Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Advanced Quantum Technologies

Optimizing Nitrogen Concentration and Temperature for Reducing Spin Relaxation in Spin‐Exchange Relaxation‐Free Co‐Magnetometers

Jiaxin Liu, Xusheng Lei, Wanqing Li, Yizhe Zhou, Yu Yuan

Published Apr 8, 2025• 4 citations
Publisher

Abstract

Abstract This study systematically investigates the spin relaxation characteristics of alkali‐metal atoms in spin‐exchange relaxation‐free (SERF) co‐magnetometers, focusing on mitigating the radiation trapping to reduce the alkali‐metal spin relaxation rate. Radiation trapping is one of the dominant mechanisms exacerbating spin relaxation in alkali‐metal atoms and is conventionally suppressed by introducing nitrogen () as a quenching agent. However, experiments reveal that the typical concentration in current SERF co‐magnetometers is insufficient to effectively suppress radiation trapping. By increasing the quenching gas concentration, additional attenuation of the radiation trapping effect is achieved. Meanwhile, to address the enhanced spin‐exchange collision relaxation arising from higher concentration, the operating temperature is adjusted to increase the alkali‐metal atom number density, thereby effectively curtailing this adverse effect. Experimental results demonstrate that the synergistic optimization of concentration and temperature reduces alkali‐metal spin relaxation by approximately 55% and decreases the noise power spectral density of the co‐magnetometer by 48.5% at 1 Hz. These findings confirm the effectiveness of this approach in improving the accuracy and sensitivity of SERF co‐magnetometers.

DOI
10.1002/qute.202500033

Related papers

Suppression of thermal coupling noise in the SERF atomic co-magnetometer

Jiasen Ruan, Lihong Duan, Yang Fu +4 more

Heating the alkali metal vapor cell to obtain high atomic density is a prerequisite for realizing the high-precision measurement for spin-exchange relaxation-free (SERF) co-magnetometer. However, the thermo-magnetic and thermo-optical coupling noise caused by the temperature diffusion from the alkali vapor cell is one of the main factors restricting the co-magnetometer performance at present. Here the influence of heating on the SERF co-magnetometer was comprehensively studied, and the thermal error model of the system was established. A novel heat insulation structure for the co-magnetometer was designed, and the effectiveness was verified through monitoring of characteristic temperature points. Compared to the conventional oven support, the average maximum temperature difference within 12 h of the optical path and magnetic shielding systems (OPMSS) decreased by 52%, the bias instability of the co-magnetometer decreased by 24%, and the noise of the co-magnetometer at 1 Hz decreased by 33%. The experimental results demonstrate that this method reduces the temperature fluctuation of the OPMSS, effectively suppresses the thermal coupling noise, and thus improves the performance of the SERF co-magnetometer. Moreover, this method is also applicable to other quantum sensors based on alkali metal vapor cell.

Results in Physics•Sep 22, 2023•14 citations

Enhancing Dynamic Performance in K-Rb-21Ne Co-Magnetometers through Atomic Density Optimization

Yang Lv, Haoying Pang, Wei Quan

The K-Rb-21Ne co-magnetometer exhibits poorer dynamic performance due to the larger equivalent magnetic field generated by alkali metal atoms. In this study, the impact of the atomic number density of alkali metal atoms and noble gas atoms in the cell on the dynamic performance of the atomic ensemble is investigated quantitatively. Relationships between the slow-decay term in the transient response attenuation of the Spin-Exchange Relaxation-Free (SERF) co-magnetometer to interference magnetic fields and the number densities of noble gas atoms as well as alkali metal atoms are established. Based on the established model, the relationship between the number density of 21Ne atoms and dynamic performance is investigated using cells with five different noble gas pressures. Then, we investigate the impact of the number density of alkali metal atoms using a cell with a pressure of 2.1 atm at different temperatures. The results indicate that, as the number density of alkali metal atoms or noble gas atoms in the cell increases, the dynamic performance of the system improves, which provides a theoretical basis for the design of cell parameters for SERF co-magnetometers.

