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Fractionalization and disorder in strongly correlated systems

Shackleton, Henry Joseph

Published Jan 1, 2024• 0 citations
OpenAlex

Abstract

Emergence in systems of many electrons can lead to macroscopic demonstrations of quantum mechanics which are intrinsically many-body. A primary focus of this dissertation is the phenomena of fractionalization, where the effective quasiparticles which emerge at long distances exhibit fractional quantum numbers of the microscopic degrees of freedom. The interplay between these emergent degrees of freedom and the microscopic symmetries can lead to a number of exotic properties including competing orders and unconventional phase transitions. I explore this phenomena in a number of platforms. This includes quantum antiferromagnets which can give rise to \textit{quantum spin liquids}, where we predict critical properties of phase transitions between spin liquids and conventionally-ordered phases - due to the fractionalized excitations, such critical theories deviate from traditional Landau-Ginzburg predictions. I also study the interplay between fractionalized spin and charge excitations, as well as fractionalization in non-equilibrium contexts. The second goal of this dissertation is to investigate the properties of disordered, strongly interacting, zero dimensional systems which exemplify many notable properties of higher-dimensional systems, such as doping-induced quantum criticality and non-Fermi liquid transport. The effects of disorder play an essential role in these models, leading to phenomena such as spin glass phases and conductance fluctuations which we investigate through both numerical and analytical methods.

