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Optica

Photonic chip for laser stabilization to an atomic vapor with 10−11 instability

Matthew T. Hummon, Songbai Kang, Douglas G. Bopp, Qing Li, Daron Westly, Sangsik Kim, Connor D. Fredrick, Scott A. Diddams, Kartik A. Srinivasan, Vladimir Aksyuk, John E. Kitching

Published Apr 10, 2018• 167 citations
Publisher

Abstract

Devices based on spectroscopy of atomic vapors can measure physical quantities such as magnetic fields, RF electric fields, time and length, and rotation and have applications in a broad range of fields including communications, medicine, and navigation. We present a type of photonic device that interfaces single-mode silicon nitride optical waveguides with warm atomic vapors, enabling precision spectroscopy in an extremely compact (<1  cm3) package. We perform precision spectroscopy of rubidium confined in a micro-machined, 27  mm3 volume, vapor cell using a collimated free-space 120 μm diameter laser beam derived directly from a single-mode silicon nitride waveguide. With this optical-fiber integrated photonic spectrometer, we demonstrate an optical frequency reference at 780 nm with a stability of 10−11 from 1 to 104  s. This device harnesses the benefits of both photonic integration and precision spectroscopy for the next generation of quantum sensors and devices based on atomic vapors.

DOI
10.1364/optica.5.000443

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Devices based on spectroscopy of atomic vapors can measure physical quantities such as magnetic fields, RF electric fields, time and length, and rotation and have applications in a broad range of fields including communications, medicine, and navigation. We present a type of photonic device that interfaces single-mode silicon nitride optical waveguides with warm atomic vapors, enabling precision spectroscopy in an extremely compact (<1  cm3) package. We perform precision spectroscopy of rubidium confined in a micro-machined, 27  mm3 volume, vapor cell using a collimated free-space 120 μm diameter laser beam derived directly from a single-mode silicon nitride waveguide. With this optical-fiber integrated photonic spectrometer, we demonstrate an optical frequency reference at 780 nm with a stability of 10−11 from 1 to 104  s. This device harnesses the benefits of both photonic integration and precision spectroscopy for the next generation of quantum sensors and devices based on atomic vapors.
The integration of nanophotonic optical phased arrays (OPA) with alkali vapor cells has the potential to enhance the performance of chip-scale atomic systems by enabling novel methods for beam shaping and active alignment in atomic spectroscopy. In this work, we present the first demonstration of an OPA used for precision saturated absorption spectroscopy with a rubidium vapor cell integrated directly on the chip. The OPA, consisting of 64 emitters, expands a sub-micron waveguide mode into a >100 µm diameter free-space beam, optimized for the D2 absorption line of rubidium. We resolved the sub-Doppler hyperfine splittings in both 85Rb and 87Rb isotopes, achieving Lorentzian linewidths ranging from 25 to 40 MHz suitable for stabilizing the cooling lasers in rubidium cold atom systems.
We investigate an integrated optical chip immersed in atomic vapor providing several waveguide geometries for spectroscopy applications. The narrow-band transmission through a silicon nitride waveguide and interferometer is altered when the guided light is coupled to a vapor of rubidium atoms via the evanescent tail of the waveguide mode. We use grating couplers to couple between the waveguide mode and the radiating wave, which allow for addressing arbitrary coupling positions on the chip surface. The evanescent atom-light interaction can be numerically simulated and shows excellent agreement with our experimental data. This work demonstrates a next step towards miniaturization and integration of alkali atom spectroscopy and provides a platform for further fundamental studies of complex waveguide structures.