Photonics•Feb 16, 2024•2 citations

Buffer Gas Pressure Optimization for Atomic Spin Relaxation Suppression in Ultra-High-Sensitivity SERF Magnetometers

Siran Li, X.-G. Lu, Yinghui Zhang +3 more

Optically pumped magnetometers (OPM) are core quantum payloads for geomagnetic remote sensing. Among them, the spin-exchange relaxation-free (SERF) OPM with aT-level ultimate sensitivity stands as mainstream. While enlarging the alkali-metal vapor cell of the SERF OPM enhances sensitivity, it triggers complex atomic spin relaxation, notably intensified magnetic field gradient relaxation. To address the dilemma of atomic spin relaxation regulation and the engineering requirements of ultra-high-sensitivity SERF magnetometers, this paper constructs an analytical model of the total relaxation rate that comprehensively considers wall-collision relaxation, spin-destruction collision relaxation, and longitudinal/transverse magnetic field gradient relaxation, etc. The analytical relationship between buffer gas pressure and total relaxation rate for a commonly used spherical vapor cell is derived, revealing the intrinsic correlation among cell size, atomic spin relaxation, and optimal pressure. Based on the theoretical model, the filling parameters of the vapor cell are optimized, and experimental measurements are carried out. The theoretical relaxation results are highly consistent with the experimental ones, realizing the precise optimization of buffer gas pressure. The optimization method proposed in this paper provides a theoretical basis and parameter guidance for the engineering preparation of alkali-metal vapor cells for high-sensitivity SERF magnetometers in remote sensing applications.

Photonics•Jun 1, 2026•0 citations

Effects of Stochastic Magnetic Noise on the SERF Co‐Magnetometer

Feng Li, Zhuo Wang, Wenfeng Fan +4 more

Abstract Stochastic magnetic field noise has a non‐negligible negative impact on the performance of quantum precision measurement instruments such as spin‐exchange relaxation‐free (SERF) co‐magnetometer in terms of sensitivity and stability. Conventional magnetic field error analysis and suppression methods are not applicable to stochastic magnetic field noise. In this paper, a stochastic model of the SERF co‐magnetometer is proposed to analyze the mechanism of stochastic magnetic field noise. The mean and covariance propagation model of the SERF co‐magnetometer is given based on the stochasticity model and statistical principles. The analysis of simulation experiments reveals that reducing the longitudinal electron spin polarization can somewhat reduce the standard deviation of the system output caused by stochastic magnetic field noise. And the atomic ensembles are most resistant to stochastic magnetic field noise when the electron spin polarization strongly couples with the nuclear spin polarization. Finally, the experiments verified the above conclusions. In conclusion, this paper provides theoretical and experimental support for analyzing and suppressing the effect of stochastic magnetic field noise on the SERF co‐magnetometer, which is of great significance for improving the sensitivity and stability of the measurement.

Advanced Quantum Technologies•Apr 19, 2024•6 citations

Examination of Spin-Exchange Relaxation in the Alkali Metal-Noble Gas Comagnetometer With a Large Electron Magnetic Field

Liwei Jiang, Lihong Duan, Jiali Liu +3 more

Alkali metal-noble gas comagnetometers operated in the regime of spin-exchange relaxation-free (SERF) have been widely used in fundamental physics tests and rotation sensing as gyroscope. Spin-exchange relaxation is an important systematic bias of the comagnetometer, which could limit sensitivity significantly. However, the suppression effect of the spin-exchange relaxation has not been examined quantitatively so far. Herein, we systematically investigate the relaxation of the alkali metal atoms and find that the spin-exchange relaxation is not completely eliminated under the normal operating condition of the K-Rb-21Ne comagnetometer. In addition to the optical pumping rate, the spin-exchange relaxation still plays a dominant role in the broadening of electron Zeeman resonances due to the large electron magnetic field. This is the first demonstration that the alkali metal atoms are operated in the near-SERF regime in the alkali metal-noble gas comagnetometer with a large election magnetic field, which will shed light on the way to reduce the relaxation of the alkali metal atoms and enhance the sensitivity of the comagnetometer.

