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Physical Review Letters

Zero-Dead-Time Strontium Lattice Clock with a Stability at 10 − 19 Level

Xiao-Yong Liu, Peng Liu, Jie Li, Yu-Chen Zhang, Yuan-Bo Wang, Zhi-Peng Jia, Xiang Zhang, Xian-Qing Zhu, De-Quan Kong, Wen-Lan Song, Guo-Zhen Niu, Yu-Meng Yang, Pei-Jun Feng, Xiang-Pei Liu, Xing-Yang Cui, Ping Xu, Xiao Jiang, Juan Yin, Sheng-Kai Liao, Cheng-Zhi Peng, Han-Ning Dai, Yu-Ao Chen, Jian-Wei Pan

Published Nov 26, 2025• 9 citations
Publisher

Abstract

Optical atomic clocks play a crucial role in fundamental physics, relativistic geodesy, and the future redefinition of the Systeme International second. Standard operation relies on cyclic interrogation sequences, which alternate between atomic interrogation and dead time used for state preparation and readout. This approach introduces the Dick effect, where laser frequency noise aliases onto the atomic transition frequency. Although reducing laser noise improves clock stability, the Dick effect remains a key limitation. In this Letter, we demonstrate a zero-dead-time optical clock based on two interleaved ensembles of cold ^{87}Sr atoms. Our system significantly suppresses this noise and achieves a fractional frequency instability at the 10^{-19} level between 10 000 and 20 000 s over repeated measurements, with a best value of 2.9×10^{-19} at τ=20000 s. The estimated long-term stability based on the combined data of these measurements reaches 2.5×10^{-19} at 1 day. These results represent a more than ninefold improvement over a conventional single-ensemble clock, highlighting its potential for next-generation timekeeping applications.

DOI
10.1103/zbpb-6qxb

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Frequency metrology underpins precise measurements. At the forefront of this field are optical clocks which can perform measurements that are accurate to more digits than those in the number representing seconds elapsed from the beginning of the universe. Frequency estimation errors in the operation of optical clocks lead to frequency instability, prohibiting them from reaching high accuracies on short to medium time scales, and limiting access to interesting measurements of the atomic environment and exotic external perturbations such as gravity fields or fields of fundamentally new physical origins. Optical lattice traps are typically employed in state-of-the-art optical clocks to suppress Doppler effects. By carefully tuning the optical lattice to the magic wavelength, unwanted Stark shifts can be suppressed significantly, allowing operation with thousands of atoms and minimising the fundamental source of frequency estimation errors, namely the quantum projection noise, to around 3 × 10−17 at 1 s. In this thesis, the status of the two Strontium optical lattice clocks at NPL, Sr1 and Sr2, is presented going over a few interesting measurement campaigns from the past years involving Sr1 and the latest experimental efforts to re-enable operation of Sr2. A model of clock stability is developed by incorporating known and new frameworks to characterise the relation between the operating parameters of optical clocks and their performance, with relevance to the NPL lattice clocks and beyond. In particular, a method is identified for addressing the main technical noise for optical lattice clocks, the Dick effect, which typically has a magnitude of 10−16 at 1 s and prevents optical lattice clocks from reaching the quantum projection noise level. By taking advantage of dynamical decoupling we can engineer an optimised duty cycle with benefits in general for systems limited by the optical coherence of the clock laser. Moreover, a study of other noise sources in the NPL lattice clocks is conducted using synchronous measurements between Sr1 and Sr2, revealing a large contribution from linear Zeeman shifts, also at the 10−16 level, and a plan to tackle them is detailed. A hybrid clock architecture is discussed showing how optical lattice clocks can improve the optical coherence of ion clocks thanks to their higher servo rate, and a preliminary experimental demonstration is reported. Finally, a new type of spectroscopy is presented which completely avoids aliasing of linear Zeeman shifts by simultaneously driving transitions with opposite Zeeman sensitivities. Such a technique also enables the continuous interrogation of atoms, a crucial missing component in the Dick-free conveyor belt lattice clock concept heralded as the next standard of stable optical clocks.

