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Manipulating Two-Photon Interference Using Metasurfaces

Wai Hin Fan

Published Jan 1, 2025• 0 citations
Publisher

Abstract

Interference experiments like the light and electron double-slit are crucially important to quantum mechanics since they illustrate the core principle of wave-particle duality, by demonstrating the wave-like aspect of particle phenomena. In such experiments, a device is typically required to manipulate the particle-wave dual phenomenon, producing controllable interference. Metasurfaces, with their highly flexible configurability, can serve as more versatile versions of such devices. They are powerful tools capable of modulating a broader category of effects beyond classical interference, such as the quantum Hong-Ou-Mandel (HOM) effect. The HOM effect is caused by interference taking place not between coherent waves from distinct sources which intersect in real space, but rather between parallel processes indistinguishable to the measurement apparatus. Existing research has highlighted the outsized importance of measurement in HOM interferometry, by showing that the occurrence of process interference depends only on indistinguishability at the detectors and nowhere else. We are therefore interested in how quantum measurement occurs in HOM, and how metasurfaces can be used to enhance the HOM effect. In this thesis, we extend a formulation of quantum trajectory theory in two-eigenstate systems to 𝑁-state systems, producing a three-state formalism which serves as a possible description of coincidence pair detection in HOM experiments. We then develop an analytic model of polarisation HOM interferometry capturing both the width and the 𝑔2 ratio of the HOM dip; finally, we design and fabricate a metasurface that exhibits polarisation filtering with respect to two-photon coincidence, whereupon HOM photon bunching occurs only at select metasurface orientations relative to photon polarisation. Our three-state quantum state collapse model offers a promising explanation for how state measurement takes place in an HOM interferometer, where the interferometer output is a superimposition of three two-photon eigenstates. Meanwhile, our interferometer model and experiments provide evidence of successful polarisation filtering in HOM interferometry.

