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SPIE Quantum Technologies for Defence and Security

Metrology of RF electromagnetic fields using trap loss spectroscopy in cold Rydberg atoms

Romain Duverger, Sylvain Schwartz

Published Nov 15, 2024• 0 citations
Publisher

Abstract

Due to their high sensitivity, wide frequency range, SI-traceability and reduced size at low frequency, Rydberg atoms based- sensors of RF/THz fields hold great prospects for many applications including telecommunications, radar, and THz imaging. So far, almost all of these sensors have consisted in probing by means of EIT spectroscopy the Autler-Townes effect resulting from the interaction between the field and a warm vapor of alkaline Rydberg atoms. Despite significant improvement using heterodyning, this approach suffers several limitations caused by broadening mechanisms inherent to warm vapors, and by using EIT as a probe. We report here on a new approach based on trap-loss spectroscopy of the Autler-Townes effect in cold 87Rb atoms confined in a MOT. The doublet of dressed Rydberg states measured this way obeys well the theoretical model of Autler-Townes effect provided lightshifts from neighboring Rydberg states are considered, suggesting the possibility to infer the characteristics of the field from those of the doublet. Study of the resulting sensor revealed a very good linearity, with residual errors of 1%, and a resolution of 5 µV/cm after an integration time of 2600s.