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The stability of an optical atomic clock is a critical figure of merit for almost all clock applications. To this end, much optical atomic clock research has focused on reducing clock instability by increasing the atom number, lengthening the coherent interrogation times, and introducing entanglement to push beyond the standard quantum limit. In this work, we experimentally demonstrate an alternative approach to reducing clock instability using a phase estimation approach based on individually controlled atomic ensembles in a strontium (Sr) optical lattice clock. We first demonstrate joint Ramsey interrogation of two spatially resolved atom ensembles that are out of phase with respect to each other, which we call “quadrature Ramsey spectroscopy,” resulting in a factor of 1.36(5) reduction in absolute clock instability as measured with interleaved self-comparisons. We then leverage the rich hyperfine structure of Sr87 to realize independent coherent control over multiple ensembles with only global laser addressing. Finally, we utilize this independent control over four atom ensembles to implement a form of phase estimation, achieving a factor of greater than 3 enhancement in coherent interrogation time and a factor of 2.08(6) reduction in instability over an otherwise identical single-ensemble clock with the same local oscillator and the same number of atoms. We expect that multiensemble protocols similar to those demonstrated here will result in reduction in the instability of any optical lattice clock with an interrogation time limited by the local oscillator. Published by the American Physical Society 2024

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Optical atomic clocks play a crucial role in fundamental physics, relativistic geodesy, and the future redefinition of the Systeme International second. Standard operation relies on cyclic interrogation sequences, which alternate between atomic interrogation and dead time used for state preparation and readout. This approach introduces the Dick effect, where laser frequency noise aliases onto the atomic transition frequency. Although reducing laser noise improves clock stability, the Dick effect remains a key limitation. In this Letter, we demonstrate a zero-dead-time optical clock based on two interleaved ensembles of cold ^{87}Sr atoms. Our system significantly suppresses this noise and achieves a fractional frequency instability at the 10^{-19} level between 10 000 and 20 000 s over repeated measurements, with a best value of 2.9×10^{-19} at τ=20000 s. The estimated long-term stability based on the combined data of these measurements reaches 2.5×10^{-19} at 1 day. These results represent a more than ninefold improvement over a conventional single-ensemble clock, highlighting its potential for next-generation timekeeping applications.
Abstract We describe a method of duty cycle engineering in optical lattice clocks to reduce clock instability through tailoring of the Dick effect noise contribution. We apply dynamically decoupled interrogation sequences to realise an estimated improvement in single clock instability approaching a factor of two, as well as providing a route to zero dead-time operation for two interleaved clocks which are otherwise unable to reach the required duty cycle. We show through simulations and synchronous measurements of clocks NPL-Sr1 and NPL-Sr2 that a quantum projection noise limited instability < 3 − 10−17 τ −1/2 can be realised in a near ideal zero dead-time configuration.
The stability of current state-of-the-art optical atomic clocks [1]-[5] is mostly limited by the frequency noise of the interrogation oscillator through the Dick effect. To achieve the heralded ultimate stability, future optical frequency standards will need to produce light sources with frequency stability at the 10−17fractional level or below at one second of integration time. Recently, a new frontier in cavity stabilized laser sources has pushed the fractional instability to the lower 10−16level at one second of integration time [6]-[8]. However, this instability is limited by thermal noise in the reference cavity elements and may be difficult to reduce further. These state-of-the-art reference cavities are technically challenging to construct and their stability is still at least an order of magnitude too large for lattice clocks to achieve their ultimate performance.
Frequency metrology underpins precise measurements. At the forefront of this field are optical clocks which can perform measurements that are accurate to more digits than those in the number representing seconds elapsed from the beginning of the universe. Frequency estimation errors in the operation of optical clocks lead to frequency instability, prohibiting them from reaching high accuracies on short to medium time scales, and limiting access to interesting measurements of the atomic environment and exotic external perturbations such as gravity fields or fields of fundamentally new physical origins. Optical lattice traps are typically employed in state-of-the-art optical clocks to suppress Doppler effects. By carefully tuning the optical lattice to the magic wavelength, unwanted Stark shifts can be suppressed significantly, allowing operation with thousands of atoms and minimising the fundamental source of frequency estimation errors, namely the quantum projection noise, to around 3 × 10−17 at 1 s. In this thesis, the status of the two Strontium optical lattice clocks at NPL, Sr1 and Sr2, is presented going over a few interesting measurement campaigns from the past years involving Sr1 and the latest experimental efforts to re-enable operation of Sr2. A model of clock stability is developed by incorporating known and new frameworks to characterise the relation between the operating parameters of optical clocks and their performance, with relevance to the NPL lattice clocks and beyond. In particular, a method is identified for addressing the main technical noise for optical lattice clocks, the Dick effect, which typically has a magnitude of 10−16 at 