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Acta Physica Sinica

A method of modulating spin-polarized states with high spatiotemporal resolution in alkali-metal atomic vapor cell

Donghui Ma, HE Xinxin, HUA Zeyu, Yanjun Li, Dong Haifeng, Huan Fei Wen, Yasuhiro Sugawara, Tang Jun, Ma Zongmin, Jun Liu

Published Jan 1, 2025• 2 citations
Publisher

Abstract

With the state-of-the-art quantum measurement devices, such as atomic clocks, atomic gyroscopes, and atomic magnetometers, as their central components, the spatiotemporal evolution of atomic spin polarization in the atomic vapor cell has a major effect on both increasing the bandwidth of magnetometer and improving the accuracy of magnetic gradient measurements. However, the major factor impeding the further improvement of the performance of quantum measurement instrument is the inherent static nature of the traditional intra-vapor cell segmentation imaging technique, which makes it challenging to achieve the real-time capture of the dynamic evolution of atomic spin states. In this work, we suggest a dynamic spin imaging method for alkali metal atomic vapor cells with real-time modification of atomic spin polarization states in order to overcome this technological difficulty. In particular, to ensure that the laser can precisely act on the alkali metal atoms in various regions in the vapor cell, we employ a complex beam array management system to modify the on/off state of the laser beams at various positions in the spatial dimension in real time. In the meantime, we generate laser fields with particular spatial distribution and frequency characteristics by using frequency modulation techniques in the time series to accurately regulate the on-off frequency of each laser beam in the beam array. These laser beams cause dynamic changes in the atomic spin polarization state by interacting with alkali metal atoms at various points in the vapor cell. Through precise adjustment of the laser properties, we can see and study the dynamic evolution of the atomic spin-polarization state in real time. According to the experimental data, the technology outperforms the traditional static spin imaging techniques by achieving an excellent temporal resolution of 355 frames per second and a spatial resolution of 95.9 micrometers. The effective use of this method enables us to monitor and evaluate the dynamic aspects of magnetic field distribution with unprecedented precision, also greatly enhance our understanding of the dynamic characteristics of atomic spin polarization.

