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Clock to Rydberg state transition measurement in a neutral strontium atom cloud

Hamers, Carolus G.H.P.

Published Aug 1, 2025• 0 citations
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Clouds of ultracold strontium $5s48s\phantom{\rule{4pt}{0ex}}{}^{1}{S}_{0}$ or $5s47d\phantom{\rule{4pt}{0ex}}{}^{1}{D}_{2}$ Rydberg atoms are created by two-photon excitation of laser-cooled $5{s}^{2}\phantom{\rule{4pt}{0ex}}{}^{1}{S}_{0}$ atoms. The spontaneous evolution of the cloud of low orbital angular momentum (low-$\ensuremath{\ell}$) Rydberg states towards an ultracold neutral plasma is observed by imaging resonant light scattered from core ions, a technique that provides both spatial and temporal resolution. Evolution is observed to be faster for the $S$ states, which display isotropic attractive interactions, than for the $D$ states, which exhibit anisotropic, principally repulsive interactions. Immersion of the atoms in a dilute ultracold neutral plasma speeds up the evolution and allows the number of Rydberg atoms initially created to be determined.

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We present a proposal of determination of the density shift of the1S0-3P0clock transition in neutral cold strontium atoms. Since the direct use of the double forbidden, intercombination clock transition (698 nm) may be difficult we propose to use a three photon photoassociation. The measurement will be performed with the magneto-optical trap set-up designed for the experiments with both88Sr and87Sr isotopes.

Joint Conference of the European Frequency and Time Forum and IEEE International Frequency Control Symposium (EFTF/IFCS)•Jul 1, 2013•0 citations
We show that optical spectroscopy of Rydberg states can provide accurate in situ thermometry at room temperature. Transitions from a metastable state to Rydberg states with principal quantum numbers of 25-30 have 200 times larger fractional frequency sensitivities to blackbody radiation than the strontium clock transition. We demonstrate that magic-wavelength lattices exist for both strontium and ytterbium transitions between the metastable and Rydberg states. Frequency measurements of Rydberg transitions with 10(-16) accuracy provide 10 mK resolution and yield a blackbody uncertainty for the clock transition of 10(-18).
Clouds of ultracold strontium 5s48s1S05s48s\phantom{\rule{4pt}{0ex}}{}^{1}{S}_{0}5s48s1S0​ or 5s47d1D25s47d\phantom{\rule{4pt}{0ex}}{}^{1}{D}_{2}5s47d1D2​ Rydberg atoms are created by two-photon excitation of laser-cooled 5s21S05{s}^{2}\phantom{\rule{4pt}{0ex}}{}^{1}{S}_{0}5s21S0​ atoms. The spontaneous evolution of the cloud of low orbital angular momentum (low-$\ensuremath{\ell}$) Rydberg states towards an ultracold neutral plasma is observed by imaging resonant light scattered from core ions, a technique that provides both spatial and temporal resolution. Evolution is observed to be faster for the SSS states, which display isotropic attractive interactions, than for the DDD states, which exhibit anisotropic, principally repulsive interactions. Immersion of the atoms in a dilute ultracold neutral plasma speeds up the evolution and allows the number of Rydberg atoms initially created to be determined.