1 s and prevents optical lattice clocks from reaching the quantum projection noise level. By taking advantage of dynamical decoupling we can engineer an optimised duty cycle with benefits in general for systems limited by the optical coherence of the clock laser. Moreover, a study of other noise sources in the NPL lattice clocks is conducted using synchronous measurements between Sr1 and Sr2, revealing a large contribution from linear Zeeman shifts, also at the 10−16 level, and a plan to tackle them is detailed. A hybrid clock architecture is discussed showing how optical lattice clocks can improve the optical coherence of ion clocks thanks to their higher servo rate, and a preliminary experimental demonstration is reported. Finally, a new type of spectroscopy is presented which completely avoids aliasing of linear Zeeman shifts by simultaneously driving transitions with opposite Zeeman sensitivities. Such a technique also enables the continuous interrogation of atoms, a crucial missing component in the Dick-free conveyor belt lattice clock concept heralded as the next standard of stable optical clocks.
Optical atomic clocks have spurred a range of precision frequency comparison experiments and proposals including tests of general relativity, gravitational wave detection, and relativistic geodesy. Current measurements using optical atomic clocks are often limited by the coherence of the clock laser rather than the atomic samples used as a frequency reference. In order to overcome the performance limits imposed by clock laser coherence, we realize a multiplexed optical clock system where multiple spatially resolved ensembles each consisting of thousands of strontium atoms trapped in a 1D optical lattice function as separate atomic frequency references that can be simultaneously interrogated with a shared clock laser. This scheme allows us to make differential frequency comparisons with a quantum projection noise limited fractional instability of 9.7(4)×10−18/ √τ and a differential fractional uncertainty of 8.9×10−20 after 3.3 hours of averaging. We then use this system to perform a lab-based test of the gravitational redshift at the centimeter scale, where we measure a fractional frequency gradient of [−12.4±0.7stat ±2.5sys]×10−19/cm, consistent with the predicted value of 10.9×10−19/cm. Having demonstrated that our differential comparisons are no longer limited by the local oscillator, we turn to fundamental limits on atom–atom coherence. We perform a direct decay measurement of the natural lifetime of the excited clock state 3P0 in 87Sr, in which we use measurements of simultaneously loaded high and low density atomic ensembles and compare decay rates of 87Sr and 88Sr to help isolate natural lifetime decay from other population dynamics. We measure a lifetime of 167+79 −40, which is consistent with previously reported experimental and theoretical values. Lastly, we demonstrate a hyperfine-resolved readout scheme in 87Sr that converts depolarization errors during interrogation into erasure errors, extending coherence times between ensembles in our optical lattice clock up to 150s using spin-echo measurements. These results taken together demonstrate the advantages of differential clock measurements that aren’t limited by clock laser coherence and how to characterize and improve on the performance limits that arise in that regime.
Optical lattice clocks achieve fractional frequency uncertainties of 10⁻¹⁸, yet stability is constrained by the dead time between cooling, preparation, interrogation, and detection. This sampling aliases local-oscillator noise into the clock signal (the Dick effect) and prevents continuous accumulation of oscillator phase information. We demonstrate spatially defined Rabi spectroscopy of ultracold ⁸⁸Sr atoms continuously transported in a moving optical lattice. A longitudinal excitation geometry preserves Lamb-Dicke confinement and suppresses Doppler broadening. Clock excitation is enabled only within a localised region by a transverse magnetic mixing field, defining the atom-laser interaction in space rather than in time and decoupling interrogation from preparation and detection. Transporting atoms at 16 mm s⁻¹ through a 12-mm interaction region yields a 1.2-Hz-wide spectrum close to the transit-time Fourier limit while maintaining uninterrupted atom delivery. This approach provides a practical route toward dead-time-free optical clock interrogation of continuously delivered atomic ensembles.
The stability of an optical atomic clock is a critical figure of merit for almost all clock applications. To this end, much optical atomic clock research has focused on reducing clock instability by increasing the atom number, lengthening the coherent interrogation times, and introducing entanglement to push beyond the standard quantum limit. In this work, we experimentally demonstrate an alternative approach to reducing clock instability using a phase estimation approach based on individually controlled atomic ensembles in a strontium (Sr) optical lattice clock. We first demonstrate joint Ramsey interrogation of two spatially resolved atom ensembles that are out of phase with respect to each other, which we call “quadrature Ramsey spectroscopy,” resulting in a factor of 1.36(5) reduction in absolute clock instability as measured with interleaved self-comparisons. We then leverage the rich hyperfine structure of Sr87 to realize independent coherent control over multiple ensembles with only global laser addressing. Finally, we utilize this independent control over four atom ensembles to implement a form of phase estimation, achieving a factor of greater than 3 enhancement in coherent interrogation time and a factor of 2.08(6) reduction in instability over an otherwise identical single-ensemble clock with the same local oscillator and the same number of atoms. We expect that multiensemble protocols similar to those demonstrated here will result in reduction in the instability of any optical lattice clock with an interrogation time limited by the local oscillator. Published by the American Physical Society 2024