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APL Photonics

Chip-scale atomic spectrometer with silicon nitride optical phased array

Jeremi Januszewicz, A. McWilliam, S. Dyer, J. P. McGilligan, Paul F. Griffin, Erling Riis, Eugenio Di Gaetano, Marc Sorel, Douglas J. Paul, Kevin Francis Gallacher

Published Jul 1, 2025• 12 citations
Publisher

Abstract

The integration of nanophotonic optical phased arrays (OPA) with alkali vapor cells has the potential to enhance the performance of chip-scale atomic systems by enabling novel methods for beam shaping and active alignment in atomic spectroscopy. In this work, we present the first demonstration of an OPA used for precision saturated absorption spectroscopy with a rubidium vapor cell integrated directly on the chip. The OPA, consisting of 64 emitters, expands a sub-micron waveguide mode into a >100 µm diameter free-space beam, optimized for the D2 absorption line of rubidium. We resolved the sub-Doppler hyperfine splittings in both 85Rb and 87Rb isotopes, achieving Lorentzian linewidths ranging from 25 to 40 MHz suitable for stabilizing the cooling lasers in rubidium cold atom systems.

DOI
10.1063/5.0273108

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•Jan 1, 2007•1 citation
The integration of nanophotonic optical phased arrays (OPA) with alkali vapor cells has the potential to enhance the performance of chip-scale atomic systems by enabling novel methods for beam shaping and active alignment in atomic spectroscopy. In this work, we present the first demonstration of an OPA used for precision saturated absorption spectroscopy with a rubidium vapor cell integrated directly on the chip. The OPA, consisting of 64 emitters, expands a sub-micron waveguide mode into a >100 µm diameter free-space beam, optimized for the D2 absorption line of rubidium. We resolved the sub-Doppler hyperfine splittings in both 85Rb and 87Rb isotopes, achieving Lorentzian linewidths ranging from 25 to 40 MHz suitable for stabilizing the cooling lasers in rubidium cold atom systems.
Devices based on spectroscopy of atomic vapors can measure physical quantities such as magnetic fields, RF electric fields, time and length, and rotation and have applications in a broad range of fields including communications, medicine, and navigation. We present a type of photonic device that interfaces single-mode silicon nitride optical waveguides with warm atomic vapors, enabling precision spectroscopy in an extremely compact (<1  cm3) package. We perform precision spectroscopy of rubidium confined in a micro-machined, 27  mm3 volume, vapor cell using a collimated free-space 120 μm diameter laser beam derived directly from a single-mode silicon nitride waveguide. With this optical-fiber integrated photonic spectrometer, we demonstrate an optical frequency reference at 780 nm with a stability of 10−11 from 1 to 104  s. This device harnesses the benefits of both photonic integration and precision spectroscopy for the next generation of quantum sensors and devices based on atomic vapors.
We demonstrate chip-scale sub-Doppler spectroscopy in an integrated and fiber-coupled photonic-metasurface device. The device is a stack of three planar components: a photonic mode expanding grating emitter circuit with a monolithically integrated tilt-compensating dielectric metasurface, a microfabricated atomic vapor cell, and a mirror. The metasurface photonic circuit efficiently emits a 130 μm wide (1/e2 diameter) collimated surface-normal beam with only −6.3 dB loss and couples the reflected beam back into the waveguide and connecting fiber, requiring no alignment between the stacked components. We develop a simple model based on light propagation through the photonic device to interpret the atomic spectroscopy signals and explain spectral features covering the full Rb hyperfine state manifold. The demonstration of waveguide-to-waveguide coupling through the vapor cell paves the way for atomic ensembles to be used as components in complex photonic integrated circuits, allowing the unique properties of atomic systems to be available for future highly miniaturized optical devices and systems.
This thesis presents the integration of atomic vapor cells with anti-resonant reflecting optical waveguides (ARROWs) fabricated on silicon chips. These potentially provide a compact platform for a number of optical applications, including the study of quantum coherence effects such as electromagnetically induced transparency and single-photon nonlinearities, as well as frequency stabilization standards. The use of hollow waveguides allows for light propagation in low index (vapor) media with compact mode areas. ARROWs make particularly attractive waveguides for this purpose because they can be interfaced with solid core waveguides, microfabricated on a planar substrate, and are effectively single mode. ARROW fabrication utilizes an acid-removed sacrificial core surrounded by alternating plasma deposited dielectric layers, which act as Fabry-Perot reflectors. To demonstrate the effectiveness of the ARROW as a vapor cell, a platform consisting of solid and hollow core waveguides integrated with rubidium vapor cells was developed. A variety of sealing techniques were tested for vapor cell integration with the ARROW chip and for compatibility with rubidium. Rubidium was used because it is of particular interest for studying quantum coherence effects. Liquefied rubidium was transferred from a bulk supply into an on-chip vapor cell in an anaerobic atmosphere glovebox. Optical absorption measurements confirmed the presence of rubidium vapor within the hollow waveguide platform. Further analysis of the measurements revealed high optical density of rubidium atoms in the hollow core. Saturated absorption spectroscopy measurements verified that the on-chip integrated vapor cell was suitable for common precision spectroscopy applications.