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Emergence in systems of many electrons can lead to macroscopic demonstrations of quantum mechanics which are intrinsically many-body. A primary focus of this dissertation is the phenomena of fractionalization, where the effective quasiparticles which emerge at long distances exhibit fractional quantum numbers of the microscopic degrees of freedom. The interplay between these emergent degrees of freedom and the microscopic symmetries can lead to a number of exotic properties including competing orders and unconventional phase transitions. I explore this phenomena in a number of platforms. This includes quantum antiferromagnets which can give rise to \textit{quantum spin liquids}, where we predict critical properties of phase transitions between spin liquids and conventionally-ordered phases - due to the fractionalized excitations, such critical theories deviate from traditional Landau-Ginzburg predictions. I also study the interplay between fractionalized spin and charge excitations, as well as fractionalization in non-equilibrium contexts. The second goal of this dissertation is to investigate the properties of disordered, strongly interacting, zero dimensional systems which exemplify many notable properties of higher-dimensional systems, such as doping-induced quantum criticality and non-Fermi liquid transport. The effects of disorder play an essential role in these models, leading to phenomena such as spin glass phases and conductance fluctuations which we investigate through both numerical and analytical methods.
The emergence of quasiparticles at low temperature provides a powerful organizing principle for many quantum phases of matter, ranging from conventional magnets and superconductors to exotic insulators with topological order. In this thesis, I describe my research in gapless quantum phases in which the framework of quasiparticles breaks down. The main characters are two categories of gapless phases that feature the interplay between strong interactions and two additional ingredients – Fermi surfaces and fractional statistics. Chapter 2 through Chapter 5 focus on strongly interacting metals with Fermi surfaces. The most salient examples are a class of Hertz-Millis models describing the onset of spontaneous symmetry breaking in a metallic environment. At the quantum critical point, gapless order parameter fluctuations destroy quasiparticles living on the Fermi surface, giving rise to a strongly coupled non-Fermi liquid metal. A key result of these chapters is the identification of an infinite-dimensional symmetry that survives in these non-Fermi liquid metals despite the death of quasiparticles. This infinite-dimensional symmetry and its quantum anomaly lead to a series of non-perturbative results on thermodynamics and transport, which are confirmed by perturbative diagrammatic calculations in special examples. Chapter 6 through Chapter 8 explore quantum phases in which anyonic quasiparticles with fractional statistics play an essential role. When parameters in the system are tuned to close the anyon energy gaps, the original anyons lose their coherence and a variety of novel phases emerge. A highlight in this direction is a new mechanism for topological superconductivity in itinerant abelian and non-abelian anyon fluids, which could make contact with experiments on doped fractional quantum anomalous Hall states in the near future.
In this dissertation we study the properties of quantum many-body systems whose behavior is governed by strong correlation effects between large numbers of degrees of freedom. We begin with a review of various types of condensed matter settings and a general discussion of how interactions can lead to qualitatively new properties. In Chapter 2 we discuss a class of spin models which generate nontrivial realizations of a global symmetry, both in the presence and absence of topological order. In Chapter 3, we examine a model of a non-Fermi liquid. This model is built out of electron-like degrees of freedom and has a Fermi surface, yet has no stable quasiparticle excitations. In Chapter 4 we discuss some aspects of entanglement entropy in gapless multi-component systems, and suggest a way of measuring the topological properties of Kondo lattice wavefunctions.
The discovery of high-temperature superconductors has raises questions that extend beyond the scope of quasiparticles, a foundational concept in condensed matter theory. This dissertation explores new theoretical approaches to quantum matter without quasiparticle excitations, with a particular focus on quantum criticality and the associated superconductivity in correlated electron compounds. The soluble Sachdev-Ye-Kitaev (SYK) model has recently emerged as a fascinating platform to address the unusual metallic states with T-linear resistivity. We first consider differ- ent variants of random Hubbard models, which share many similarities to key aspects of the original SYK model. Using a large M analysis and a renormalization group method, we propose the existence of quantum critical points with fractionalized excitations separating two distinct phases, which provides insights into the quantum phase transitions and non-Fermi liquid behaviors observed in cuprate superconductors. In the second part of this dissertation, we examine the interplay between non-Fermi liquids and superconductivity with two different pairing mechanisms. Under the framework of random Hubbard model, we demonstrate that superconductivity emerging from non-Fermi liquids strongly deviates from the BCS theory by tuning the relative strength of hopping and exchange interactions. Furthermore, we investigate a two-dimensional Yukawa-SYK model with spatially randomn interactions coupling a Fermi surface to a scalar field associated with a quantum phase transition. Our theory agrees well with transport properties analysed in cuprates, such as a T-linear resistivity and Planckian dissipation.