Integrating alkali atomic vapors with nanophotonic devices offers a scalable route to quantum technologies that leverage strong atom–photon interactions. While there have been many approaches to such integration, the general reliance on traditional glass vapor cells, distilled alkali metals, and epoxy sealing limits reproducibility and scalability. Moreover, mitigating adverse Rb-photonics interactions is essential, particularly as devices become more compact and the alkali source lies in close proximity to the photonic elements. Here, we demonstrate the successful operation of compact and fully integrated devices that combine silicon nitride photonic integrated circuits (PICs) with microfabricated borosilicate vapor cells and pill-type rubidium (Rb) dispensers through hermetic seals via anodic bonding. We show how successful operation hinges on optically activating the dispenser in a low-power pulsed mode, releasing controlled amounts of Rb vapor on demand while mitigating photonic degradation. Simultaneously, a counter-propagating desorption laser completely suppresses Rb-induced losses and enables waveguide-based atomic vapor spectroscopy. Using this approach, we demonstrate repeatable control of vapor density by tuning activation pulse length, duty cycle, and device temperature. These results establish a compact, manufacturable, and scalable vapor–PIC device, and set the stage for future demonstrations in cavity quantum electrodynamics, quantum nonlinear optics, and chip-scale atomic sensors.
Integrating alkali atomic vapors with nanophotonic devices offers a scalable route to quantum technologies that leverage strong atom-photon interactions. While there have been many approaches to such integration, the general reliance on traditional glass vapor cells, distilled alkali metals, and epoxy sealing limits reproducibility and scalability. Moreover, mitigating adverse Rb-photonics interactions is essential, particularly as devices become more compact and the alkali source lies in close proximity to the photonic elements. Here, we demonstrate the successful operation of compact and fully integrated devices that combine silicon nitride photonic integrated circuits (PICs) with microfabricated borosilicate vapor cells and pill-type rubidium (Rb) dispensers through hermetic seals via anodic bonding. We show how successful operation hinges on optically activating the dispenser in a low-power pulsed mode, releasing controlled amounts of Rb vapor on demand while mitigating photonic degradation. Simultaneously, a counter-propagating desorption laser completely suppresses Rb-induced losses and enables waveguide-based atomic vapor spectroscopy. Using this approach, we demonstrate repeatable control of vapor density by tuning activation pulse length, duty cycle, and device temperature. These results establish a compact, manufacturable, and scalable vapor-PIC device, and set the stage for future demonstrations in cavity quantum electrodynamics, quantum nonlinear optics, and chip-scale atomic sensors.
Atomic spectroscopy relies on photons to probe the energy states of atoms, typically in a gas state. In addition to providing fundamental scientific information, this technique can be applied to a number of photonic devices including atomic clocks, laser stabilization references, slow light elements, and eventually quantum communications components. Atomic spectroscopy has classically been done using bulk optics and evacuated transparent vapor cells. Recently, a number of methods have been introduced to dramatically decrease the size of atomic spectroscopy systems by integrating optical functionality. We review three of these techniques including: 1) photonic crystal fiber based experiments, 2) wafer bonded mini-cells containing atomic vapors and integrated with lasers and detectors, and 3) hollow waveguides containing atomic vapors fabricated on silicon substrates. In the context of silicon photonics, we will emphasize the hollow waveguide platform. At the heart of these devices is the anti-resonant reflecting optical waveguide (ARROW). ARROW fabrication techniques will be described for both hollow and solid core designs. Solid-core waveguides are necessary to direct light on and off the silicon chip while confining atomic vapors to hollow-core waveguides. We will also discuss the methods and challenges of attaching rubidium vapor reservoirs to the chip. Experimental results for optical spectroscopy of rubidium atoms on a chip will be presented.
We investigate an integrated optical chip immersed in atomic vapor providing several waveguide geometries for spectroscopy applications. The narrow-band transmission through a silicon nitride waveguide and interferometer is altered when the guided light is coupled to a vapor of rubidium atoms via the evanescent tail of the waveguide mode. We use grating couplers to couple between the waveguide mode and the radiating wave, which allow for addressing arbitrary coupling positions on the chip surface. The evanescent atom-light interaction can be numerically simulated and shows excellent agreement with our experimental data. This work demonstrates a next step towards miniaturization and integration of alkali atom spectroscopy and provides a platform for further fundamental studies of complex waveguide structures.