IEEE Transactions on Instrumentation and Measurement•Oct 26, 2020•18 citations

Spin-exchange-relaxation-free magnetometry with Cs vapor

M. P. Ledbetter, Igor Savukov, Víctor M. Acosta +2 more

We describe a Cs atomic magnetometer operating in the spin-exchange-relaxation-free (SERF) regime. With a vapor cell temperature of $103\text{ }\ifmmode^\circ\else\textdegree\fi{}\text{C}$ we achieve intrinsic magnetic resonance widths $\ensuremath{\Delta}B=17\text{ }\ensuremath{\mu}\text{G}$ corresponding to an electron spin-relaxation rate of $300\text{ }{\text{s}}^{\ensuremath{-}1}$ when the spin-exchange rate is ${\ensuremath{\Gamma}}_{\text{SE}}=14\text{ }000\text{ }{\text{s}}^{\ensuremath{-}1}$. We also observe an interesting narrowing effect due to diffusion. Signal-to-noise measurements yield a sensitivity of about $400\text{ }\text{pG}/\sqrt{\text{Hz}}$. Based on photon shot noise, we project a sensitivity of $40\text{ }\text{pG}/\sqrt{\text{Hz}}$. A theoretical optimization of the magnetometer indicates sensitivities on the order of $2\text{ }\text{pG}/\sqrt{\text{Hz}}$ should be achievable in a $1\text{ }{\text{cm}}^{3}$ volume. Because Cs has a higher saturated vapor pressure than other alkali metals, SERF magnetometers using Cs atoms are particularly attractive in applications requiring lower temperatures.