This thesis is devoted to the study of strongly correlated phases of quantum matter in two spatial dimensions. In presence of strong interactions, the electron can split up into separate spin and charge degrees of freedom. The diagnosis of such fractionalized excitations in recent experiments, as well as finding new probes for their detection, comprise the two major themes of this thesis.\nThe first part of the thesis, comprising chapters 2-6, discusses the relevance of fractionalization to the pseudogap phase of the underdoped high Tc cuprate superconductors. This is motivated by transport experiments that show a violation of Luttinger's theorem, possible only in the presence of topological order that can arise naturally as a consequence of fractionalization. Chapters 2 and 3 focus on phenomenological models with bosonic charge carriers and fermionic spin carriers, and investigate transport properties as well as various confinement transitions to symmetry broken phases. Chapters 4, 5 and 6 deal with a different framework of electron fractionalization, where the charge carriers are fermionic and spin carriers are bosonic. We find that these models can better explain the thermal and electrical transport properties in chapter 5. In chapters 6 and 7, we show how such models arise naturally from quantum fluctuations of antiferromagnetism, and can simultaneously intertwine the anti-nodal spectral gap with the discrete broken symmetries that are observed in the cuprates. \nThe second part of the thesis, comprising chapters 7 and 8, proposes new experimental probes to study the behavior of insulating two dimensional quantum magnets. Aided by geometric frustration and strong quantum fluctuations, they may realize a spin liquid ground state which can be extremely difficult to detect via conventional probes. Chapter 7 discusses how novel spin-transport probes from the spintronics community can be used to detect fractionalized excitations in a quantum spin liquid. Chapter 8 studies how the temperature dependent anisotropy of in-plane versus out-of-plane thermal conductivities can serve as an explicit signature of fractionalization in layered two-dimensional materials.
This dissertation establishes and investigates new phenomena in diverse interacting many-body quantum systems guided by three distinct, but complementary, themes: (i) symmetry and topology, (ii) localization, and (iii) non-Fermi liquids. The first theme concerns how the interplay of symmetry and topology can offer robust protection for a many-body system. We investigate low-dimensional quantum fermionic models from a general structural perspective. These phases can exhibit fractionalized Majorana zero-energy modes on their boundary. We devise experimentally relevant nonlocal measurements that can be used to detect these topological phases. While our primary focus is on quantum systems, topologically protected behavior can arise in classical mechanical models as well. We extend a recent connection between the topological band theory of electrons and classical physics by proposing a mechanical analogue of a topological nodal semimetal.The second theme concerns that of many-body localization. We demonstrate that the combination of localization, symmetry, and topology can have radical consequences for quantum systems at high energies, such as the existence of protected gapless boundary modes. We show that, even at these high energies, quantum information can be preserved, and quantum coherence recovered. Quantum coherent dynamics in this regime is unexpected and of great interest for quantum computation.The third direction in our study of interacting many-body systems concerns non-Fermi liquids. We construct a non-Fermi liquid by bringing together a spin-orbit coupled Fermi surface and fluctuating magnetic order. Using newly developed analytic tools for strongly coupled systems, we demonstrate the stability of the non-Fermi liquid to ordering. This identifies an experimentally accessible candidate for exploring physics that lies beyond Fermi liquid theory.
The interplay among symmetry, topology and condensed matter systems has deepened our understandings of matter and lead to tremendous recent progresses in finding new topological phases of matter such as topological insulators, superconductors and semi-metals. Most examples of the aforementioned topological materials are free fermion systems, in this thesis, however, we focus on their strongly correlated counterparts where electron-electron interactions play a major role. With interactions, exotic topological phases and quantum critical points with fractionalized quantum degrees of freedom emerge. In the first part of this thesis, we study the problem of resonant tunneling through a quantum dot in a spinful Luttinger liquid. It provides the simplest example of a (0+1)d system with symmetry-protected phase transitions. We show that the problem is equivalent to a two channel SU(3) Kondo problem and can be mapped to a quantum Brownian motion model on a Kagome lattice. Utilizing boundary conformal field theory, we find the universal peak conductance and compute the scaling behavior of the resonance line-shape.\nFor the second part, we present a model of interacting Majorana fermions that describes a superconducting phase with a topological order characterized by the Fibonacci topological field theory. Our theory is based on a SO(7)1=SO(7)1/(G2)1 x (G2)1 coset construction and implemented by a solvable two-dimensional network model. In addition, we predict a closely related ''anti-Fibonacci'' phase, whose topological order is characterized by the tricritical Ising model. Finally, we propose an interferometer that generalizes the Z2 Majorana interferometer and directly probes the Fibonacci non-Abelian statistics.\nFor the third part, we argue that a correlated fluid of electrons and holes can exhibit fractional quantum Hall effects at zero magnetic field. We first show that a Chern insulator can be realized as a free fermion model with p-wave(m=1) excitonic pairing. Its ground state wavefunction is then worked out and generalized to m>1. We give several pieces of evidence that this conjectured wavefunction correctly describes a topological phase, dubbed ''fractional excitonic insulator'', within the same universality class as the corresponding Laughlin state at filling 1/m. We present physical arguments that gapless states with higher angular momentum pairing between energy bands are conducive to forming the fractional excitonic insulator in the presence of repulsive interactions. Without interactions, these gapless states appear at topological phase transitions which separate the trivial insulator from a Chern insulator with higher Chern number. Since the nonvanishing density of states at these higher angular momentum band inversion transitions can give rise to interesting many-body effects, we introduce a series of minimal lattice models realizations in two dimensions. We also study the effect of rotational symmetry broken electron-hole exciton condensation in our lattice models using mean field theory.