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Joint Conference of the European Frequency and Time Forum and IEEE International Frequency Control Symposium (EFTF/IFCS)

Prospects for frequency stabilization using collective effects of strontium atoms in an optical cavity

Bjarke T. R. Christensen, Martin R. Henriksen, Philip G. Westergaard, Jun Ye, Jan W. Thomsen

Published May 1, 2014• 0 citations
Publisher

Abstract

The stability of current state-of-the-art optical atomic clocks [1]-[5] is mostly limited by the frequency noise of the interrogation oscillator through the Dick effect. To achieve the heralded ultimate stability, future optical frequency standards will need to produce light sources with frequency stability at the 10−17fractional level or below at one second of integration time. Recently, a new frontier in cavity stabilized laser sources has pushed the fractional instability to the lower 10−16level at one second of integration time [6]-[8]. However, this instability is limited by thermal noise in the reference cavity elements and may be difficult to reduce further. These state-of-the-art reference cavities are technically challenging to construct and their stability is still at least an order of magnitude too large for lattice clocks to achieve their ultimate performance.

DOI
10.1109/fcs.2014.6859907

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The stability of current state-of-the-art optical atomic clocks [1]-[5] is mostly limited by the frequency noise of the interrogation oscillator through the Dick effect. To achieve the heralded ultimate stability, future optical frequency standards will need to produce light sources with frequency stability at the 10−17fractional level or below at one second of integration time. Recently, a new frontier in cavity stabilized laser sources has pushed the fractional instability to the lower 10−16level at one second of integration time [6]-[8]. However, this instability is limited by thermal noise in the reference cavity elements and may be difficult to reduce further. These state-of-the-art reference cavities are technically challenging to construct and their stability is still at least an order of magnitude too large for lattice clocks to achieve their ultimate performance.
Optical atomic clocks play a crucial role in fundamental physics, relativistic geodesy, and the future redefinition of the Systeme International second. Standard operation relies on cyclic interrogation sequences, which alternate between atomic interrogation and dead time used for state preparation and readout. This approach introduces the Dick effect, where laser frequency noise aliases onto the atomic transition frequency. Although reducing laser noise improves clock stability, the Dick effect remains a key limitation. In this Letter, we demonstrate a zero-dead-time optical clock based on two interleaved ensembles of cold ^{87}Sr atoms. Our system significantly suppresses this noise and achieves a fractional frequency instability at the 10^{-19} level between 10 000 and 20 000 s over repeated measurements, with a best value of 2.9×10^{-19} at τ=20000 s. The estimated long-term stability based on the combined data of these measurements reaches 2.5×10^{-19} at 1 day. These results represent a more than ninefold improvement over a conventional single-ensemble clock, highlighting its potential for next-generation timekeeping applications.
Ultra stable frequency references such as the ones used in optical atomic clocks and for quantum metrology may be obtained by stabilizing a laser to an optical cavity that is stable over time. State-of-the-art frequency references are constructed in this way, but their stabilities are currently limited by thermally induced length fluctuations in the reference cavity. Several alternative approaches using the potential for frequency discriminating of highly forbidden narrow atomic transitions have been proposed in, e.g., [1] and [2]. In this proceeding we will present some of the ongoing experimental efforts derived from these proposals, to use cavity-enhanced interaction with atomic 88 Sr samples as a frequency reference for laser stabilization. Such systems can be realized using both passive and active approaches where either the atomic phase response is used as an error signal, or the narrow atomic transition itself is used as a source for a spectrally pure laser. Both approaches shows the promise of being able to compete with the current state of the art in stable lasers and have similar limitations on their ultimately achievable linewidths [1, 2].
