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Physical Review Letters

Dipole Moment of a Superatom

Bijun Yang, Y. Li, Saiwei Nie, Yefeng Mei, Huy Minh Nguyen, P. R. Berman, A. Kuzmich

Published Nov 19, 2024• 3 citations
Publisher

Abstract

Homodyne detection is used to measure the (collective) atomic dipole moment for an atomic ensemble that is prepared in a superposition of spatially phased Dicke states having at most two excitations (a so-called "superatom"). Homodyne detection allows one to isolate the contributions to the radiated intensity that depend linearly on the average value of the collective atomic dipole moment operator. Depending on whether the atom-reference field interference is constructive or destructive, either super-Poisson or sub-Poisson statistics for the combined field is observed.

DOI
10.1103/physrevlett.133.213601

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Homodyne detection is used to measure the (collective) atomic dipole moment for an atomic ensemble that is prepared in a superposition of spatially phased Dicke states having at most two excitations (a so-called "superatom"). Homodyne detection allows one to isolate the contributions to the radiated intensity that depend linearly on the average value of the collective atomic dipole moment operator. Depending on whether the atom-reference field interference is constructive or destructive, either super-Poisson or sub-Poisson statistics for the combined field is observed.
Quantum information is a rapidly developing field that merges the principles of quantum mechanics with information theory to explore new ways of processing and transmitting information. Qubits, which utilize superposition and entanglement, offer the potential for exponentially faster computation and secure communication methods that are fundamentally different from classical systems. This thesis contributes to the future of quantum information by studying two key platforms using neutral atoms: atomic arrays and atomic ensembles. It summarizes essential theoretical and experimental methods in the field and discusses key findings. To achieve entanglement among atomic qubits, Rydberg interactions are utilized, with two main effects discussed in this thesis. The Rydberg blockade effect is introduced where atoms trapped in an ensemble can form a two-level superatom. A state-insensitive optical lattice is used to achieve long coherence time for both the ground and Rydberg states. Long-lived Rabi oscillations and Ramsey interference are reported to demonstrate the collective enhancement of √N in a superatom. Furthermore, Rydberg dephasing is separated from Rydberg blockade and is investigated as a method to generate single photons from multiply excited states. This thesis presents both theoretical models and temporal evolution measurements of Rydberg dephasing from an initially unentangled Rydberg spinwave into an entangled single photon state. Additionally, this thesis examines the collective atomic dipole moment of a superatom, ⟨E⟩. Theoretical and experimental work are conducted to study the dipole moment when the phase-matched emission is combined with a coherent field in a homodyne detection method. This work advances our understanding of Rydberg interactions and collective dipole moments, contributing to the rapidly developing field of quantum information. The goal is to pave the way for the next era of quantum information through collaborative efforts and innovative research.
Information carried by an optical beam of light can usually be conveyed in the form of a temporal modulation of the intensity, phase, frequency or the polarization of the constituent mode(s). In that regard, homodyne detection is one of the most popular and standard method to measure the quantum mechanical properties of light Yuen & Shapiro (1978); Yuen et al. (1979); Yuen & Shapiro (1980); Yurke (1985). The quantum theory of homodyne detection originated principally from the works of Yuen and Shapiro et al. Yuen & Shapiro (1978); Yuen et al. (1979). In this method, a weak signal field is combined with a strong local oscillator field at a beam splitter, and the resulting signal is measured as a photocurrent. With the homodyne detection method, the quantum state of the signal field, such as the quadrature amplitude of the squeezed state, is easily measured Slusher et al. (1985); Wu et al. (1986 ); Polzik et al. (1992), and the quasiprobability distribution function can be measured by using the so-called optical homodyne tomography Smithey et al. (1993); Banaszek & W’odkiewicz (1996); Wallentowitz & Vogel (1996); Youn et al. (2001). Furthermore, optical homodyne detection is used to eavesdrop on the quantum key in quantum cryptography Hirano et al. (2000).
Owing to the unique physical characteristics of Rydberg atoms, which play an important role in quantum information and quantum computation, the theoretical and applied research of Rydberg atoms have become the hot spots of scientific research in recent years. With the large polarizability of Rydberg atoms, even a small electric field could cause a considerable electric dipole moment, resulting in a strong dipole-dipole interaction between Rydberg atoms. The multiple excitations of the Rydberg states are strongly inhibited because of the strong dipole interaction between atoms within a mesoscopic interaction (blockade) region. We call this phenomenon the dipole blockade effect. The dipole blockade effect makes it possible to build single-photon quantum devices, implement quantum gates, generate quantum entanglement, and simulate many-body quantum problems, etc. A Rydberg atomic ensemble in the same blockade region can be regarded as a superatom. In the same way, if these atoms trapped in two optical dipole traps, each sub-ensemble can be considered as a sub-superatom which is closely related to the superatom. According to the fact that two Rydberg sub-superatoms can be strongly correlated due to sharing no more than one excited Rydberg atom, we study correlated collective excitation and quantum entanglement between two Rydberg sub-superatoms in a steady state. With the superatom model, the problem of exponentially increasing system size with the number of atoms can be circumvented to a certain extent in studying many-body physics. By solving the two-body Lindblad’s master equation accurately, we obtain the analytical expressions for the collective excitation probabilities of the two sub-superatoms, and the concurrence measuring the bipartite entanglement between them. Our results show that they are all sensitive to the number of atoms in each Rydberg superatom: the bigger (including more atoms) the Rydberg superatom, the higher the collective Rydberg excitation probability is. And that the maximally entangled state can only be obtained with two equal-sized Rydberg superatoms. When this condition is fulfilled, the mesoscopic entanglement can be generated by adding the number of atoms in each Rydberg superatom. This may provide an attractive platform for studying the quantum-classical correspondence and have potential promising applications in quantum information processing.
Dicke superradiance, i.e., the enhanced spontaneous emission of coherent radiation, is often attributed to radiation emitted by synchronized dipoles coherently oscillating in phase. At the same time, Dicke derived superradiance assuming atoms in entangled Dicke states which do not display any dipole moment. To shed light on this apparent paradox, we study the intensity distribution arising from two identical two-level atoms prepared either in an entangled Dicke state or in a separable atomic state with a nonvanishing dipole moment. We find that the two configurations produce similar far-field intensity patterns, although they stem from fundamentally distinct types of coherence: while in the second case the atoms display coherence among the individual particles, leading to Young-type interference like that known from classical dipoles, atoms in Dicke states possess collective quantum coherence stemming from entanglement and quantum correlations of the state, leading to an interference pattern resulting from enhanced spontaneous emission. This demonstrates that the radiation generated by synchronized dipoles and Dicke superradiance---even if they do produce the same interference pattern---are fundamentally distinct phenomena and have to be interpreted in different ways.