DOI
10.1117/12.3031688

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Due to their high sensitivity, wide frequency range, SI-traceability and reduced size at low frequency, Rydberg atoms based- sensors of RF/THz fields hold great prospects for many applications including telecommunications, radar, and THz imaging. So far, almost all of these sensors have consisted in probing by means of EIT spectroscopy the Autler-Townes effect resulting from the interaction between the field and a warm vapor of alkaline Rydberg atoms. Despite significant improvement using heterodyning, this approach suffers several limitations caused by broadening mechanisms inherent to warm vapors, and by using EIT as a probe. We report here on a new approach based on trap-loss spectroscopy of the Autler-Townes effect in cold 87Rb atoms confined in a MOT. The doublet of dressed Rydberg states measured this way obeys well the theoretical model of Autler-Townes effect provided lightshifts from neighboring Rydberg states are considered, suggesting the possibility to infer the characteristics of the field from those of the doublet. Study of the resulting sensor revealed a very good linearity, with residual errors of 1%, and a resolution of 5 µV/cm after an integration time of 2600s.
We investigate the relationship between the Rabi frequency (ΩRF, related to the applied electric field) and Autler-Townes (AT) splitting, when performing atom-based radio-frequency (RF) electric (E) field strength measurements using Rydberg states and electromagnetically induced transparency (EIT) in an atomic vapor. The AT splitting satisfies, under certain conditions, a well-defined linear relationship with the applied RF field amplitude. The EIT/AT-based E-field measurement approach derived from these principles is currently being investigated by several groups around the world as a means to develop a new SI-traceable RF E-field measurement technique. We establish conditions under which the measured AT-splitting is an approximately linear function of the RF electric field. A quantitative description of systematic deviations from the linear relationship is key to exploiting EIT/AT-based atomic-vapor spectroscopy for SI-traceable field measurement. We show that the linear relationship is valid and can be used to determine the E-field strength, with minimal error, as long as the EIT linewidth is small compared to the AT-splitting. We also discuss interesting aspects of the thermal dependence (i.e., hot- versus cold-atom) of this EIT-AT technique. An analysis of the transition from cold- to hot-atom EIT in a Doppler-mismatched cascade system reveals a significant change of the dependence of the EIT linewidth on the optical Rabi frequencies and of the AT-splitting on ΩRF.
Rydberg atoms are neutral atoms excited to high principal quantum number states, which endows them with exaggerated properties such as large electric dipole moments, long lifetimes, and extreme sensitivity to external electromagnetic fields. These characteristics form the foundation of Rydberg atom-based sensors, an emerging class of quantum devices capable of optically detecting electric fields across frequencies from DC to the terahertz regime. Rydberg-based electrometry operates through both Autler–Townes (AT) splitting of resonant Rydberg transitions and Stark-shift measurements for high-frequency or far-detuned fields, enabling broadband field sensing from DC to the THz regime. Using ladder-type electromagnetically induced transparency (EIT) and AT splitting, these sensors enable non-invasive, SI-traceable measurements of field amplitude, frequency, phase, and polarization. Recent developments have demonstrated broadband electric field probes, voltage calibration standards, and compact RF receivers based on thermal vapor cells and integrated photonic architectures. Furthermore, innovations in multi-photon EIT, superheterodyne readout, and multi wave mixing have expanded the dynamic range and bandwidth of Rydberg-based electrometry. Despite challenges related to environmental perturbations, linewidth broadening, and laser stabilization, ongoing advances in atomic control, hybrid photonic integration, and EIT-based readout promise scalable, chip-compatible sensors. This review summarizes the physical principles, experimental progress, and emerging applications of Rydberg atom-based sensing, emphasizing their potential for next generation quantum metrology, wireless communication, and precision field mapping.
We discuss a fundamentally new method for electric (E) field strength (V/m) metrology applicable to the near-field. This new approach is significantly different from currently used field measurement techniques in that it is based on the interaction of radio-frequency (RF) E-fields with Rydberg atoms (alkali atoms placed in a glass vapor cell that are excited optically to Rydberg states). The applied RF E-field alters the state of the atoms. The Rydberg atoms act like an RF-to-optical transducer, converting an RF E-field strength to an optical-frequency response. In this new approach, we employ the phenomena of electromagnetically induced transparency (EIT) and Autler-Townes splitting. The RF transition in the four-level atomic system causes a split of the EIT transmission spectrum of a probe laser into two peaks. This splitting is easily measured and is directly proportional to the applied RF E-field amplitude. The significant dipole response of Rydberg atoms enables this technique to make self-calibrating measurements over a large frequency band including 500 MHz to 500 GHz (and possibly up to 1 THz and down to 10s of megahertz). In this paper, we report on our results in the development of this metrology approach, including the first fiber-coupled vapor-cell for E-field measurements. We also discuss key applications, including self-calibrated measurements, millimeter-wave and sub-THz measurements, field mapping, and sub-wavelength and near-field imaging. We show results for mapping the fields inside vapor cells, for measuring the E-field distribution along the surface of a circuit board, and for measuring the near-field at the aperture in a cavity. We also discuss the uncertainties of this measurement technique.
Atom-based radio-frequency (RF) electric field probes have the potential to improve electric field measurements for a broad range of frequencies (from a few GHz to 100s of GHz) and field strengths (mV/m to kV/m). For these probes to become a common measurement method, their range must be extended to high frequency (>100 GHz) and low field strength regimes. We present SI-traceable electric field measurements of RF fields above 100 GHz, using Autler-Townes splitting of Rydberg electromagnetically-induced transparency in a rubidium (Rb) vapor. We also demonstrate several techniques, including RF detuning from resonance and enhanced absorption, for increasing the probe sensitivity.
Rydberg atoms have been used for measuring radio-frequency (RF) electric (E)-fields due to their strong dipole moments over the frequency range of 500 MHz-1 THz. For this, electromagnetically induced transparency (EIT) within the Autler-Townes (AT) regime is used such that the detected E-field is proportional to AT splitting. However, for weak E-fields AT peak separation becomes unresolvable thus limiting the minimum detectable E-field. Here, we demonstrate using the Rydberg atoms as an RF mixer for weak E-field detection well below the AT regime with frequency discrimination better than 1 Hz resolution. A heterodyne detection scenario with two E-fields incident on a vapor cell filled with cesium atoms is used. One E-field at 19.626000 GHz drives the 34D5/2 → 35P3/2 Rydberg transition and acts as a local oscillator (LO) and a second signal E-field (Sig) of interest is at 19.626090 GHz. In the presence of the LO, the Rydberg atoms naturally down convert the Sig field to a 90 kHz intermediate frequency (IF) signal. This IF signal manifests as an oscillation in the probe laser intensity through the Rydberg vapor and is easily detected with a photodiode and lock-in amplifier. In the configuration used here, E-field strength down to ≈ 46 μV/m ± 2 μV/m were detected with a sensitivity of ≈ 79 μVm−1Hz−1/2. Furthermore, neighboring fields 0.1 Hz away and equal in strength to Sig could be discriminated without any leakage into the lock-in signal. For signals 1 Hz away and as high as +60 dB above Sig, leakage into the lock-in signal could be kept below -3 dB.
Significant progress has been made in atom-based measurements of length, time, gravity and electromagnetic fields in recently years. Rydberg atom-based microwave electric field measurement, using electromagnetically induced transparency (EIT) in room temperature alkali-metal vapors, has been extensively investigated and aroused the broad interest. This approach may establish a new standard for the measurements of microwave (MW) and radio frequency (RF) electric fields.In this review, we describe the work on a new method of measuring electric fields based on quantum interference by using either cesium or rubidium atoms contained in a dielectric vapor cell. Rydberg atoms with principal quantum number n >>1 have large direct current (DC) polarizabilities and microwave transition dipole moments, thereby making them extremely sensitive to external electric fields. Using the Rydberg three-level EIT to detect the level splitting and shift that is induced by the external field, we can realize a rapid and robust self-calibration method of measuring the electric field in a frequency range from 0.01 GHz to 1000 GHz. For the MW electric field (frequency range > 1 GHz), the MW field causes the Rydberg states to split, known as an Autler-Townes splitting (A-T) effect when the applied microwave can resonate with adjacent Rydberg states. The MW coupled A-T splitting is proportional to the applied electric field strength, from which the field strength is measured. Using the EIT window, a high sensitivity of 3 μV·cm-1·Hz-1/2 and small electric field of 1 μV/cm are expected to be achieved with a modest setup, and the limitations of the sensitivity are also addressed in the review. For the RF field at frequency mj EIT lines, and avoided crossings formed with the fine-structure levels of equal mj and different J's, which is used to calibrate and measure the RF field amplitude. On the other hand, the dependence of the EIT-line strength on the RF field polarization provides a fast and robust polarization measurement of RF fields based on matching experimental data with a theoretical simulation. The measurements of minimum strengths and sensitivity of RF fields based on Rydberg atoms are one order magnitude below the values obtained by traditional antenna methods. The atom-based field measurement paves the way for determining fields through calibration-free, invariable atomic properties and miniaturization. We also propose its various potential applications in the future.