), these solutions lead to the existing solutions under the short-time approximation. The present analytical solutions are exploited to investigate the squeezing and the antibunching of photons of the input coherent light coupled to the said second-order nonlinear medium. We report the squeezing and antibunching effects of the pump field even for solutions up to the second order and hence the present results are consistent with earlier results. However, for the second harmonic mode, we report the squeezing involving the leading cubic term in the interaction constant.