Current state-of-the-art frequency standards are passive optical atomic clocks where the frequency of an optical resonator is stabilized to a narrow atomic transition. Passive clocks have achieved unprecedented stabilities of 6.6 x 10--19 over one hour of averaging time [1]. However, they face intrinsic limitations, particularly due to thermal and mechanical fluctuations of the local oscillator. To surpass the limitations of the passive clocks and go beyond the state-of-the-art, the idea of building active optical atomic clocks emerges. These clocks would be optical counterparts of hydrogen masers, with the emitted frequency defined by the atomic transition and therefore inherently stable against cavity instabilities. This paper discusses the latest developments and future prospects in the field of active optical atomic clocks.
Frequency metrology underpins precise measurements. At the forefront of this field are optical clocks which can perform measurements that are accurate to more digits than those in the number representing seconds elapsed from the beginning of the universe. Frequency estimation errors in the operation of optical clocks lead to frequency instability, prohibiting them from reaching high accuracies on short to medium time scales, and limiting access to interesting measurements of the atomic environment and exotic external perturbations such as gravity fields or fields of fundamentally new physical origins. Optical lattice traps are typically employed in state-of-the-art optical clocks to suppress Doppler effects. By carefully tuning the optical lattice to the magic wavelength, unwanted Stark shifts can be suppressed significantly, allowing operation with thousands of atoms and minimising the fundamental source of frequency estimation errors, namely the quantum projection noise, to around 3 × 10−17 at 1 s. In this thesis, the status of the two Strontium optical lattice clocks at NPL, Sr1 and Sr2, is presented going over a few interesting measurement campaigns from the past years involving Sr1 and the latest experimental efforts to re-enable operation of Sr2. A model of clock stability is developed by incorporating known and new frameworks to characterise the relation between the operating parameters of optical clocks and their performance, with relevance to the NPL lattice clocks and beyond. In particular, a method is identified for addressing the main technical noise for optical lattice clocks, the Dick effect, which typically has a magnitude of 10−16 at 1 s and prevents optical lattice clocks from reaching the quantum projection noise level. By taking advantage of dynamical decoupling we can engineer an optimised duty cycle with benefits in general for systems limited by the optical coherence of the clock laser. Moreover, a study of other noise sources in the NPL lattice clocks is conducted using synchronous measurements between Sr1 and Sr2, revealing a large contribution from linear Zeeman shifts, also at the 10−16 level, and a plan to tackle them is detailed. A hybrid clock architecture is discussed showing how optical lattice clocks can improve the optical coherence of ion clocks thanks to their higher servo rate, and a preliminary experimental demonstration is reported. Finally, a new type of spectroscopy is presented which completely avoids aliasing of linear Zeeman shifts by simultaneously driving transitions with opposite Zeeman sensitivities. Such a technique also enables the continuous interrogation of atoms, a crucial missing component in the Dick-free conveyor belt lattice clock concept heralded as the next standard of stable optical clocks.
Abstract Current state-of-the-art frequency standards are passive optical atomic clocks where the frequency of an optical resonator is stabilized to a narrow atomic transition. Passive clocks have achieved unprecedented stabilities of 6.6 × 10−19 over one hour of averaging time [1]. However, they face intrinsic limitations, particularly due to thermal and mechanical fluctuations of the local oscillator. To surpass the limitations of the passive clocks and go beyond the state-of-the-art, the idea of building active optical atomic clocks emerges. These clocks would be optical counterparts of hydrogen masers, with the emitted frequency defined by the atomic transition and therefore inherently stable against cavity instabilities. This paper discusses the latest developments and future prospects in the field of active optical atomic clocks.
We present the advancement toward the realization of a new optical clock apparatus based on ultracold strontium atoms. The atomic source employs a novel design based on two dimensional magneto optical trapping which is advantageous because of the suppression of thermal atoms in the interrogation volume, and the elimination of hot BBR in the view of the science cell. Compact frequency stabilization of cooling and trapping lasers is achieved via single PDH lock to a three-color ultrastable optical resonator. We also study different lattice topologies to operate the ultracold atomic ensemble in the high-cooperativity regime toward sub-quantum projection noise instability and millihertz-linewidth frequency stabilization by cavity QED.