arXiv:0708.1012•Physical Review A•Mar 13, 2008•400 citations
Abstract This study systematically investigates the spin relaxation characteristics of alkali‐metal atoms in spin‐exchange relaxation‐free (SERF) co‐magnetometers, focusing on mitigating the radiation trapping to reduce the alkali‐metal spin relaxation rate. Radiation trapping is one of the dominant mechanisms exacerbating spin relaxation in alkali‐metal atoms and is conventionally suppressed by introducing nitrogen () as a quenching agent. However, experiments reveal that the typical concentration in current SERF co‐magnetometers is insufficient to effectively suppress radiation trapping. By increasing the quenching gas concentration, additional attenuation of the radiation trapping effect is achieved. Meanwhile, to address the enhanced spin‐exchange collision relaxation arising from higher concentration, the operating temperature is adjusted to increase the alkali‐metal atom number density, thereby effectively curtailing this adverse effect. Experimental results demonstrate that the synergistic optimization of concentration and temperature reduces alkali‐metal spin relaxation by approximately 55% and decreases the noise power spectral density of the co‐magnetometer by 48.5% at 1 Hz. These findings confirm the effectiveness of this approach in improving the accuracy and sensitivity of SERF co‐magnetometers.
Heating the alkali metal vapor cell to obtain high atomic density is a prerequisite for realizing the high-precision measurement for spin-exchange relaxation-free (SERF) co-magnetometer. However, the thermo-magnetic and thermo-optical coupling noise caused by the temperature diffusion from the alkali vapor cell is one of the main factors restricting the co-magnetometer performance at present. Here the influence of heating on the SERF co-magnetometer was comprehensively studied, and the thermal error model of the system was established. A novel heat insulation structure for the co-magnetometer was designed, and the effectiveness was verified through monitoring of characteristic temperature points. Compared to the conventional oven support, the average maximum temperature difference within 12 h of the optical path and magnetic shielding systems (OPMSS) decreased by 52%, the bias instability of the co-magnetometer decreased by 24%, and the noise of the co-magnetometer at 1 Hz decreased by 33%. The experimental results demonstrate that this method reduces the temperature fluctuation of the OPMSS, effectively suppresses the thermal coupling noise, and thus improves the performance of the SERF co-magnetometer. Moreover, this method is also applicable to other quantum sensors based on alkali metal vapor cell.
The K-Rb-21Ne co-magnetometer exhibits poorer dynamic performance due to the larger equivalent magnetic field generated by alkali metal atoms. In this study, the impact of the atomic number density of alkali metal atoms and noble gas atoms in the cell on the dynamic performance of the atomic ensemble is investigated quantitatively. Relationships between the slow-decay term in the transient response attenuation of the Spin-Exchange Relaxation-Free (SERF) co-magnetometer to interference magnetic fields and the number densities of noble gas atoms as well as alkali metal atoms are established. Based on the established model, the relationship between the number density of 21Ne atoms and dynamic performance is investigated using cells with five different noble gas pressures. Then, we investigate the impact of the number density of alkali metal atoms using a cell with a pressure of 2.1 atm at different temperatures. The results indicate that, as the number density of alkali metal atoms or noble gas atoms in the cell increases, the dynamic performance of the system improves, which provides a theoretical basis for the design of cell parameters for SERF co-magnetometers.
Optically pumped magnetometers (OPM) are core quantum payloads for geomagnetic remote sensing. Among them, the spin-exchange relaxation-free (SERF) OPM with aT-level ultimate sensitivity stands as mainstream. While enlarging the alkali-metal vapor cell of the SERF OPM enhances sensitivity, it triggers complex atomic spin relaxation, notably intensified magnetic field gradient relaxation. To address the dilemma of atomic spin relaxation regulation and the engineering requirements of ultra-high-sensitivity SERF magnetometers, this paper constructs an analytical model of the total relaxation rate that comprehensively considers wall-collision relaxation, spin-destruction collision relaxation, and longitudinal/transverse magnetic field gradient relaxation, etc. The analytical relationship between buffer gas pressure and total relaxation rate for a commonly used spherical vapor cell is derived, revealing the intrinsic correlation among cell size, atomic spin relaxation, and optimal pressure. Based on the theoretical model, the filling parameters of the vapor cell are optimized, and experimental measurements are carried out. The theoretical relaxation results are highly consistent with the experimental ones, realizing the precise optimization of buffer gas pressure. The optimization method proposed in this paper provides a theoretical basis and parameter guidance for the engineering preparation of alkali-metal vapor cells for high-sensitivity SERF magnetometers in remote sensing applications.
Abstract Stochastic magnetic field noise has a non‐negligible negative impact on the performance of quantum precision measurement instruments such as spin‐exchange relaxation‐free (SERF) co‐magnetometer in terms of sensitivity and stability. Conventional magnetic field error analysis and suppression methods are not applicable to stochastic magnetic field noise. In this paper, a stochastic model of the SERF co‐magnetometer is proposed to analyze the mechanism of stochastic magnetic field noise. The mean and covariance propagation model of the SERF co‐magnetometer is given based on the stochasticity model and statistical principles. The analysis of simulation experiments reveals that reducing the longitudinal electron spin polarization can somewhat reduce the standard deviation of the system output caused by stochastic magnetic field noise. And the atomic ensembles are most resistant to stochastic magnetic field noise when the electron spin polarization strongly couples with the nuclear spin polarization. Finally, the experiments verified the above conclusions. In conclusion, this paper provides theoretical and experimental support for analyzing and suppressing the effect of stochastic magnetic field noise on the SERF co‐magnetometer, which is of great significance for improving the sensitivity and stability of the measurement.
Alkali metal-noble gas comagnetometers operated in the regime of spin-exchange relaxation-free (SERF) have been widely used in fundamental physics tests and rotation sensing as gyroscope. Spin-exchange relaxation is an important systematic bias of the comagnetometer, which could limit sensitivity significantly. However, the suppression effect of the spin-exchange relaxation has not been examined quantitatively so far. Herein, we systematically investigate the relaxation of the alkali metal atoms and find that the spin-exchange relaxation is not completely eliminated under the normal operating condition of the K-Rb-21Ne comagnetometer. In addition to the optical pumping rate, the spin-exchange relaxation still plays a dominant role in the broadening of electron Zeeman resonances due to the large electron magnetic field. This is the first demonstration that the alkali metal atoms are operated in the near-SERF regime in the alkali metal-noble gas comagnetometer with a large election magnetic field, which will shed light on the way to reduce the relaxation of the alkali metal atoms and enhance the sensitivity of the comagnetometer.
We describe a Cs atomic magnetometer operating in the spin-exchange-relaxation-free (SERF) regime. With a vapor cell temperature of $103\text{ }\ifmmode^\circ\else\textdegree\fi{}\text{C}$ we achieve intrinsic magnetic resonance widths $\ensuremath{\Delta}B=17\text{ }\ensuremath{\mu}\text{G}$ corresponding to an electron spin-relaxation rate of $300\text{ }{\text{s}}^{\ensuremath{-}1}$ when the spin-exchange rate is ${\ensuremath{\Gamma}}_{\text{SE}}=14\text{ }000\text{ }{\text{s}}^{\ensuremath{-}1}$. We also observe an interesting narrowing effect due to diffusion. Signal-to-noise measurements yield a sensitivity of about 400 pG/Hz400\text{ }\text{pG}/\sqrt{\text{Hz}}400 pG/Hz​. Based on photon shot noise, we project a sensitivity of 40 pG/Hz40\text{ }\text{pG}/\sqrt{\text{Hz}}40 pG/Hz​. A theoretical optimization of the magnetometer indicates sensitivities on the order of 2 pG/Hz2\text{ }\text{pG}/\sqrt{\text{Hz}}2 pG/Hz​ should be achievable in a 1 cm31\text{ }{\text{cm}}^{3}1 cm3 volume. Because Cs has a higher saturated vapor pressure than other alkali metals, SERF magnetometers using Cs atoms are particularly attractive in applications requiring lower temperatures.