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Optics & Laser Technology

Optically pumped magnetometers based on symmetric frequency-detuning modulated light

Yifan Yan, Zehua Liu, Yuesong Wu, Xinsheng Ding, Min Xiang, Yaxiang Wang, Jixi Lu

Published Mar 22, 2025• 9 citations
Publisher
DOI
10.1016/j.optlastec.2025.112833

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The frequency drifts of the probe laser could be coupled into the calibrated scale factor of the optically pumped magnetometer (OPM) and induce an error of the measurement accuracy. We propose a method to reduce the far off-resonance laser frequency drifts based on the second harmonic of the electro-optic modulator (EOM) detection system in the all-optical K-Rb hybrid pumping magnetometer. Adopting the closed-loop feedback by monitoring the second-harmonic component in real time, the frequency drift of the probe laser has been effectively reduced by about five times to ∼30 MHz/0.5 h at the detuning of 130 GHz and the cell temperature of 443 K. Besides, this technique has been demonstrated to be helpful for reducing the frequency drifts at different detuning points and temperatures. This method is not only suitable for the development of more compact, high-sensitivity OPMs due to the long-term stability improvement with no extra optical path, but also can be applied to other atomic devices and EOM detection systems for reducing the influence of the laser.
The ultrasensitive magnetometer has a vital importance in fundamental research and applications. Currently, the spin-exchange relaxation-free (SERF) atomic magnetometer has been reported with a sensitivity around the level of fT/Hz 1/2 . To enhance the sensitivity, a gradiometer configuration has usually been introduced to cancel the common-mode noise between two separate channels. However, the signal and response from different channels are not the same due to the attenuation of the pump beam. Here, we proposed a counter-propagating optical sideband pumping method to polarize the atoms, using the electro-optic modulator to modulate the single-pump beam, generating two symmetrically red- and blue-detuned sidebands of frequency. This scheme leads to a significant reduction of undesirable effects coming along with the optical pumping, such as light shifts and spatial inhomogeneity in atomic spin polarization. With the help of this pumping scheme, the two channels have the same magnetic response, and we have built a gradiometer atomic magnetometer with a sensitivity of 0.5 fT/Hz 1/2 ranging from 5 to 40 Hz. Our results propose the possibility of creating larger arrays of atomic magnetometers (AMs) with high sensitivity and spatial resolution based on single-vapor cells for magnetocardiography and magnetoencephalography imaging or searching for exotic spin-dependent interactions.
In recent years, arrayed atomic magnetometers have been continuously applied in biomagnetic scenarios. However, the crosstalk between adjacent sensors introduced by the modulated magnetic fields significantly compromises the imaging accuracy of arrayed atomic magnetometers. To solve this problem, a detuned square-wave optical modulation zero-field atomic magnetometer configuration is developed and we provide an analytical solution of this method. In this scheme, the circularly polarized pump light is used to polarize alkali metal atoms longitudinally, and a beam of detuned square-wave modulated circularly polarized light is applied transversely to generate a light-shift modulation instead of the coil-generated modulated magnetic field. Then the transverse magnetic field is measured by the optical absorption method of longitudinally circularly polarized pump light. This scheme maintains the inherent advantage of high sensitivity in spinexchange relaxation-free (SERF) atomic magnetometers. Additionally, the all-optical configuration eliminates the need for additional modulated magnetic fields or radio frequency (RF) fields, thereby mitigating crosstalk issues associated with modulated magnetic fields in array applications. Consequently, this scheme exhibits great potential for arraying and is expected to be employed in magnetocardiography (MCG) and magnetoencephalography (MEG).