DOI
10.14711/thesis-hdl152591

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•Aug 31, 2017•1 citation
Interference experiments like the light and electron double-slit are crucially important to quantum mechanics since they illustrate the core principle of wave-particle duality, by demonstrating the wave-like aspect of particle phenomena. In such experiments, a device is typically required to manipulate the particle-wave dual phenomenon, producing controllable interference. Metasurfaces, with their highly flexible configurability, can serve as more versatile versions of such devices. They are powerful tools capable of modulating a broader category of effects beyond classical interference, such as the quantum Hong-Ou-Mandel (HOM) effect. The HOM effect is caused by interference taking place not between coherent waves from distinct sources which intersect in real space, but rather between parallel processes indistinguishable to the measurement apparatus. Existing research has highlighted the outsized importance of measurement in HOM interferometry, by showing that the occurrence of process interference depends only on indistinguishability at the detectors and nowhere else. We are therefore interested in how quantum measurement occurs in HOM, and how metasurfaces can be used to enhance the HOM effect. In this thesis, we extend a formulation of quantum trajectory theory in two-eigenstate systems to 𝑁-state systems, producing a three-state formalism which serves as a possible description of coincidence pair detection in HOM experiments. We then develop an analytic model of polarisation HOM interferometry capturing both the width and the 𝑔2 ratio of the HOM dip; finally, we design and fabricate a metasurface that exhibits polarisation filtering with respect to two-photon coincidence, whereupon HOM photon bunching occurs only at select metasurface orientations relative to photon polarisation. Our three-state quantum state collapse model offers a promising explanation for how state measurement takes place in an HOM interferometer, where the interferometer output is a superimposition of three two-photon eigenstates. Meanwhile, our interferometer model and experiments provide evidence of successful polarisation filtering in HOM interferometry.
Hong-Ou-Mandel (HOM) interference [1] is a bunching phenomenon based on the bosonic nature of photons. When two photons that are perfectly indistinguishable from each other are mixed using a half beam splitter (HBS), they always bunch and exhibit the absence of coincidence resulting in a specific interferogram called HOM dip. The important property of the HOM interference is that the decrease in coincidence reflects the degree of indistinguishability of the input photons, i.e., it provides information regarding the probability of overlap of the input photons. Thus, this property should enable the estimation of a target photon in an unknown quantum state using a probe photon in a known state. In this work, we realize the above concept as the quantum state tomography (QST) applicable to d-dimensional photonic qudits, which we call HOM-QST [2]. Interestingly, we observe that HOM-QST is robust against various imperfections and that the probe photon can be replaced by classical light. Furthermore, we confirm this by demonstrating a proof-of-principle experiment using two-dimensional polarization qubits.
Quantum interference forces two indistinguishable input photons to depart a beamsplitter in the same (of two possible) spatial output modes; this is known as the Hong-Ou-Mandel (HOM) effect. It provides a quantitative way of measuring the distinguishability between two photons and also has been utilised to determine their relative temporal delays [1, 2]. HOM interferometry offers numerous advantages over its classical counterpart, most importantly it lacks any dependence on the phase of the photons and therefore can potentially provide reliable measurements in environments where the phase is unstable. To date there have been very few investigations on the precision that is achievable with HOM interferometry. Experiments with collinear geometries have yielded sensitivities as low as 0.1fs however these approaches are limited to measurements of birefringence and other polarisation dependent effects [3, 4], as the precision derives from the inherently stable shared path of the photon pairs. Typical non-shared path HOM interferometers exhibit resolution of roughly 1–3 fs (0.3–1 μm).
Quantum interference constitutes one of the sharpest divides between our classical intuition and the weirdness of the quantum world. Whenever there are multiple paths leading to the same outcome, it is the interplay of associated probability amplitudes that determines measurement results. In the double slit experiment, wave-like interference governs the distribution of particles on a detection screen. Extending to multiple particles allows behaviour that cannot be described by a classical wave, such as the bunching of photon pairs in Hong-Ou-Mandel interference. In both these examples, the ability to distinguish the interfering paths leads to degradation of interference and a return to behaviour described by probabilities. Understanding how this transition evolves for larger multiparticle quantum systems is of fundamental interest and also vital for developing photonic quantum technologies that rely on many-photon interference. In this thesis we investigate the role of distinguishability in the interference of three and four independent photons by using polarisation and time delays. For three photons, a new type of collective distinguishing phase appears that goes beyond a pairwise description of the similarity of quantum states. We use nonlinear photon sources and a fibre interferometer to experimentally demonstrate the ability to tune and isolate this phase in interference statistics. Extending to four photons we show that, contrary to intuition from two-photon experiments, the interference of photons prepared in distinguishable states is possible due to a four-particle phase. This is confirmed experimentally using a bulk four-mode interferometer. We then extend our study to include the effects of state impurity in the interference of three photons. New properties of this interference enable diagnosis of realistic experimental imperfections and characterisation tasks impossible using only two photons. Finally, we link discussions of state distinguishability to the group representations underpinning the exchange symmetry of multiparticle wavefunctions.
Hong-Ou-Mandel (HOM) interference [1] is a bunching phenomenon based on the bosonic nature of photons. When two photons that are perfectly indistinguishable from each other are mixed using a half beam splitter (HBS), they always bunch and exhibit the absence of coincidence resulting in a specific interferogram called HOM dip. The important property of the HOM interference is that the decrease in coincidence reflects the degree of indistinguishability of the input photons, i.e., it provides information regarding the probability of overlap of the input photons. Thus, this property should enable the estimation of a target photon in an unknown quantum state using a probe photon in a known state. In this work, we realize the above concept as the quantum state tomography (QST) applicable tod-dimensionald\text{-dimensional}d-dimensionalphotonic qudits, which we call HOM-QST [2]. Interestingly, we observe that HOM-QST is robust against various imperfections and that the probe photon can be replaced by classical light. Furthermore, we confirm this by demonstrating a proof-of-principle experiment using two-dimensional polarization qubits.
Metasurfaces provide a promising route for structuring light and generating holograms with designed amplitude, phase, and polarization profiles, leading to a versatile platform for integrating and constructing optical components beyond the conventional ones. At the same time, incorporating coincidence in imaging allows a high signal-to-noise ratio for imaging in very low light levels. As beneficial from the recent development in both metasurfaces and single-photon avalanche diode (SPAD) cameras, we combine the polarization-sensitive capability of metasurfaces with Hong-Ou-Mandel (HOM)-type interference in generating images with tailor-made two-photon interference and polarization coincidence signatures. By using orthogonal linear-polarized photons as incidence, correlated, anticorrelated, and uncorrelated polarization coincidence features can be observed within the same image from the pairwise second-order coherence statistics across different pixels of the image. Our work adds polarization to the demonstrated amplitude and phase sensitivity in the domain of "HOM microscopy" and can be useful for biological and security applications.
Earth, Moon and Sun unite when they star together in the three-body problem, whose intricate plot still baffles us today. For some reason, the factorization of the two-body problem into two one-body problems does not, in general, cross the N=2 border. Is computational irreducibility responsible for this emergence of complexity, as Stephen Wolfram likes to think? We don't know. The introduction to this thesis in Chapter 1, however, makes it clear that the history of science is marked by intermittent encounters of sudden complexities when the number 2 is left behind. In Chapter 2, I present an experiment that is quite similar in spirit, for my colleagues and I observe three-photon interference without two-photon and single-photon interference. We had to overcome significant experimental challenges that are typical for most quantum interference experiments involving more than two photons. Next in line is the three-slit interference experiment. Again a deceptively simple extension of the famous double-slit experiment, we are faced with questions that are difficult to access experimentally: the existence of genuine three-slit interference was first denied and then affirmed, though no experiment has decided yet. My contribution to the study of this problem is outlined in Chapter 3, where I use symmetry of measurement settings in such interference experiments to theoretically derive higher-order interference terms. In Chapter 4, I take a step back in one sense, for we study a two-photon phenomenon, but we also leap forward and discover entirely new interference landscapes. Theoretically and experimentally, I demonstrate how to use a polarization-modulated lasers to go beyond the standard Hong-Ou-Mandel (HOM) dip, and generate both triangular and square wave HOM interference patterns. Two-photon interference is also subject of Chapter 5, but with an interesting twist. While laser HOM interference relies on two independent photons, here we endow the pair with the strongest known correlations, namely entanglement. More specifically, we entangle a polarization and a time-bin qubit and use this hybrid to assess the viability of a rather special interferometer for quantum communication purposes.