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Physical review. B./Physical review. B

Field-induced triplon Bose-Einstein condensation in the spin- 1 2 quantum dimer magnet Cu(en) 2 SO 4

Fangli Li, Lei Xu, Jiong Yang, Han Ge, Nan Zhao, Zhitao Zhang, Wei Tong, Zhentao Wang, Jieming Sheng, Liusuo Wu

Published Dec 10, 2025• 1 citation
Publisher
DOI
10.1103/j2xg-rghr

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Motivated by recent experiments on Ba3Cr2O8{\text{Ba}}_{3}{\text{Cr}}_{2}{\text{O}}_{8}Ba3​Cr2​O8​, a new spin-dimer compound with spin-1/2 moments of Cr5+{\text{Cr}}^{5+}Cr5+ ions, we theoretically investigate the field-induced magnetic ordering in this material in view of the Bose-Einstein condensation (BEC) of triplet excitations (triplons). We apply the self-consistent Hartree-Fock-Popov (HFP) approach to a microscopic Hamiltonian, using the realistic triplon dispersion measured in an inelastic neutron-scattering experiment. In particular, we ask to what extent the BEC of dilute triplons near the critical field can explain the magnetic ordering in this material. For example, we investigate the temperature range where the BEC picture of triplons can be applied via the HFP approach. We also determine the temperature regime where a quadratic approximation of the triplon dispersion works. It is found that the strength of the effective repulsive interaction between triplons is much weaker in Ba3Cr2O8{\text{Ba}}_{3}{\text{Cr}}_{2}{\text{O}}_{8}Ba3​Cr2​O8​ than in the canonical spin-dimer compound TlCuCl3{\text{TlCuCl}}_{3}TlCuCl3​. Small effective repulsive interaction in combination with the narrow band of triplons leads to higher density of triplons ncr{n}_{\text{cr}}ncr​ at the critical point. The combined effect points to a bigger HFP correction UncrU{n}_{\text{cr}}Uncr​ in Ba3Cr2O8{\text{Ba}}_{3}{\text{Cr}}_{2}{\text{O}}_{8}Ba3​Cr2​O8​ than in TlCuCl3{\text{TlCuCl}}_{3}TlCuCl3​. Nonetheless, the HFP approach provides a reasonable explanation of the transverse magnetization and the specific-heat data of Ba3Cr2O8{\text{Ba}}_{3}{\text{Cr}}_{2}{\text{O}}_{8}Ba3​Cr2​O8​.