DOI
10.7498/aps.74.20241634

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With the state-of-the-art quantum measurement devices, such as atomic clocks, atomic gyroscopes, and atomic magnetometers, as their central components, the spatiotemporal evolution of atomic spin polarization in the atomic vapor cell has a major effect on both increasing the bandwidth of magnetometer and improving the accuracy of magnetic gradient measurements. However, the major factor impeding the further improvement of the performance of quantum measurement instrument is the inherent static nature of the traditional intra-vapor cell segmentation imaging technique, which makes it challenging to achieve the real-time capture of the dynamic evolution of atomic spin states. In this work, we suggest a dynamic spin imaging method for alkali metal atomic vapor cells with real-time modification of atomic spin polarization states in order to overcome this technological difficulty. In particular, to ensure that the laser can precisely act on the alkali metal atoms in various regions in the vapor cell, we employ a complex beam array management system to modify the on/off state of the laser beams at various positions in the spatial dimension in real time. In the meantime, we generate laser fields with particular spatial distribution and frequency characteristics by using frequency modulation techniques in the time series to accurately regulate the on-off frequency of each laser beam in the beam array. These laser beams cause dynamic changes in the atomic spin polarization state by interacting with alkali metal atoms at various points in the vapor cell. Through precise adjustment of the laser properties, we can see and study the dynamic evolution of the atomic spin-polarization state in real time. According to the experimental data, the technology outperforms the traditional static spin imaging techniques by achieving an excellent temporal resolution of 355 frames per second and a spatial resolution of 95.9 micrometers. The effective use of this method enables us to monitor and evaluate the dynamic aspects of magnetic field distribution with unprecedented precision, also greatly enhance our understanding of the dynamic characteristics of atomic spin polarization.
A laser beam with left-/right-handed circular polarization is generally used to create the oriented atomic spins for precision measurements in a spin-exchange relaxation-free (SERF) co-magnetometer. The fluctuation of laser polarization interferes with the spin polarization of alkali metal atoms, leading to the system performance degradation. Here, we report a method for real-time polarization state measurement by using the transmitted light intensity of the pump beam passing through the vapor cell. Based on the principle of circular dichroism, the optical absorption model of polarized alkali metal atoms is established. The simulation results of the transmittance of the pump laser with different polarization states through the alkali metal vapor cell are given and verified by experiments. The experimental results show that the circularly polarized beam has the weakest absorption, while the linearly polarized laser beam is absorbed the strongest. The achieved measurement accuracy stands at an impressive 98.83 %. This work provides a simple and easy-to-use way to measure the polarization state of the laser beam used in the vapor cell devices, particularly the microfabricated prototypes with limited space.
The atomic density of an alkali vapor cell is a critical factor in determining the performance of atomic magnetometers. This paper presents a novel method to detect the density of an alkali atomic ensemble under arbitrary polarization states. By establishing a comprehensive model that correlates the absorption spectrum with the incident light’s polarization, our approach enables real-time and flexible measurements across varying temperatures and polarization angles. Experimental validations are conducted by systematically rotating a quarter-wave plate and controlling the vapor cell temperature, thereby collecting transmission spectra at multiple polarizations. The results demonstrate that the proposed method simplifies density measurements while preserving high accuracy, laying a solid foundation for further research on Spin-Exchange Relaxation-Free (SERF) atomic magnetometers. This technique serves as a versatile and effective tool for in-situ monitoring of alkali metal vapor density in various sensor applications.
Abstract In an optically pumped alkali vapor cell with a high density of atoms, the attenuation of the pump light generates a spatially non-uniform distribution of the electronic spin polarization of alkali atoms, which is detrimental to biomagnetism applications of magnetometers as well as the hyperpolarization of noble gas atoms. Therefore, in this study, we propose a new scheme to generate a nearly uniform, unsaturated spin polarization region based on counter-propagating pump beams and atomic diffusion. A finite element method-based simulation is used to demonstrate the three-dimensional distribution of the spin polarization in a spherical cell. The effects of cell temperature and pump light power on the homogeneity of the spin polarization are studied. The distribution of spin polarization near the center of the cell is experimentally measured and a 1 cm uniform spin polarization region is achieved in the center of the cell. The uniformity of spin polarization in the center region of the cell increased by 50% compared with single beam pumping. The advantage of our proposed scheme is that it can generate an unsaturated uniform region of spin polarization in the center of a cell using a single species of alkali atoms.
The number density of alkali atoms in vaper cell is an important parameter for atomic magnetometer. The vapor cell is usually heated to a high temperature for the number density exceed to 1018m−3to achieve the spin-exchange-relaxation-free (SERF) process. The optical rotation of multichannel atomic magnetometers is affected by the number density distribution. We present an effective method for monitoring and analyzing the spatial distribution homogeneity of the atomic number density in the alkali metal cell within the SERF magnetometer. The numerical results from researching the model of electric heating films and ovens show that the temperature gradient increases with an increase in the cell temperature. This causes an nonuniform number density distribution based on the saturated vapor pressure curve. We present a laser absorption spectroscopy method by using the high-resolution beam profiling camera to record the power of the beam before and after the cell. An optimized optical system of the atomic magnetometer has been established by measuring the the number density variation in the spatial distribution in mm scale. The number density variation coefficient, which is introduced to evaluate the distribution homogeneity, increases from 0.0257 to 0.0333 when the temperature of the oven wall rises from 140°C to 190 °C, showing the same trend as the simulation results. The optical rotation distribution is calculated according to the magnetometer output signal formula. This study is of great interest for optimizing the oven structure and improving the stability of atomic spin polarization and sensitivity of the multichannel magnetometer.
High sensitivity measurements of inertia and magnetic field could be achieved by utilizing a category of devices, which manipulate the atomic spins in the spin-exchange-relaxation-free regime. The alkali cell which contains the alkali metal vapor is used to sense magnetic field and inertia. The atomic number density of alkali vapor and the polarization of alkali metal vapor are two of the most important parameters of the cell. They play an important role in the research on atomic spins in the spin-exchange-relaxation-free regime. Besides, optical polarization plays an important role in quantum computing and atomic physics. We propose a measurement of alkali vapor polarization and alkali number density by detecting the optical rotation in one system. This method simplifies existing experimental equipment and processes. A constant bias magnetic field is applied and the Faraday rotation angle is detected by a bunch of the probe beam to deduce alkali-metal density. Then the magnetic field is closed and a bunch of the pump laser is utilized to polarize alkali-metal. Again, the probe beam is utilized to obtain the polarization of alkali metal. The alkali density obtained at first is used to deduce the polarization. This paper applies a numerical method to analyze the Faraday rotation and the polarization rotation. According to the numerical method, the optimal wavelength for the experiment is given. Finally, the fluctuation of magnetic field and wavelength on signal analysis are analyzed.
We measured the spatial homogeneity of spin polarization, which is directly related to the sensitivity and magnetic linewidth of an optically pumped atomic magnetometer with a hybrid cell of K and Rb atoms. This was done by changing the position of the probe beam. Furthermore, for comparison, we also measured the sensitivity and magnetic linewidth of atomic magnetometers with single K and single Rb cells, and found that optically thick atoms were spin polarized homogeneously with the hybrid cell. Optically thin alkali metal vapor can be spin polarized homogeneously, and the spin polarization transfers to an optically thick alkali metal vapor. An atomic magnetometer with the hybrid cell was found to be more effective in realizing simultaneous signal measurements at different locations with the uniform sensitivity and magnetic linewidth.